Polaronic correlations and phonon renormalization in La1–xSrxMnO3(x = 0.2, 0.3)

Maschek, M.; Castellan, J. -P.; Lamago, D.; Reznik, Dmitry; Weber, F.

doi:10.1103/physrevb.97.245139

Polaronic correlations and phonon renormalization in La_1–xSr_xMnO₃(x = 0.2, 0.3)

Journal Article · Mon Jun 25 00:00:00 EDT 2018 · Physical Review. B

DOI:https://doi.org/10.1103/physrevb.97.245139· OSTI ID:1842510

Maschek, M. ^[1]; Castellan, J. -P. ^[2]; Lamago, D. ^[2]; ^[3]; Weber, F. ^[4]

Karlsruhe Inst. of Technology (KIT) (Germany); Delft Univ. of Technology (Netherlands); University of Colorado Boulder, Dept. of Physics
Karlsruhe Inst. of Technology (KIT) (Germany); Laboratoire Léon Brillouin (CEA-CNRS), Gif-sur-Yvette (France)
Univ. of Colorado, Boulder, CO (United States)
Karlsruhe Inst. of Technology (KIT) (Germany)

According to standard theory the magnetoresistance magnitude in ferromagnetic manganites crucially depends on the electron-phonon coupling strength. We showed that in La_0.7Sr_0.3MnO₃ the phonon renormalization is strong, despite its relatively small magnetoresistance. Here, we report results of a similar inelastic neutron-scattering investigation of a closely related compound, La_0.8Sr_0.2MnO₃, where the magnetoresistance is enhanced. We find similar phonon renormalization and dynamic CE-type polaron correlations as in La_0.7Sr_0.3MnO₃. Furthermore, quantitative comparison of the results for the two samples shows that only polaron lifetime is well correlated with the strength of the colossal magnetoresistance.

View Accepted Manuscript (DOE)

Research Organization:: Univ. of Colorado, Boulder, CO (United States)

Sponsoring Organization:: USDOE; USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0006939

OSTI ID:: 1842510

Alternate ID(s):: OSTI ID: 1540885
OSTI ID: 1457075

Journal Information:: Physical Review. B, Journal Name: Physical Review. B Journal Issue: 24 Vol. 97; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

References (29)

