Quantum Computing with Exciton Qubits in Colloidal Semiconductor Nanocrystals

Harankahage, Dulanjan; Cassidy, James; Yang, Mingrui; Porotnikov, Dmitry; Williams, Maia; Kholmicheva, Natalia; Zamkov, Mikhail

doi:10.1021/acs.jpcc.1c05009

Title: Quantum Computing with Exciton Qubits in Colloidal Semiconductor Nanocrystals

Journal Article · Mon Oct 04 00:00:00 EDT 2021 · Journal of Physical Chemistry. C

DOI:https://doi.org/10.1021/acs.jpcc.1c05009· OSTI ID:1831439

Harankahage, Dulanjan ^[1]; Cassidy, James ^[1]; Yang, Mingrui ^[1]; Porotnikov, Dmitry ^[1]; Williams, Maia ^[1]; Kholmicheva, Natalia ^[1];

^[1]

Bowling Green State Univ., OH (United States)

The present work evaluates the feasibility of quantum computing with exciton qubits in coupled colloidal semiconductor nanocrystals (NCs). A strategy for manipulating two-qubit states of colloidal NC hetero-dimers is described. We show that a sequence of laser pulses with the same photon energy can bring excitonic states of a nanocrystal hetero-dimer into entanglement and perform arbitrary qubit rotations (quantum gates). Our simulations of a realistic two-particle assembly of CdSe/CdS core/shell NCs demonstrate that such two-qubit gate operations can be driven by optical parametric oscillators with a theoretical error of 0.1%. A strategy for upscaling two-qubit hetero-dimers to N-qubit exciton gates in semiconductor NC assemblies is discussed.

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Research Organization:: Bowling Green State Univ., OH (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0016872

OSTI ID:: 1831439

Alternate ID(s):: OSTI ID: 1865408

Journal Information:: Journal of Physical Chemistry. C, Vol. 125, Issue 40; ISSN 1932-7447

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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