Perspective: multi-dimensional coherent spectroscopy of perovskite nanocrystals

Liu, Albert; Almeida, Diogo B.; Padilha, Lazaro A.; Cundiff, Steven T.

doi:10.1088/2515-7639/ac4fa5

Perspective: multi-dimensional coherent spectroscopy of perovskite nanocrystals

Journal Article · Wed Feb 09 23:00:00 EST 2022 · JPhys Materials

DOI:https://doi.org/10.1088/2515-7639/ac4fa5· OSTI ID:1844012

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Abstract

Recently, colloidal perovskite nanocrystals (PNCs) have emerged as an exciting material platform for optoelectronic applications due to their combination of facile synthesis routes, quantum size effects, and exceptional optical properties among other favorable characteristics. Given the focus on their optoelectronic properties, spectroscopic characterization of PNCs is crucial to rational design of their structure and device implementation. In this Perspective, we discuss how multi-dimensional coherent spectroscopy (MDCS) can resolve exciton dynamics and circumvent inhomogeneous broadening to reveal underlying homogeneous spectral lineshapes. We highlight recent applications of MDCS to PNCs in the literature, and suggest compelling problems concerning their microscopic physics to be addressed by MDCS in the future.

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Sponsoring Organization:: USDOE

Grant/Contract Number:: SC0015782

OSTI ID:: 1844012

Alternate ID(s):: OSTI ID: 1842549

Journal Information:: JPhys Materials, Journal Name: JPhys Materials Journal Issue: 2 Vol. 5; ISSN 2515-7639

Publisher:: IOP PublishingCopyright Statement

Country of Publication:: United Kingdom

Language:: English

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