Spin-textured Chern bands in AB-stacked transition metal dichalcogenide bilayers

Zhang, Yang; Devakul, Trithep; Fu, Liang

doi:10.1073/pnas.2112673118

Title: Spin-textured Chern bands in AB-stacked transition metal dichalcogenide bilayers

Journal Article · Thu Sep 02 00:00:00 EDT 2021 · Proceedings of the National Academy of Sciences of the United States of America

DOI:https://doi.org/10.1073/pnas.2112673118· OSTI ID:1819966

^[1];

^[1]; Fu, Liang ^[1]

Department of Physics, Massachusetts Institute of Technology, Cambridge, MA 02139

Significance The long-wavelength moiré superlattices in twisted two-dimensional (2D) structures have emerged as a highly tunable platform for strongly correlated electron physics. In this work, we reveal the displacement field–induced topological moiré bands in AB-stacked transition-metal dichalcogenide (TMD) heterobilayer ${M o T e}_{2}$ / ${W S e}_{2}$ . Valley-contrasting Chern bands with nontrivial spin texture are formed from interlayer hybridization between ${M o T e}_{2}$ and ${W S e}_{2}$ bands of nominally opposite spins. The general mechanism for band inversion we uncovered in AB-stacked TMD bilayers is quite robust and can be applied to other material combinations as well. Our study establishes a recipe for creating topological bands in AB-stacked TMD bilayers in general, which provides a highly tunable platform for realizing quantum-spin Hall and interaction-induced quantum anomalous Hall effects.

View Journal Article

Cite

Export

Save

Research Organization:: Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division

Grant/Contract Number:: SC0018945; SC0020149

OSTI ID:: 1819966

Alternate ID(s):: OSTI ID: 1852725

Journal Information:: Proceedings of the National Academy of Sciences of the United States of America, Journal Name: Proceedings of the National Academy of Sciences of the United States of America Vol. 118 Journal Issue: 36; ISSN 0027-8424

Publisher:: Proceedings of the National Academy of SciencesCopyright Statement

Country of Publication:: United States

Language:: English

References (39)

