Tropospheric and stratospheric wildfire smoke profiling with lidar: mass, surface area, CCN, and INP retrieval

Ansmann, Albert; Ohneiser, Kevin; Mamouri, Rodanthi-Elisavet; Knopf, Daniel A.; Veselovskii, Igor; Baars, Holger; Engelmann, Ronny; Foth, Andreas; Jimenez, Cristofer; Seifert, Patric; Barja, Boris

doi:10.5194/acp-21-9779-2021

Title: Tropospheric and stratospheric wildfire smoke profiling with lidar: mass, surface area, CCN, and INP retrieval

Journal Article · Tue Jun 29 00:00:00 EDT 2021 · Atmospheric Chemistry and Physics (Online)

DOI:https://doi.org/10.5194/acp-21-9779-2021· OSTI ID:1805691

Ansmann, Albert ^[1]; Ohneiser, Kevin ^[1];

^[2];

^[3]; Veselovskii, Igor ^[4];

^[1];

^[5];

^[1];

^[6]

Leibniz Inst. for Tropospheric Research (Germany)
Cyprus Univ. of Technology, Limassol (Cyprus); ERATOSTHENES Center of Excellence, Limassol (Cyprus)
Stony Brook Univ., NY (United States)
Prokhorov General Physics Inst. of the Russian Academy of Sciences, Moscow (Russia)
Univ. of Leipzig (Germany)
Univ. of Magallanes, Punta Arenas (Chile)

We present retrievals of tropospheric and stratospheric height profiles of particle mass, volume, surface area, and number concentrations in the case of wildfire smoke layers as well as estimates of smoke-related cloud condensation nuclei (CCN) and ice-nucleating particle (INP) concentrations from backscatter lidar measurements on the ground and in space. Conversion factors used to convert the optical measurements into microphysical properties play a central role in the data analysis, in addition to estimates of the smoke extinction-to-backscatter ratios required to obtain smoke extinction coefficients. The set of needed conversion parameters for wildfire smoke is derived from AERONET observations of major smoke events, e.g., in western Canada in August 2017, California in September 2020, and southeastern Australia in January–February 2020 as well as from AERONET long-term observations of smoke in the Amazon region, southern Africa, and Southeast Asia. The new smoke analysis scheme is applied to CALIPSO observations of tropospheric smoke plumes over the United States in September 2020 and to ground-based lidar observation in Punta Arenas, in southern Chile, in aged Australian smoke layers in the stratosphere in January 2020. These case studies show the potential of spaceborne and ground-based lidars to document large-scale and long-lasting wildfire smoke events in detail and thus to provide valuable information for climate, cloud, and air chemistry modeling efforts performed to investigate the role of wildfire smoke in the atmospheric system.

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Research Organization:: Stony Brook Univ., NY (United States); Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Atmospheric Radiation Measurement (ARM) Data Center

Sponsoring Organization:: USDOE Office of Science (SC), Biological and Environmental Research (BER). Earth and Environmental Systems Science Division; USDOE Office of Science (SC), Biological and Environmental Research (BER)

Contributing Organization:: PNNL, BNL, ANL, ORNL

Grant/Contract Number:: SC0021034

OSTI ID:: 1805691

Alternate ID(s):: OSTI ID: 1810051

Journal Information:: Atmospheric Chemistry and Physics (Online), Vol. 21, Issue 12; ISSN 1680-7324

Publisher:: Copernicus Publications, EGUCopyright Statement

Country of Publication:: United States

Language:: English

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