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Hyperuniform Structures Formed by Shearing Colloidal Suspensions

Journal Article · · Physical Review Letters
In periodically sheared suspensions there is a dynamical phase transition, characterized by a critical strain amplitude $$γ_c$$, between an absorbing state where particle trajectories are reversible and an active state where trajectories are chaotic and diffusive. Repulsive nonhydrodynamic interactions between “colliding” particles’ surfaces have been proposed as a source of this broken time reversal symmetry. A simple toy model called random organization qualitatively reproduces the dynamical features of this transition. Random organization and other absorbing state models exhibit hyperuniformity, a strong suppression of density fluctuations on long length scales quantified by a structure factor $S(q → 0) ~q^α$ with $$\textit{α}$$ > 0, at criticality. In this work, we show experimentally that the particles in periodically sheared suspensions organize into structures with anisotropic short-range order but isotropic, long-range hyperuniform order when oscillatory shear amplitudes approach $$γ_c$$.
Research Organization:
Energy Frontier Research Centers (EFRC) (United States). Center for Bio-Inspired Energy Science (CBES); Northwestern Univ., Evanston, IL (United States)
Sponsoring Organization:
National Aeronautics and Space Administration (NASA); National Science Foundation (NSF); USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
SC0000989
OSTI ID:
1801367
Journal Information:
Physical Review Letters, Journal Name: Physical Review Letters Journal Issue: 14 Vol. 125; ISSN 0031-9007
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English

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