An unusual continuous paramagnetic-limited superconducting phase transition in 2D NbSe 2 Sohn, Egon; Xi, Xiaoxiang; He, Wen-Yu Nature Materials, Vol. 17, Issue 6 https://doi.org/10.1038/s41563-018-0061-1	journal	April 2018
Coupled Spin and Valley Physics in Monolayers of ${MoS}_{2}$ and Other Group-VI Dichalcogenides Xiao, Di; Liu, Gui-Bin; Feng, Wanxiang Physical Review Letters, Vol. 108, Issue 19 https://doi.org/10.1103/PhysRevLett.108.196802	journal	May 2012
Generalized Gradient Approximation Made Simple Perdew, John P.; Burke, Kieron; Ernzerhof, Matthias Physical Review Letters, Vol. 77, Issue 18, p. 3865-3868 https://doi.org/10.1103/PhysRevLett.77.3865	journal	October 1996
Correlated electronic phases in twisted bilayer transition metal dichalcogenides Wang, Lei; Shih, En-Min; Ghiotto, Augusto Nature Materials, Vol. 19, Issue 8 https://doi.org/10.1038/s41563-020-0708-6	journal	June 2020
Observation of the quantum spin Hall effect up to 100 kelvin in a monolayer crystal Wu, Sanfeng; Fatemi, Valla; Gibson, Quinn D. Science, Vol. 359, Issue 6371 https://doi.org/10.1126/science.aan6003	journal	January 2018
Mott and generalized Wigner crystal states in WSe2/WS2 moiré superlattices Regan, Emma C.; Wang, Danqing; Jin, Chenhao Nature, Vol. 579, Issue 7799 https://doi.org/10.1038/s41586-020-2092-4	journal	March 2020
Hubbard Model Physics in Transition Metal Dichalcogenide Moiré Bands Wu, Fengcheng; Lovorn, Timothy; Tutuc, Emanuel Physical Review Letters, Vol. 121, Issue 2 https://doi.org/10.1103/PhysRevLett.121.026402	journal	July 2018
Efficiency of ab-initio total energy calculations for metals and semiconductors using a plane-wave basis set Kresse, G.; Furthmüller, J. Computational Materials Science, Vol. 6, Issue 1, p. 15-50 https://doi.org/10.1016/0927-0256(96)00008-0	journal	July 1996
Electronic structures, charge transfer, and charge order in twisted transition metal dichalcogenide bilayers Zhang, Yang; Liu, Tongtong; Fu, Liang Physical Review B, Vol. 103, Issue 15 https://doi.org/10.1103/PhysRevB.103.155142	journal	April 2021
Quantum Spin Hall Effect in Two-Dimensional Crystals of Transition-Metal Dichalcogenides Cazalilla, M. A.; Ochoa, H.; Guinea, F. Physical Review Letters, Vol. 113, Issue 7 https://doi.org/10.1103/PhysRevLett.113.077201	journal	August 2014
Imaging moiré flat bands in three-dimensional reconstructed WSe2/WS2 superlattices Li, Hongyuan; Li, Shaowei; Naik, Mit H. Nature Materials, Vol. 20, Issue 7 https://doi.org/10.1038/s41563-021-00923-6	journal	February 2021
Magic in twisted transition metal dichalcogenide bilayers Devakul, Trithep; Crépel, Valentin; Zhang, Yang Nature Communications, Vol. 12, Issue 1 https://doi.org/10.1038/s41467-021-27042-9	journal	November 2021
Ising pairing in superconducting NbSe2 atomic layers Xi, Xiaoxiang; Wang, Zefang; Zhao, Weiwei Nature Physics, Vol. 12, Issue 2 https://doi.org/10.1038/nphys3538	journal	November 2015
Room-temperature ferroelectricity in MoTe2 down to the atomic monolayer limit Yuan, Shuoguo; Luo, Xin; Chan, Hung Lit Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-09669-x	journal	April 2019
Excitonic density wave and spin-valley superfluid in bilayer transition metal dichalcogenide Bi, Zhen; Fu, Liang Nature Communications, Vol. 12, Issue 1 https://doi.org/10.1038/s41467-020-20802-z	journal	January 2021
Simulation of Hubbard model physics in WSe2/WS2 moiré superlattices Tang, Yanhao; Li, Lizhong; Li, Tingxin Nature, Vol. 579, Issue 7799 https://doi.org/10.1038/s41586-020-2085-3	journal	March 2020
Correlated insulating states at fractional fillings of moiré superlattices Xu, Yang; Liu, Song; Rhodes, Daniel A. Nature, Vol. 587, Issue 7833 https://doi.org/10.1038/s41586-020-2868-6	journal	November 2020
Moiré heterostructures as a condensed-matter quantum simulator Kennes, Dante M.; Claassen, Martin; Xian, Lede Nature Physics, Vol. 17, Issue 2 https://doi.org/10.1038/s41567-020-01154-3	journal	February 2021
Quantum Spin Hall Effect in Inverted Type-II Semiconductors Liu, Chaoxing; Hughes, Taylor L.; Qi, Xiao-Liang Physical Review Letters, Vol. 100, Issue 23 https://doi.org/10.1103/PhysRevLett.100.236601	journal	June 2008
Generalized Wigner crystallization in moiré materials Padhi, Bikash; Chitra, R.; Phillips, Philip W. Physical Review B, Vol. 103, Issue 12 https://doi.org/10.1103/PhysRevB.103.125146	journal	March 2021
Metal-insulator transition in transition metal dichalcogenide heterobilayer moiré superlattices Morales-Durán, Nicolás; MacDonald, Allan H.; Potasz, Pawel Physical Review B, Vol. 103, Issue 24 https://doi.org/10.1103/PhysRevB.103.L241110	journal	June 2021
Band topology, Hubbard model, Heisenberg model, and Dzyaloshinskii-Moriya interaction in twisted bilayer ${WSe}_{2}$ Pan, Haining; Wu, Fengcheng; Das Sarma, Sankar Physical Review Research, Vol. 2, Issue 3 https://doi.org/10.1103/PhysRevResearch.2.033087	journal	July 2020
