skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Evidence for anisotropic spin-triplet Andreev reflection at the 2D van der Waals ferromagnet/superconductor interface

Journal Article · · Nature Communications
 [1];  [1];  [2];  [1];  [1];  [1];  [1];  [1];  [3]; ORCiD logo [4];  [4];  [3]; ORCiD logo [4]; ORCiD logo [1]
  1. Peking Univ., Beijing (China); Collaborative Innovation Center of Quantum Matter, Beijing (China)
  2. Wuhan Univ. of Technology (China)
  3. State Univ. of New York at Buffalo, NY (United States)
  4. Peking Univ., Beijing (China); Collaborative Innovation Center of Quantum Matter, Beijing (China); University of Chinese Academy of Sciences, Beijing (China); Beijing Academy of Quantum Information Sciences, Beijing (China)

Fundamental symmetry breaking and relativistic spin–orbit coupling give rise to fascinating phenomena in quantum materials. Of particular interest are the interfaces between ferromagnets and common s-wave superconductors, where the emergent spin-orbit fields support elusive spin-triplet superconductivity, crucial for superconducting spintronics and topologically-protected Majorana bound states. Here, we report the observation of large magnetoresistances at the interface between a quasi-two-dimensional van der Waals ferromagnet Fe0.29TaS2 and a conventional s-wave superconductor NbN, which provides the possible experimental evidence for the spin-triplet Andreev reflection and induced spin-triplet superconductivity at ferromagnet/superconductor interface arising from Rashba spin-orbit coupling. The temperature, voltage, and interfacial barrier dependences of the magnetoresistance further support the induced spin-triplet superconductivity and spin-triplet Andreev reflection. This discovery, together with the impressive advances in two-dimensional van der Waals ferromagnets, opens an important opportunity to design and probe superconducting interfaces with exotic properties.

Research Organization:
State Univ. of New York (SUNY), Amherst, NY (United States); State Univ. of New York at Buffalo, NY (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division; National Basic Research Programs of China; National Natural Science Foundation of China (NSFC); Beijing Natural Science Foundation; Key Research Program of the Chinese Academy of Sciences; Hubei Provincial Natural Science Foundation of China
Grant/Contract Number:
SC0004890; XDB28000000
OSTI ID:
1831506
Journal Information:
Nature Communications, Vol. 12, Issue 1; ISSN 2041-1723
Publisher:
Nature Publishing GroupCopyright Statement
Country of Publication:
United States
Language:
English

References (31)

Magnetoanisotropic spin-triplet Andreev reflection in ferromagnet-Ising superconductor junctions journal April 2018
Spin-polarized supercurrents for spintronics: a review of current progress journal September 2015
Spintronics: Fundamentals and applications journal April 2004
Towards properties on demand in quantum materials journal October 2017
Spin current as a probe of quantum materials journal August 2019
Tunneling Anisotropic Magnetoresistance: A Spin-Valve-Like Tunnel Magnetoresistance Using a Single Magnetic Layer journal September 2004
Gate-tunable room-temperature ferromagnetism in two-dimensional Fe3GeTe2 journal October 2018
Synthetic spin–orbit interaction for Majorana devices journal August 2019
Wireless Majorana Bound States: From Magnetic Tunability to Braiding journal August 2016
Enhanced spin pumping into superconductors provides evidence for superconducting pure spin currents journal April 2018
Spin-orbit coupling as a source of long-range triplet proximity effect in superconductor-ferromagnet hybrid structures journal April 2014
Probing and controlling magnetic states in 2D layered magnetic materials journal September 2019
Observation of Spin-Triplet Superconductivity in Co-Based Josephson Junctions journal March 2010
Odd triplet superconductivity and related phenomena in superconductor-ferromagnet structures journal November 2005
Superconducting 2D System with Lifted Spin Degeneracy: Mixed Singlet-Triplet State journal July 2001
Reversible control of spin-polarized supercurrents in ferromagnetic Josephson junctions journal August 2014
Milestones Toward Majorana-Based Quantum Computing journal August 2016
Tunneling Anisotropic Magnetoresistance and Spin-Orbit Coupling in Fe / GaAs / Au Tunnel Junctions journal August 2007
Next steps of quantum transport in Majorana nanowire devices journal November 2019
Spin-polarized electron tunneling journal March 1994
Proximity effects in superconductor-ferromagnet heterostructures journal September 2005
Generic New Platform for Topological Quantum Computation Using Semiconductor Heterostructures journal January 2010
Magnetoanisotropic Andreev Reflection in Ferromagnet-Superconductor Junctions journal September 2015
Magnetism in two-dimensional van der Waals materials journal October 2018
Equal-spin Andreev reflection and long-range coherent transport in high-temperature superconductor/half-metallic ferromagnet junctions journal May 2012
Magnetic 2D materials and heterostructures journal May 2019
Superconducting spintronics journal April 2015
Anomalous Hall effect mechanisms in the quasi-two-dimensional van der Waals ferromagnet F e 0.29 Ta S 2 journal August 2019
Transition from metallic to tunneling regimes in superconducting microconstrictions: Excess current, charge imbalance, and supercurrent conversion journal April 1982
Emergent functions of quantum materials journal September 2017
Two-dimensional magnetic crystals and emergent heterostructure devices journal February 2019