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The In Situ Ion Irradiation Toolbox: Time-Resolved Structure and Property Measurements

Journal Article · · JOM. Journal of the Minerals, Metals & Materials Society

Abstract

The dynamic interactions of ions with matter drive a host of complex evolution mechanisms, requiring monitoring on short spatial and temporal scales to gain a full picture of a material response. Understanding the evolution of materials under ion irradiation and displacement damage is vital for many fields, including semiconductor processing, nuclear reactors, and space systems. Despite materials in service having a dynamic response to radiation damage, typical characterization is performed post-irradiation, washing out all information from transient processes. Characterizing active processes in situ during irradiation allows the mechanisms at play during the dynamic ion-material interaction process to be deciphered. In this review, we examine the in situ characterization techniques utilized for examining material structure, composition, and property evolution under ion irradiation. Covering analyses of microstructure, surface composition, and material properties, this work offers a perspective on the recent advances in methods for in situ monitoring of materials under ion irradiation, including a future outlook examining the role of complementary and combined characterization techniques in understanding dynamic materials evolution.

Sponsoring Organization:
USDOE National Nuclear Security Administration (NNSA), Office of Defense Nuclear Nonproliferation
Grant/Contract Number:
AC07-05ID14517
OSTI ID:
1832495
Alternate ID(s):
OSTI ID: 1834323
Journal Information:
JOM. Journal of the Minerals, Metals & Materials Society, Journal Name: JOM. Journal of the Minerals, Metals & Materials Society Journal Issue: 1 Vol. 74; ISSN 1047-4838
Publisher:
Springer Science + Business MediaCopyright Statement
Country of Publication:
United States
Language:
English

References (133)

