Interlayer Triplet-Sensitized Luminescence in Layered Two-Dimensional Hybrid Metal-Halide Perovskites

Lin, YunHui L.; Blackburn, Jeffrey L.; Beard, Matthew C.; Johnson, Justin C.

doi:10.1021/acsenergylett.1c02011

Interlayer Triplet-Sensitized Luminescence in Layered Two-Dimensional Hybrid Metal-Halide Perovskites

Journal Article · Thu Oct 28 00:00:00 EDT 2021 · ACS Energy Letters

DOI:https://doi.org/10.1021/acsenergylett.1c02011· OSTI ID:1832437

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National Renewable Energy Lab. (NREL), Golden, CO (United States)

In this work, we review an emerging class of 2D layered metal-halide perovskites that exhibit important photophysical behavior involving inorganic exciton-to-molecular triplet energy flow. These novel systems have potential to impact several energy-related fields and processes, including optoelectronics, photon upconversion strategies, and triplet-based photocatalysis. Early studies provided initial guidance and revealed several intriguing questions that more recent developments, in terms of both expanded and diversified compositional tuning and more sophisticated characterization, have begun to answer. These questions center around the delicate interplay between physical and electronic structure that is perturbed by choice of perovskite structural motif and organic spacer properties. In addition to their distinct natures, the energy offsets between the metal-halide and molecular excitons can be leveraged for a variety of unique effects and emergent properties, including fast interlayer energy transfer. We review the key advances with an eye toward strategies for controlling photophysical outcomes based on structure-energy-function relationships.

View Accepted Manuscript (DOE)

Research Organization:: National Renewable Energy Laboratory (NREL), Golden, CO (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Chemical Sciences, Geosciences & Biosciences Division

Grant/Contract Number:: AC36-08GO28308

OSTI ID:: 1832437

Report Number(s):: NREL/JA--5900-81018; MainId:79794; UUID:a2cba2d9-cd9a-4c2c-a439-296a865fe571; MainAdminID:63340

Journal Information:: ACS Energy Letters, Journal Name: ACS Energy Letters Journal Issue: 11 Vol. 6; ISSN 2380-8195

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

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