Opportunities in electrically tunable 2D materials beyond graphene: Recent progress and future outlook

Vincent, Tom; Liang, Jiayun; Singh, Simrjit; Castanon, Eli G.; Zhang, Xiaotian; McCreary, Amber; Jariwala, Deep; Kazakova, Olga; Al Balushi, Zakaria Y.

doi:10.1063/5.0051394

Title: Opportunities in electrically tunable 2D materials beyond graphene: Recent progress and future outlook

Journal Article · Tue Nov 30 00:00:00 EST 2021 · Applied Physics Reviews

DOI:https://doi.org/10.1063/5.0051394· OSTI ID:1833108

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The interest in two-dimensional and layered materials continues to expand, driven by the compelling properties of individual atomic layers that can be stacked and/or twisted into synthetic heterostructures. The plethora of electronic properties as well as the emergence of many different quasiparticles, including plasmons, polaritons, trions, and excitons with large, tunable binding energies that all can be controlled and modulated through electrical means, has given rise to many device applications. In addition, these materials exhibit both room-temperature spin and valley polarization, magnetism, superconductivity, piezoelectricity that are intricately dependent on the composition, crystal structure, stacking, twist angle, layer number, and phases of these materials. Initial results on graphene exfoliated from single bulk crystals motivated the development of wide-area, high purity synthesis and heterojunctions with atomically clean interfaces. Now by opening this design space to new synthetic two-dimensional materials “beyond graphene,” it is possible to explore uncharted opportunities in designing novel heterostructures for electrically tunable devices. To fully reveal the emerging functionalities and opportunities of these atomically thin materials in practical applications, this review highlights several representative and noteworthy research directions in the use of electrical means to tune these aforementioned physical and structural properties, with an emphasis on discussing major applications of beyond graphene 2D materials in tunable devices in recent years and an outlook of what is to come in the next decade.

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Sponsoring Organization:: USDOE

Grant/Contract Number:: AC02- 05CH11231

OSTI ID:: 1833108

Journal Information:: Applied Physics Reviews, Journal Name: Applied Physics Reviews Vol. 8 Journal Issue: 4; ISSN 1931-9401

Publisher:: American Institute of PhysicsCopyright Statement

Country of Publication:: United States

Language:: English

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