Plasma-Assisted Approaches in Inorganic Nanostructure Fabrication journal March 2010
In situ Raman monitoring of materials under irradiation: study of uranium dioxide alteration by water radiolysis journal May 2012
Monitoring of the microstructure of ion-irradiated nuclear ceramics by in situ Raman spectroscopy : Microstructure of ion-irradiated nuclear ceramics journal December 2015
In Situ Positron Annihilation Spectroscopy Analysis on Low‐Temperature Irradiated Semiconductors, Challenges and Possibilities journal August 2020
High Energy Heavy Ion Irradiation of Silicon journal August 1989
Using ellipsometry for the evaluation of surface damage and sputtering yield in organic films with irradiation of argon cluster ion beams journal May 2010
The photon‐ion merged‐beams experiment PIPE at PETRA III—The first five years journal April 2019
Electron beam damage during testing of wood in the SEM journal January 1989
In situ TEM investigation of self-ion irradiation of nanoporous gold journal January 2019
In situ Evidence of Defect Cluster Absorption by Grain Boundaries in Kr Ion Irradiated Nanocrystalline Ni journal February 2013
An in situ field-ion microscope study of the recovery behavior of ion-irradiated tungsten and tungsten alloys journal January 1980
The irradiation creep of nickel and AISI 321 stainless steel during 4 MeV proton bombardment journal March 1977
Surface acoustic waves in the study of ion implanted surface layers journal April 1981
A review of the analysis of surfaces and thin films by AES and XPS journal March 1984
Change of electrical properties of alloys and excitation of low-temperature atom mobility by ion bombardment
  • Ovchinnikov, V. V.; Chernoborodov, V. I.; Ignatenko, Yu. G.
  • Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 103, Issue 3 https://doi.org/10.1016/0168-583X(95)00603-6
journal November 1995
Experimental study by “in situ” resistivity measurements of swift heavy ion induced defects in GaAs crystals journal February 1996
Development of ion irradiation system for in situ observation of ion irradiated semiconductor surfaces by ultra high vacuum scanning tunneling microscope journal July 1996
Radiation Damage Using Ion Beams book January 2012
Microstructure evolution in tungsten during low-energy helium ion irradiation journal December 2000
Accumulation and thermal recovery of disorder in Au2+-irradiated SrTiO3 journal February 2001
In-situ observation of damage evolution in SiC crystals during He+ and H2+ dual-ion beam irradiation journal September 1992
Irradiation-induced amorphization in β-SiC journal March 1998
Two-beam irradiation chamber for in situ ion-implantation and RBS at temperatures from 15 K to 300 K journal March 2001
A role for ion implantation in quantum computing journal April 2001
Ion implantation of semiconductors journal September 1998
Single- and dual-beam in situ irradiations of high-purity iron in a transmission electron microscope: Effects of heavy ion irradiation and helium injection journal February 2014
In situ Resonant Ultrasound Spectroscopy during irradiation of solids with relativistic heavy ions journal May 2015
In situ studies on radiation tolerance of nanotwinned Cu journal June 2016
Unprecedented irradiation resistance of nanocrystalline tungsten with equiaxed nanocrystalline grains to dislocation loop accumulation journal February 2019
Irradiation induced creep in nanocrystalline high entropy alloys journal January 2020
In situ microstructural evolution in face-centered and body-centered cubic complex concentrated solid-solution alloys under heavy ion irradiation journal October 2020
In-situ TEM study of irradiation-induced damage mechanisms in monoclinic-ZrO2 journal October 2020
Suppressing irradiation induced grain growth and defect accumulation in nanocrystalline tungsten through grain boundary doping journal March 2021
The dynamic evolution of swelling in nickel concentrated solid solution alloys through in situ property monitoring journal December 2021
Application of near-ambient pressure X-ray photoelectron spectroscopy (NAP-XPS) in an in-situ analysis of the stability of the surface-supported metal-organic framework HKUST-1 in water, methanol and pyridine atmospheres journal February 2021
Effect of ion irradiation on current–voltage characteristics of Au/n-GaN Schottky diodes journal July 2009
In situ FTIR study of photocatalytic NO reaction on photocatalysts under UV irradiation journal January 2006
Damage microstructure evolution of helium ion irradiated SiC under fusion relevant temperatures journal September 2018
Vacancy-type defect production in iron under ion beam irradiation investigated with positron beam Doppler broadening technique journal August 2004
Luminescence characteristics and defect formation in silica glasses under H and He ion irradiation journal August 2007
Degradation of reflectivity in stainless steel mirrors under irradiation with low-energy helium ions journal April 2009
In situ proton irradiation-induced creep at very high temperature journal February 2013
Radiation damage in nanocrystalline Ni under irradiation studied using positron annihilation spectroscopy journal November 2013
In situ proton irradiation creep of ferritic–martensitic steel T91 journal October 2013
In situ probing of the evolution of irradiation-induced defects in copper journal August 2013
Helium bubble formation in ultrafine and nanocrystalline tungsten under different extreme conditions journal March 2015