Critical Features of Colossal Magnetoresistive Manganites Tokura, Y. ChemInform, Vol. 37, Issue 35 https://doi.org/10.1002/chin.200635250	journal	August 2006
Wide colossal magnetoresistance around room temperature in La0.7Ca0.3MnO3/La0.7Sr0.3MnO3 composite Hong, Chang Seop; Kim, Wan Seop; Hur, Nam Hwi Solid State Communications, Vol. 121, Issue 12 https://doi.org/10.1016/S0038-1098(02)00065-0	journal	March 2002
Anomalous features in the bond stretching vibrations of La1−xSrxMnO3 Reichardt, W.; Braden, M. Physica B: Condensed Matter, Vol. 263-264 https://doi.org/10.1016/S0921-4526(98)01400-8	journal	March 1999
Signature of checkerboard fluctuations in the phonon spectra of a possible polaronic metal La1.2Sr1.8Mn2O7 Weber, F.; Aliouane, N.; Zheng, H. Nature Materials, Vol. 8, Issue 10 https://doi.org/10.1038/nmat2513	journal	August 2009
Ferromagnetism and electron-phonon coupling in the manganites Edwards, D. M. Advances in Physics, Vol. 51, Issue 5 https://doi.org/10.1080/00018730210140805	journal	July 2002
Critical features of colossal magnetoresistive manganites Tokura, Y. Reports on Progress in Physics, Vol. 69, Issue 3 https://doi.org/10.1088/0034-4885/69/3/R06	journal	February 2006
Stability of polyatomic molecules in degenerate electronic states - I—Orbital degeneracy Jahn, H. A.; Teller, E. Proceedings of the Royal Society of London. Series A - Mathematical and Physical Sciences, Vol. 161, Issue 905, p. 220-235 https://doi.org/10.1098/rspa.1937.0142	journal	July 1937
Neutron Diffraction Study of the Magnetic Properties of the Series of Perovskite-Type Compounds [ ( 1 − x ) La , x Ca ] Mn O 3 Wollan, E. O.; Koehler, W. C. Physical Review, Vol. 100, Issue 2 https://doi.org/10.1103/PhysRev.100.545	journal	October 1955
Theory of the Role of Covalence in the Perovskite-Type Manganites [ La , M ( II ) ] Mn O 3 Goodenough, John B. Physical Review, Vol. 100, Issue 2 https://doi.org/10.1103/PhysRev.100.564	journal	October 1955
Insulator-metal transition and giant magnetoresistance in La 1 − x Sr x MnO 3 Urushibara, A.; Moritomo, Y.; Arima, T. Physical Review B, Vol. 51, Issue 20 https://doi.org/10.1103/PhysRevB.51.14103	journal	May 1995
Charge, orbital, and magnetic ordering in La 0.5 Ca 0.5 MnO 3 s Radaelli, P. G.; Cox, D. E.; Marezio, M. Physical Review B, Vol. 55, Issue 5 https://doi.org/10.1103/PhysRevB.55.3015	journal	February 1997
Small-polaron hopping conduction in bilayer manganite La 1.2 Sr 1.8 Mn 2 O 7 Chen, X. J.; Zhang, C. L.; Almasan, C. C. Physical Review B, Vol. 67, Issue 9 https://doi.org/10.1103/PhysRevB.67.094426	journal	March 2003
Large lattice distortions associated with the magnetic transition in La 0.7 Sr 0.3 MnO 3 Weber, F.; Argyriou, D. N.; Prokhnenko, O. Physical Review B, Vol. 88, Issue 24 https://doi.org/10.1103/PhysRevB.88.241106	journal	December 2013
Polaronic metal phases in L a 0.7 S r 0.3 Mn O 3 uncovered by inelastic neutron and x-ray scattering Maschek, M.; Lamago, D.; Castellan, J. -P. Physical Review B, Vol. 93, Issue 4 https://doi.org/10.1103/PhysRevB.93.045112	journal	January 2016
Response of Acoustic Phonons to Charge and Orbital Order in the 50% Doped Bilayer Manganite LaSr 2 Mn 2 O 7 Weber, F.; Rosenkranz, S.; Castellan, J. -P. Physical Review Letters, Vol. 107, Issue 20 https://doi.org/10.1103/PhysRevLett.107.207202	journal	November 2011
Giant negative magnetoresistance in perovskitelike La 2 / 3 Ba 1 / 3 MnO x ferromagnetic films von Helmolt, R.; Wecker, J.; Holzapfel, B. Physical Review Letters, Vol. 71, Issue 14 https://doi.org/10.1103/PhysRevLett.71.2331	journal	October 1993
Double Exchange Alone Does Not Explain the Resistivity of La 1 − x Sr x MnO 3 Millis, A. J.; Littlewood, P. B.; Shraiman, B. I. Physical Review Letters, Vol. 74, Issue 25 https://doi.org/10.1103/PhysRevLett.74.5144	journal	June 1995
Low Temperature Magnetoresistance and the Magnetic Phase Diagram of La 1 − x Ca x MnO 3 Schiffer, P.; Ramirez, A. P.; Bao, W. Physical Review Letters, Vol. 75, Issue 18 https://doi.org/10.1103/PhysRevLett.75.3336	journal	October 1995
Dynamic Jahn-Teller Effect and Colossal Magnetoresistance in La 1 − x Sr x MnO 3 Millis, A. J.; Shraiman, Boris I.; Mueller, R. Physical Review Letters, Vol. 77, Issue 1 https://doi.org/10.1103/PhysRevLett.77.175	journal	July 1996
Short-Range Polaron Correlations in the Ferromagnetic La 1 − x Ca x MnO 3 Dai, Pengcheng; Fernandez-Baca, J. A.; Wakabayashi, N. Physical Review Letters, Vol. 85, Issue 12 https://doi.org/10.1103/PhysRevLett.85.2553	journal	September 2000
Charge Ordering and Polaron Formation in the Magnetoresistive Oxide La 0.7 Ca 0.3 MnO 3 Adams, C. P.; Lynn, J. W.; Mukovskii, Y. M. Physical Review Letters, Vol. 85, Issue 18 https://doi.org/10.1103/PhysRevLett.85.3954	journal	October 2000
Glass Transition in the Polaron Dynamics of Colossal Magnetoresistive Manganites Argyriou, D. N.; Lynn, J. W.; Osborn, R. Physical Review Letters, Vol. 89, Issue 3 https://doi.org/10.1103/PhysRevLett.89.036401	journal	July 2002
Reentrant Orbital Order and the True Ground State of LaSr 2 Mn 2 O 7 Li, Qing’An; Gray, K. E.; Zheng, H. Physical Review Letters, Vol. 98, Issue 16 https://doi.org/10.1103/PhysRevLett.98.167201	journal	April 2007
Thousandfold Change in Resistivity in Magnetoresistive La-Ca-Mn-O Films Jin, S.; Tiefel, T. H.; McCormack, M. Science, Vol. 264, Issue 5157 https://doi.org/10.1126/science.264.5157.413	journal	April 1994
Giant Magnetotransport Phenomena in Filling-Controlled Kondo Lattice System: La _{1- x} Sr _x MnO ₃ Tokura, Yoshinori; Urushibara, Akira; Moritomo, Yutaka Journal of the Physical Society of Japan, Vol. 63, Issue 11 https://doi.org/10.1143/JPSJ.63.3931	journal	November 1994
Reentrant Orbital Order and the True Ground State of LaSr2Mn2O7 Li, Qing'An; Gray, K. E.; Zheng, H. arXiv https://doi.org/10.48550/arxiv.0704.1929	text	January 2007
Signature of checkerboard fluctuations in the phonon spectra of a possible polaronic metal La1.2Sr1.8Mn2O7 Weber, F.; Aliouane, N.; Zheng, H. arXiv https://doi.org/10.48550/arxiv.1001.4636	text	January 2010
Short-range polaron correlations in the ferromagnetic La(1-x)Ca(x)MnO(3) Dai, Pengcheng; Fernandez-Baca, J. A.; Wakabayashi, N. arXiv https://doi.org/10.48550/arxiv.cond-mat/0008303	text	January 2000
Ferromagnetism and electron-phonon coupling in the manganites Edwards, D. M. arXiv https://doi.org/10.48550/arxiv.cond-mat/0201558	text	January 2002

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Polaronic correlations and phonon renormalization in La1–xSrxMnO3(x = 0.2, 0.3)

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References (29)

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