Process modeling, techno-economic assessment, and life cycle assessment of the electrochemical reduction of CO2: a review

Somoza-Tornos, Ana; Guerra, Omar J.; Crow, Allison M.; Smith, Wilson A.; Hodge, Bri-Mathias

doi:10.1016/j.isci.2021.102813

Title: Process modeling, techno-economic assessment, and life cycle assessment of the electrochemical reduction of CO₂: a review

Journal Article · Thu Jul 01 00:00:00 EDT 2021 · iScience

DOI:https://doi.org/10.1016/j.isci.2021.102813· OSTI ID:1812705

Somoza-Tornos, Ana ^[1]; Guerra, Omar J. ^[2]; Crow, Allison M. ^[3]; Smith, Wilson A. ^[3]; Hodge, Bri-Mathias ^[3]

Univ. of Colorado, Boulder, CO (United States). Renewable and Sustainable Energy Inst.
National Renewable Energy Lab. (NREL), Golden, CO (United States)
Univ. of Colorado, Boulder, CO (United States). Renewable and Sustainable Energy Inst.; National Renewable Energy Lab. (NREL), Golden, CO (United States)

The electrochemical reduction of CO₂ has emerged as a promising alternative to traditional fossil-based technologies for the synthesis of chemicals. Its industrial implementation could lead to a reduction in the carbon footprint of chemicals and the mitigation of climate change impacts caused by hard-to-decarbonize industrial applications, among other benefits. However, the current low technology readiness levels of such emerging technologies make it hard to predict their performance at industrial scales. During the past few years, researchers have developed diverse techniques to model and assess the electrochemical reduction of CO₂ toward its industrial implementation. The aim of this literature review is to provide a comprehensive overview of techno-economic and life cycle assessment methods and pave the way for future assessment approaches. First, we identify which modeling approaches have been conducted to extend analysis to the production scale. Next, we explore the metrics used to evaluate such systems, regarding technical, environmental, and economic aspects. Finally, we assess the challenges and research opportunities for the industrial implementation of CO₂ reduction via electrolysis.

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Research Organization:: National Renewable Energy Lab. (NREL), Golden, CO (United States)

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE)

Grant/Contract Number:: AC36-08GO28308

OSTI ID:: 1812705

Report Number(s):: NREL/JA-5C00-80633; MainId:66364; UUID:1d233076-9350-4a30-a6e0-a3040f8e1579; MainAdminID:48439

Journal Information:: iScience, Vol. 24, Issue 7; ISSN 2589-0042

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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Title: Process modeling, techno-economic assessment, and life cycle assessment of the electrochemical reduction of CO2: a review

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Title: Process modeling, techno-economic assessment, and life cycle assessment of the electrochemical reduction of CO₂: a review