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Characterization of single-shot attosecond pulses with angular streaking photoelectron spectra

Journal Article · · Physical Review A
 [1];  [2];  [2];  [3];  [4];  [2];  [2];  [3]
  1. Kansas State Univ., Manhattan, KS (United States); , Atomic, Molecular, and Optical Sciences Chemical Sciences, Geosciences, and Biosciences Division Office of Basic Energy Sciences U.S. Department of Energy
  2. SLAC National Accelerator Lab., Menlo Park, CA (United States)
  3. Kansas State Univ., Manhattan, KS (United States)
  4. Missouri Univ. of Science and Technology, Rolla, MO (United States)
Most of the traditional attosecond pulse retrieval algorithms are based on a so-called attosecond streak camera technique, in which the momentum of the electron is shifted by an amount depending on the relative time delay between the attosecond pulse and the streaking infrared pulse. Thus, temporal information of the attosecond pulse is encoded in the amount of momentum shift in the streaked photoelectron momentum spectrogram S(p,τ), where p is the momentum of the electron along the polarization direction and τ is the time delay. An iterative algorithm is then employed to reconstruct the attosecond pulse from the streaking spectrogram. This method, however, cannot be applied to attosecond pulses generated from free-electron x-ray lasers where each single shot is different and stochastic in time. However, using a circularly polarized infrared laser as the streaking field, a two (or three)-dimensional angular streaking electron spectrum can be used to retrieve attosecond pulses for each shot, as well as the time delay with respect to the circularly polarized IR field. Here we show that a retrieval algorithm previously developed for the traditional streaking spectrogram can be modified to efficiently characterize single-shot attosecond pulses. The methods have been applied to retrieve 188 single shots from recent experiments. We analyze the statistical behavior of these 188 pulses in terms of pulse duration, bandwidth, pulse peak energy, and time delay with respect to the IR field. Furthermore, the retrieval algorithm is efficient and can be easily used to characterize a large number of shots in future experiments for attosecond pulses at free-electron x-ray laser facilities.
Research Organization:
Kansas State Univ., Manhattan, KS (United States); SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Office of Science (SC), Basic Energy Sciences (BES). Chemical Sciences, Geosciences & Biosciences Division
Grant/Contract Number:
AC02-76SF00515; FG02-86ER13491
OSTI ID:
1841367
Alternate ID(s):
OSTI ID: 1862042
Journal Information:
Physical Review A, Journal Name: Physical Review A Journal Issue: 1 Vol. 105; ISSN 2469-9926
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English

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