Progress of 3D network binders in silicon anodes for lithium ion batteries

Preman, Anjali N.; Lee, Hyocheol; Yoo, Jungwoo; Kim, Il Tae; Saito, Tomonori; Ahn, Suk-kyun

doi:10.1039/d0ta07713e

Progress of 3D network binders in silicon anodes for lithium ion batteries

Journal Article · Mon Nov 02 04:00:00 EST 2020 · Journal of Materials Chemistry. A

DOI:https://doi.org/10.1039/d0ta07713e· OSTI ID:1822085

Preman, Anjali N. ^[1]; Lee, Hyocheol ^[1]; Yoo, Jungwoo ^[2]; ^[3]; ^[4]; ^[1]

Pusan National Univ., Busan (Korea, Republic of)
LG Chem, Daejeon (Korea, Republic of). Advanced Automotive Battery Development Center
Gachon University (Korea, Republic of)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Prompted by its overwhelming benefits, silicon (Si) has evolved as one of the most promising anode materials for high-capacity lithium-ion batteries (LIBs). However, some of the intrinsic drawbacks such as low ionic conductivity and inevitable volume change during the alloying/dealloying process seriously hamper the commercialization of Si-based anodes in LIBs. Among the several strategies to overcome the challenges of the Si anode, the development of designed polymeric binders is imperative for enabling stable and satisfactory performance. The improved cell performance due to the designed binders is recognized as an economical and practical approach, especially from the industrial perspective. In addition to their conventional role in integrating electrode components, binders also play a significant role in alleviating the unfavorable phenomenon of volume expansion, and ultimately stabilizing the Si anode and Si-electrolyte interphase. The polymer architecture of the binders significantly influences the binder performance, and three-dimensional (3D) network binders are generally more effective at coping with the stress resulting from the huge volume change of the Si anode. To develop advanced 3D binders, substantial research efforts have been made including various crosslinking strategies in the past decade. In this review, we focus on diverse crosslinking methods including chemical-, physical-, and topological-crosslinking for rationally designing network binders for Si anodes and take a glance at dynamic interactions to construct healable binders for long-term stability.

View Accepted Manuscript (DOE)

Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1822085

Alternate ID(s):: OSTI ID: 1724232

Journal Information:: Journal of Materials Chemistry. A, Journal Name: Journal of Materials Chemistry. A Journal Issue: 48 Vol. 8; ISSN 2050-7488

Publisher:: Royal Society of ChemistryCopyright Statement

Country of Publication:: United States

Language:: English

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Interweaving 3D Network Binder for High-Areal-Capacity Si Anode through Combined Hard and Soft Polymers

Journal Article · Tue Nov 27 23:00:00 EST 2018 · Advanced Energy Materials · OSTI ID:1529547

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Progress of 3D network binders in silicon anodes for lithium ion batteries

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