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Post-compression of long-wave infrared 2 picosecond sub-terawatt pulses in bulk materials

Journal Article · · Optics Express
DOI:https://doi.org/10.1364/OE.434238· OSTI ID:1821762

We have experimentally demonstrated the post-compression of a long-wave infrared (9.2 μm) 150 GW peak power pulse from 2 ps to less than 500 fs using a sequence of two bulk materials with negative group velocity dispersion (GVD). The compression resulted in up to 1.6-fold increase of the peak power and up to 2.8-fold increase of the intensity in the center of a quasi-Gaussian beam. The partial decoupling of the self-phase modulation and chirp compensation stages by using two materials with significantly different ratios of nonlinear refractive index to GVD provides accurate optimization of the compression mechanism and promises a viable path to scaling peak powers to supra-terawatt levels. During the preparatory study, we measured, for the first time to our knowledge, the nonlinear refractive indices of NaCl, KCl, and BaF 2 for picosecond pulses in the long-wave infrared region.

Research Organization:
Brookhaven National Laboratory (BNL), Upton, NY (United States)
Sponsoring Organization:
USDOE; USDOE Laboratory Directed Research and Development (LDRD) Program; USDOE Office of Science (SC)
Grant/Contract Number:
SC0012704
OSTI ID:
1821762
Alternate ID(s):
OSTI ID: 1827704
Report Number(s):
BNL--222321-2021-JAAM
Journal Information:
Optics Express, Journal Name: Optics Express Journal Issue: 20 Vol. 29; ISSN 1094-4087; ISSN OPEXFF
Publisher:
Optical Society of AmericaCopyright Statement
Country of Publication:
United States
Language:
English

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