The role of grain size in He bubble formation: Implications for swelling resistance journal February 2017
Irradiation-induced creep in metallic nanolaminates characterized by In situ TEM pillar nanocompression journal July 2017
Effect of He implantation on the microstructure of zircaloy-4 studied using in situ TEM journal September 2017
In-situ TEM study of radiation-induced amorphization and recrystallization of hydroxyapatite journal December 2018
Multi-axial and multi-energy channeling study of disorder evolution in ion-irradiated nickel journal November 2019
Radiation damage in uranium dioxide: Coupled effect between electronic and nuclear energy losses journal April 2020
The influence of solute on irradiation damage evolution in nanocrystalline thin-films journal January 2021
In-situ ion irradiation induced grain growth in nanocrystalline ceria journal March 2021
Positron annihilation spectroscopy of defects in nuclear and irradiated materials- a review journal April 2021
Radiation damage in the TEM and SEM journal August 2004
Ion beam irradiation of phase change materials: A route to material properties investigation and engineering journal November 2021
Porosity inspection in directed energy deposition additive manufacturing based on transient thermoreflectance measurement journal September 2021
The CLEAR user facility at CERN
  • Gamba, D.; Corsini, R.; Curt, S.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 909 https://doi.org/10.1016/j.nima.2017.11.080
journal November 2018
In situ luminescence as monitor of radiation damage under swift heavy ion irradiation
  • Skuratov, V. A.; Gun, Kim Jong; Stano, J.
  • Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 245, Issue 1 https://doi.org/10.1016/j.nimb.2005.11.100
journal April 2006
A review of transmission electron microscopes with in situ ion irradiation journal December 2009
In-situ probing of near and below sputter-threshold ion-induced nanopatterning on GaSb(100) journal February 2012
The new Sandia light ion microbeam journal February 2012
Tailoring surface topographies of polymers by using ion beam: Recent advances and the potential applications in biomedical and tissue engineering
  • Hasebe, Terumitsu; Nagashima, So; Yoshimoto, Yukihiro
  • Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 282 https://doi.org/10.1016/j.nimb.2011.08.066
journal July 2012
In situ positron beam Doppler broadening measurement of ion-irradiated metals – Current status and potential journal August 2012
In situ RBS measurements for the effect of swift heavy ion irradiation on metal–insulator interfaces journal November 2013
New ion beam materials laboratory for materials modification and irradiation effects research journal November 2014
Ionoluminescence analysis of glass scintillators and application to single-ion-hit real-time detection journal March 2016
Ionoluminescence of fused silica under swift ion irradiation journal September 2016
In situ characterization of irradiation-induced microstructural evolution in urania single crystals at 773 K journal November 2018
Investigation of chemical changes in PMMA induced by 1.6 MeV He+ irradiation by ion beam analytical methods (RBS-ERDA) and infrared spectroscopy (ATR-FTIR) journal July 2019
Effect of ballistic damage in UO2 samples under ion beam irradiations studied by in situ Raman spectroscopy journal November 2018
Real-time thermomechanical property monitoring during ion beam irradiation using in situ transient grating spectroscopy
  • Dennett, Cody A.; Buller, Daniel L.; Hattar, Khalid
  • Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 440 https://doi.org/10.1016/j.nimb.2018.10.025
journal February 2019
Investigating radiation damage in nuclear energy materials using JANNuS multiple ion beams journal May 2019
SIGMA: A Set-up for In-situ Growth, Material modification and Analysis by ion beams journal January 2020
In-situ measurement of irradiation behavior in LiNbO3
  • Sha, Gaofeng; Harlow, Cole; Chernatynskiy, Aleksandr
  • Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 472 https://doi.org/10.1016/j.nimb.2020.03.007
journal June 2020
A combined thermomechanical and radiation testing platform for a 6 MV tandem accelerator
  • Briggs, Samuel A.; Steckbeck, Mackenzie; Heckman, Nathan M.
  • Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 509 https://doi.org/10.1016/j.nimb.2021.08.011
journal December 2021
Changes in surface morphology of helium-induced tungsten nanostructure during high-temperature annealing journal January 2020
Radiation damage in nanostructured materials journal July 2018
Swift heavy ion induced structural, iono and photoluminescence properties of β-CaSiO3:Dy3+ nanophosphor journal July 2012
An in situ transmission electron microscopy study of the ion irradiation induced amorphisation of silicon by He and Xe journal March 2016
Exploring Coupled Extreme Environments via In-situ Transmission Electron Microscopy journal January 2021
Percolation of Ion-Irradiation-Induced Disorder in Complex Oxide Interfaces journal June 2021
Effect of Irradiation Sources and Oxygen Concentration on the Photocatalytic Oxidation of 2-Propanol and Acetone Studied by in Situ FTIR journal May 2003
Irradiation of olivine by 4 keV He + : Simulation of space weathering by the solar wind journal January 2009
Ultrastrong nanocrystalline steel with exceptional thermal stability and radiation tolerance journal December 2018
