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Local ordering in disordered NdxZr1-xO2-0.5x pyrochlore as observed using neutron total scattering

Journal Article · · Acta Materialia
 [1];  [2];  [3];  [4];  [2]
  1. Univ. of Tennessee, Knoxville, TN (United States); University of Tennessee
  2. Univ. of Tennessee, Knoxville, TN (United States)
  3. Univ. of California, Irvine, CA (United States)
  4. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Pyrochlore complex oxides (A2B2O7) are an important class of fluorite-derivative ceramics with exceptional chemical and structural versatility which make them ideal model systems for studying disordering mechanisms over a range of spatial scales. Here, neutron total scattering methods were used to analyze the structural behavior in the non-stoichiometric series NdxZr1-xO2-0.5x (0.5 ≤ x ≤ 0.23) as a function of Nd content, x. Characterization of the structure functions using Rietveld refinement and the pair distribution functions with small-box refinement reveal complex disordering pathways; the average, long-range phase changes over a very narrow compositional range from pyrochlore ($$Fd\bar{3}m$$) to defect fluorite ($$Fm\bar{3}m$$) through full randomization of the cation and anion sublattices at x ~ 0.31, while the local, short-range structure continuously adopts a weberite-type atomic arrangement (C2221). Comparison to a previously studied Ho2Ti2-xZrxO7 solid solution series reveals how changes in chemical composition and stoichiometry modify defect formation and determine how disordering progresses across different length scales in pyrochlore oxides.
Research Organization:
Univ. of Tennessee, Knoxville, TN (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
SC0020321
OSTI ID:
1846455
Journal Information:
Acta Materialia, Journal Name: Acta Materialia Vol. 225; ISSN 1359-6454
Publisher:
ElsevierCopyright Statement
Country of Publication:
United States
Language:
English

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