Hartree-Fock study of the moiré Hubbard model for twisted bilayer transition metal dichalcogenides Zang, Jiawei; Wang, Jie; Cano, Jennifer Physical Review B, Vol. 104, Issue 7 https://doi.org/10.1103/PhysRevB.104.075150	journal	August 2021
Robust Helical Edge Transport in Gated $InAs / GaSb$ Bilayers Du, Lingjie; Knez, Ivan; Sullivan, Gerard Physical Review Letters, Vol. 114, Issue 9 https://doi.org/10.1103/PhysRevLett.114.096802	journal	March 2015
Strong room-temperature ferromagnetism in VSe2 monolayers on van der Waals substrates Bonilla, Manuel; Kolekar, Sadhu; Ma, Yujing Nature Nanotechnology, Vol. 13, Issue 4 https://doi.org/10.1038/s41565-018-0063-9	journal	February 2018
Shubnikov–de Haas Oscillations of High-Mobility Holes in Monolayer and Bilayer ${WSe}_{2}$ : Landau Level Degeneracy, Effective Mass, and Negative Compressibility Fallahazad, Babak; Movva, Hema C. P.; Kim, Kyounghwan Physical Review Letters, Vol. 116, Issue 8 https://doi.org/10.1103/PhysRevLett.116.086601	journal	February 2016
Quantum spin Hall effect in two-dimensional transition metal dichalcogenides Qian, X.; Liu, J.; Fu, L. Science, Vol. 346, Issue 6215 https://doi.org/10.1126/science.1256815	journal	November 2014
Gate-induced superconductivity in a monolayer topological insulator Sajadi, Ebrahim; Palomaki, Tauno; Fei, Zaiyao Science, Vol. 362, Issue 6417 https://doi.org/10.1126/science.aar4426	journal	October 2018
Topological Insulators in Twisted Transition Metal Dichalcogenide Homobilayers Wu, Fengcheng; Lovorn, Timothy; Tutuc, Emanuel Physical Review Letters, Vol. 122, Issue 8 https://doi.org/10.1103/PhysRevLett.122.086402	journal	February 2019
Deep moiré potentials in twisted transition metal dichalcogenide bilayers Shabani, Sara; Halbertal, Dorri; Wu, Wenjing Nature Physics https://doi.org/10.1038/s41567-021-01174-7	journal	February 2021
Imaging quantum spin Hall edges in monolayer WTe ₂ Shi, Yanmeng; Kahn, Joshua; Niu, Ben Science Advances, Vol. 5, Issue 2 https://doi.org/10.1126/sciadv.aat8799	journal	February 2019
Computational 2D Materials Database: Electronic Structure of Transition-Metal Dichalcogenides and Oxides Rasmussen, Filip A.; Thygesen, Kristian S. The Journal of Physical Chemistry C, Vol. 119, Issue 23 https://doi.org/10.1021/acs.jpcc.5b02950	journal	June 2015
Theory of tunable flux lattices in the homobilayer moiré of twisted and uniformly strained transition metal dichalcogenides Zhai, Dawei; Yao, Wang Physical Review Materials, Vol. 4, Issue 9 https://doi.org/10.1103/PhysRevMaterials.4.094002	journal	September 2020
Stripe phases in WSe2/WS2 moiré superlattices Jin, Chenhao; Tao, Zui; Li, Tingxin Nature Materials https://doi.org/10.1038/s41563-021-00959-8	journal	March 2021
Charge transfer excitations, pair density waves, and superconductivity in moiré materials Slagle, Kevin; Fu, Liang Physical Review B, Vol. 102, Issue 23 https://doi.org/10.1103/PhysRevB.102.235423	journal	December 2020
Strongly correlated electrons and hybrid excitons in a moiré heterostructure Shimazaki, Yuya; Schwartz, Ido; Watanabe, Kenji Nature, Vol. 580, Issue 7804 https://doi.org/10.1038/s41586-020-2191-2	journal	April 2020
Band alignment of two-dimensional transition metal dichalcogenides: Application in tunnel field effect transistors Gong, Cheng; Zhang, Hengji; Wang, Weihua Applied Physics Letters, Vol. 103, Issue 5 https://doi.org/10.1063/1.4817409	journal	July 2013
Moiré quantum chemistry: Charge transfer in transition metal dichalcogenide superlattices Zhang, Yang; Yuan, Noah F. Q.; Fu, Liang Physical Review B, Vol. 102, Issue 20 https://doi.org/10.1103/PhysRevB.102.201115	journal	November 2020
Quantum spin Hall state in monolayer 1T'-WTe2 Tang, Shujie; Zhang, Chaofan; Wong, Dillon Nature Physics, Vol. 13, Issue 7 https://doi.org/10.1038/nphys4174	journal	June 2017

Similar Records

First-principles calculation of gate-tunable ferromagnetism in magic-angle twisted bilayer graphene under pressure

Journal Article · Mon Jul 18 00:00:00 EDT 2022 · Journal of Physics. Condensed Matter · OSTI ID:1819966

Chen, Xiao; Liu, Shuanglong; Fry, James N.; +1 more

Strain-induced spontaneous Hall effect in an epitaxial thin film of a Luttinger semimetal

Journal Article · Mon Apr 15 00:00:00 EDT 2019 · Proceedings of the National Academy of Sciences of the United States of America · OSTI ID:1819966

Ohtsuki, Takumi; Tian, Zhaoming; Endo, Akira; +6 more

Quantum parity Hall effect in Bernal-stacked trilayer graphene

Journal Article · Fri May 03 00:00:00 EDT 2019 · Proceedings of the National Academy of Sciences of the United States of America · OSTI ID:1819966

Stepanov, Petr; Barlas, Yafis; Che, Shi; +10 more

Related Subjects

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS
moire superlattice
topological bands
first principle simulation
continuum model

Title: Spin-textured Chern bands in AB-stacked transition metal dichalcogenide bilayers

Citation Formats

References (39)

Similar Records

Related Subjects