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Title: Electrical Tuning of Tin-Vacancy Centers in Diamond

Journal Article · · Physical Review Applied

Group-IV color centers in diamond have attracted significant attention as solid-state spin qubits because of their excellent optical and spin properties. Among these color centers, the tin-vacancy (Sn-V-) center is of particular interest because its large ground-state splitting enables long spin coherence times at temperatures above 1 K. However, color centers typically suffer from inhomogeneous broadening, which can be exacerbated by nanofabrication-induced strain, hindering the implementation of quantum nodes emitting indistinguishable photons. Although strain and Raman tuning have been investigated as promising tuning techniques to overcome the spectral mismatch between distinct group-IV color centers, other approaches need to be explored to find methods that can offer more localized control without sacrificing emission intensity. Here, we study the electrical tuning of Sn-V- centers in diamond via the direct-current Stark effect. We demonstrate a tuning range beyond 1.7 GHz. We observe both quadratic and linear dependence on the applied electric field. Further, we also confirm that the tuning effect we observe is a result of the applied electric field and is distinct from thermal tuning due to Joule heating. Stark tuning is a promising avenue toward overcoming detunings between emitters and enabling the realization of multiple identical quantum nodes.

Research Organization:
Stanford Univ., CA (United States)
Sponsoring Organization:
USDOE Office of Science (SC); US Air Force Office of Scientific Research (AFOSR); National Science Foundation (NSF); Swiss National Science Foundation (SNSF)
Grant/Contract Number:
SC0020115; W911NF-13-1-0309; 1838976; FA9550-16-1-0223; P400P2 194424; ECCS-2026822
OSTI ID:
1832246
Journal Information:
Physical Review Applied, Vol. 15, Issue 6; ISSN 2331-7019
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English

References (41)

Two-Photon Quantum Interference from Separate Nitrogen Vacancy Centers in Diamond journal January 2012
Ab Initio Magneto-Optical Spectrum of Group-IV Vacancy Color Centers in Diamond journal June 2018
Tin-Vacancy Quantum Emitters in Diamond journal December 2017
Strain engineering of the silicon-vacancy center in diamond journal May 2018
Narrow-Linewidth Tin-Vacancy Centers in a Diamond Waveguide journal August 2020
Optical dephasing in defect-rich crystals journal November 1999
An integrated diamond nanophotonics platform for quantum-optical networks journal October 2016
Large-scale integration of artificial atoms in hybrid photonic circuits journal July 2020
Electric-field effects of two-level systems observed with single-molecule spectroscopy journal May 2003
Electron–phonon processes of the silicon-vacancy centre in diamond journal April 2015
Narrow-Linewidth Homogeneous Optical Emitters in Diamond Nanostructures via Silicon Ion Implantation journal April 2016
Multiple intrinsically identical single-photon emitters in the solid state journal August 2014
Cavity-Enhanced Raman Emission from a Single Color Center in a Solid journal August 2018
Photon-mediated interactions between quantum emitters in a diamond nanocavity journal September 2018
Direct Structural Identification and Quantification of the Split-Vacancy Configuration for Implanted Sn in Diamond journal July 2020
Quantum-Confined Stark Effect in Single CdSe Nanocrystallite Quantum Dots journal December 1997
Indistinguishable Photons from Separated Silicon-Vacancy Centers in Diamond journal September 2014
Wide-range electrical tunability of single-photon emission from chromium-based colour centres in diamond journal July 2011
Spectrally reconfigurable quantum emitters enabled by optimized fast modulation journal September 2020
Interference of Single Photons from Two Separate Semiconductor Quantum Dots journal April 2010
Stark Shift Control of Single Optical Centers in Diamond journal August 2006
Quantum Interference of Tunably Indistinguishable Photons from Remote Organic Molecules journal March 2010
Analytic and geometric properties of scattering from periodically modulated quantum-optical systems journal September 2020
Characterization of optical and spin properties of single tin-vacancy centers in diamond nanopillars journal May 2019
Control and imaging of single-molecule spectral dynamics using a nano-electrode journal September 2009
Spectroscopic investigations of negatively charged tin-vacancy centres in diamond journal January 2020
Transform-Limited Photons From a Coherent Tin-Vacancy Spin in Diamond journal January 2020
SRIM – The stopping and range of ions in matter (2010)
  • Ziegler, James F.; Ziegler, M. D.; Biersack, J. P.
  • Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 268, Issue 11-12 https://doi.org/10.1016/j.nimb.2010.02.091
journal June 2010
Experimental demonstration of memory-enhanced quantum communication journal March 2020
Generation of Tin-Vacancy Centers in Diamond via Shallow Ion Implantation and Subsequent Diamond Overgrowth journal February 2020
Stark Tuning of Single-Photon Emitters in Hexagonal Boron Nitride journal June 2018
Dynamic Stabilization of the Optical Resonances of Single Nitrogen-Vacancy Centers in Diamond journal May 2012
Stark tuning and electrical charge state control of single divacancies in silicon carbide journal December 2017
Stark Effect on Single Molecules of Dibenzanthanthrene in a Naphthalene Crystal and in a n -Hexadecane Shpol'skii Matrix journal March 1999
Two-photon interference of the emission from electrically tunable remote quantum dots journal July 2010
Large stark tuning of InAs/InP quantum dots journal February 2019
Quantum Network Nodes Based on Diamond Qubits with an Efficient Nanophotonic Interface journal October 2019
Quantum internet: A vision for the road ahead journal October 2018
Optical Stark spectroscopy of solids journal July 2007
Quantum Interference of Single Photons from Remote Nitrogen-Vacancy Centers in Diamond journal April 2012
The quantum internet journal June 2008