Strongly correlated and topological states in [111] grown transition metal oxide thin films and heterostructures

Chakhalian, Jak; Liu, Xiaoran; Fiete, Gregory A.

doi:10.1063/5.0009092

Title: Strongly correlated and topological states in [111] grown transition metal oxide thin films and heterostructures

Journal Article · Fri May 15 00:00:00 EDT 2020 · APL Materials

DOI:https://doi.org/10.1063/5.0009092· OSTI ID:1802333

^[1];

^[1]; Fiete, Gregory A. ^[2]

Rutgers Univ., Piscataway, NJ (United States). Dept. of Physics and Astronomy
Northeastern Univ., Boston, MA (United States). Dept. of Physics; Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States). Dept. of Physics

We highlight recent advances in the theory, materials fabrication, and experimental characterization of strongly correlated and topological states in [111] oriented transition metal oxide thin films and heterostructures, which are notoriously difficult to realize compared to their [001] oriented counterparts. We focus on two classes of complex oxides, with the chemical formulas ABO ₃ and A ₂ B ₂ O ₇ , where the B sites are occupied by an open-shell transition metal ion with a local moment and the A sites are typically a rare earth element. The [111] oriented quasi-two-dimensional lattices derived from these parent compound lattices can exhibit peculiar geometries and symmetries, namely, a buckled honeycomb lattice, as well as kagome and triangular lattices. These lattice motifs form the basis for emergent strongly correlated and topological states expressed in exotic magnetism, various forms of orbital ordering, topological insulators, topological semimetals, quantum anomalous Hall insulators, and quantum spin liquids. For transition metal ions with high atomic number, spin–orbit coupling plays a significant role and may give rise to additional topological features in the electronic band structure and in the spectrum of magnetic excitations. We conclude this perspective by articulating open challenges and opportunities in this actively developing field.

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Research Organization:: Pennsylvania State Univ., University Park, PA (United States)

Sponsoring Organization:: USDOE Office of Science (SC)

Grant/Contract Number:: SC0012375

OSTI ID:: 1802333

Alternate ID(s):: OSTI ID: 1618943

Journal Information:: APL Materials, Vol. 8, Issue 5; ISSN 2166-532X

Publisher:: American Institute of Physics (AIP)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 16 works

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