A Review of the Design of Advanced Binders for High‐Performance Batteries

Zou, Feng; Manthiram, Arumugam

doi:10.1002/aenm.202002508

A Review of the Design of Advanced Binders for High‐Performance Batteries

Journal Article · Fri Oct 16 00:00:00 EDT 2020 · Advanced Energy Materials

DOI:https://doi.org/10.1002/aenm.202002508· OSTI ID:1804561

Zou, Feng ^[1]; ^[1]

Materials Science and Engineering Program &, Texas Materials Institute The University of Texas at Austin Austin TX 78712 USA

Abstract

Polymer binders as a critical component in rechargeable batteries provide the electrodes with interconnected structures and mechanical strength to maintain the electronic/ionic transfer during battery cycling. The conventional binders, such as polyvinylidene fluoride (PVDF), are not ideal candidates due to their relatively low adhesiveness, weak mechanical strength, and poor functionality for high‐energy‐density batteries with a thick electrode and/or a high‐capacity electrode. Nevertheless, the binder has not yet received the attention that reflects its importance in batteries. The requirements of high energy density batteries make essential the exploration of advanced polymeric binders, which possess particular functions. In this review, state‐of‐the‐art binder design strategies are sorted in terms of the challenges of various electrodes (anodes and cathodes for lithium ion batteries (LIBs) and sulfur cathodes for Li–S batteries), which have been commercialized or have the potential for practical cells. A deep insight into how the polymeric binders improve the cell performance and the design principle of new binders is also provided. Finally, a perspective on the direction of future binder development for high‐energy‐density batteries with long cycle life is presented.

View Accepted Manuscript (Publisher)

Sponsoring Organization:: USDOE

Grant/Contract Number:: SC0005397

OSTI ID:: 1804561

Alternate ID(s):: OSTI ID: 1850919

Journal Information:: Advanced Energy Materials, Journal Name: Advanced Energy Materials Journal Issue: 45 Vol. 10; ISSN 1614-6832

Publisher:: Wiley Blackwell (John Wiley & Sons)Copyright Statement

Country of Publication:: Germany

Language:: English

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