Defect and structural evolution under high-energy ion irradiation informs battery materials design for extreme environments journal September 2020
A new resolution quest in electron microscopy journal December 2020
Direct Observation of Sink-Dependent Defect Evolution in Nanocrystalline Iron under Irradiation journal May 2017
In situ study of defect migration kinetics in nanoporous Ag with enhanced radiation tolerance journal January 2014
In-situ TEM observation of the response of ultrafine- and nanocrystalline-grained tungsten to extreme irradiation environments journal May 2014
Ion beam nanopatterning of III-V semiconductors: consistency of experimental and simulation trends within a chemistry-driven theory journal December 2015
In situ heavy ion irradiation studies of nanopore shrinkage and enhanced radiation tolerance of nanoporous Au journal January 2017
Raman spectroscopy of ion irradiated diamond journal July 2004
In situ x-ray scattering study of self-organized nanodot pattern formation on GaSb(001) by ion beam sputtering journal September 2007
IMPACT: A facility to study the interaction of low-energy intense particle beams with dynamic heterogeneous surfaces journal November 2007
Investigation of ion‐implanted GaP layers by Brillouin scattering journal May 1993
Online in situ x-ray diffraction setup for structural modification studies during swift heavy ion irradiation journal January 2012
Materials analysis and particle probe: A compact diagnostic system for in situ analysis of plasma-facing components (invited) journal October 2012
In situ Raman monitoring of He 2+ irradiation induced damage in a UO 2 ceramic journal July 2013
An experiment on the dynamics of ion implantation and sputtering of surfaces journal February 2014
Open volume defects and magnetic phase transition in Fe 60 Al 40 transition metal aluminide journal April 2015
In-situ evolution of helium bubbles in SiC under irradiation journal November 2015
Unraveling wall conditioning effects on plasma facing components in NSTX-U with the Materials Analysis Particle Probe (MAPP) journal July 2016
Positron annihilation lifetime and Doppler broadening spectroscopy at the ELBE facility
  • Wagner, Andreas; Butterling, Maik; Liedke, Maciej O.
  • INTERNATIONAL WORKSHOP ON PHYSICS WITH POSITRONS AT JEFFERSON LAB, AIP Conference Proceedings https://doi.org/10.1063/1.5040215
conference January 2018
Ionoluminescence to study irradiation stability of zirconia conference January 2020
Development of the materials analysis and particle probe for Proto-MPEX journal April 2021
In situ investigation of 75 MeV boron and 100 MeV oxygen ion irradiation effects on 50 GHz silicon–germanium heterojunction bipolar transistors journal August 2013
Study of defect evolution by TEM with in situ ion irradiation and coordinated modeling journal June 2012
Superior tolerance of Ag/Ni multilayers against Kr ion irradiation: an in situ study journal July 2013
Field ion microscope examination of heavy ion radiation damage in iridium: I. experimental technique journal October 1968
Cavity Formation in Molybdenum Studied In Situ in TEM journal February 2017
Cavity Evolution at Grain Boundaries as a Function of Radiation Damage and Thermal Conditions in Nanocrystalline Nickel journal December 2015
In situ spectroscopic ellipsometry as a versatile tool for studying atomic layer deposition journal March 2009
In situ x-ray reflectivity study of swift heavy ion induced interface modification in a W/Si multilayer x-ray mirror journal December 2014
Helium induced nanoscopic morphology on tungsten under fusion relevant plasma conditions journal January 2008
Effects of helium irradiation on degradation of optical properties of single and polycrystalline Mo mirrors for plasma diagnostics journal December 2009
Unraveling atomic-level self-organization at the plasma-material interface journal June 2017
Low energy Ar + ion irradiation induced surface modification in cadmium zinc telluride (CdZnTe) journal September 2014
Resistivity changes and defect mobility in ion-irradiated YBa 2 Cu 3 O 7 − x journal May 1989
In situ electrical resistivity of thin-film β-NiAl under Ar irradiation at 77 K journal May 1992
Phonon scattering effects from point and extended defects on thermal conductivity studied via ion irradiation of crystals with self-impurities journal September 2018
Formation of Ordered Nanoscale Semiconductor Dots by Ion Sputtering journal September 1999
Studying Radiation Damage in Structural Materials by Using Ion Accelerators journal January 2011
Phase Transitions in Ge-Sb-Te Alloys Induced by Ion Irradiations journal April 2016
Transmission electron microscopy with in situ ion irradiation journal February 2015
Oxidation of Zircaloy-4 during in situ proton irradiation and corrosion in PWR primary water journal March 2015
Ion irradiation and radiation effect characterization at the JANNUS-Saclay triple beam facility journal February 2015
Transient grating spectroscopy: An ultrarapid, nondestructive materials evaluation technique journal May 2019
In Situ and Operando Spectroscopy: A Powerful Approach Towards Understanding Catalysts journal July 2018
Erosion of Carbon-Based Materials Under High-Fluence Heavy-Ion Irradiation journal January 2011
In Situ TEM Multi-Beam Ion Irradiation as a Technique for Elucidating Synergistic Radiation Effects journal September 2017
Irradiation Induced Microstructure Evolution in Nanostructured Materials: A Review journal February 2016

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