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Polymers in Lithium‐Ion and Lithium Metal Batteries

Journal Article · · Advanced Energy Materials
 [1];  [2];  [2];  [3];  [4];  [2];  [5];  [6];  [2];  [1]
  1. Department of Chemical Engineering Stanford University Stanford CA 94305 USA
  2. Department of Polymer Science and Engineering Nanjing University Nanjing 210023 China
  3. Department of Chemical Engineering Stanford University Stanford CA 94305 USA, Department of Chemistry Stanford University Stanford CA 94305 USA
  4. School of Chemistry and Chemical Engineering Shanghai Jiao Tong University Shanghai 200240 China
  5. Department of Materials Science and Engineering Stanford University Stanford CA 94305 USA
  6. Department of Chemical Engineering Tsinghua University Beijing 100084 China
+ Show Author Affiliations
Abstract

Lithium‐ion batteries play a significant role in modern electronics and electric vehicles. However, current Li‐ion battery chemistries are unable to satisfy the increasingly heightened expectations regarding energy demand and reliability. To boost the overall energy density while ensuring the safety of Li batteries, researchers have focused on alternative battery materials, such as silicon, sulfur, and Li metal. These represent promising avenues, although numerous obstacles (e.g., Si cracking, polysulfide shuttling, Li dendrites, etc.) must be tackled before batteries based on these materials can enter mass production and penetrate the mainstream market. Polymers are a class of materials that are widely used in current battery systems; however, many novel polymer chemistries may offer better performance and reliability than the current ones, and even overcome the issues of the above‐mentioned new battery materials. In this review, selected polymeric materials for solving these issues are categorized into four parts: polymer electrolytes, polymer artificial solid‐electrolyte interphases, binders, and separators. Both the current progress and the characterization methods are included. Potential future directions of energy materials research are pointed out as well.

Sponsoring Organization:
USDOE
OSTI ID:
1804523
Journal Information:
Advanced Energy Materials, Journal Name: Advanced Energy Materials Journal Issue: 15 Vol. 11; ISSN 1614-6832
Publisher:
Wiley Blackwell (John Wiley & Sons)Copyright Statement
Country of Publication:
Germany
Language:
English

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  • REVIEW ON ELECTROCHEMICAL STORAGE MATERIALS AND TECHNOLOGY: Proceedings of the 1st International Freiberg Conference on Electrochemical Storage Materials, AIP Conference Proceedings https://doi.org/10.1063/1.4878480
conference January 2014
Enhanced performance of the sulfur cathode with L-cysteine-modified gelatin binder journal May 2013
Physical properties of solid polymer electrolyte PEO(LiTFSI) complexes journal August 1995
Synthesis and characterization of carboxymethyl cellulose (CMC) from salak-fruit seeds as anode binder for lithium-ion battery journal August 2018
The optimization of CMC concentration as graphite binder on the anode of LiFePO 4 battery journal May 2017
A Major Constituent of Brown Algae for Use in High-Capacity Li-Ion Batteries journal September 2011
Materials both Tough and Soft journal April 2014
Highly elastic binders integrating polyrotaxanes for silicon microparticle anodes in lithium ion batteries journal July 2017
Effect of Carboxymethyl Cellulose on Aqueous Processing of Natural Graphite Negative Electrodes and their Electrochemical Performance for Lithium Batteries journal January 2005
The Electrochemical Behavior of Alkali and Alkaline Earth Metals in Nonaqueous Battery Systems—The Solid Electrolyte Interphase Model journal January 1979
Reduction of Charge-Transfer Resistance via Artificial SEI Formation Using Electropolymerization of Borylated Thiophene Monomer on Graphite Anodes journal January 2018
Citric Acid Based Pre-SEI for Improvement of Silicon Electrodes in Lithium Ion Batteries journal January 2018
Optimizing Areal Capacities through Understanding the Limitations of Lithium-Ion Electrodes journal November 2015
Binder Based on Polyelectrolyte for High Capacity Density Lithium/Sulfur Battery journal January 2012
Lithium-sulfur batteries journal May 2014
Recent Development of Carbonaceous Materials for Lithium–Sulphur Batteries journal November 2016
Membranes in Lithium Ion Batteries journal July 2012
A Review on Inorganic Nanoparticles Modified Composite Membranes for Lithium-Ion Batteries: Recent Progress and Prospects journal July 2019

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