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Title: Nonlinear soliton confinement in weakly coupled antiferromagnetic spin chains

Journal Article · · Physical Review. B
 [1];  [2];  [3]; ORCiD logo [4]; ORCiD logo [4]; ORCiD logo [5]
  1. Univ. of Edinburgh, Scotland (United Kingdom); Science and Technology Facilities Council (STFC), Oxford (United Kingdom). Rutherford Appleton Lab. (RAL)
  2. Univ. of Edinburgh, Scotland (United Kingdom)
  3. Rutgers Univ., Piscataway, NJ (United States)
  4. Science and Technology Facilities Council (STFC), Oxford (United Kingdom). Rutherford Appleton Lab. (RAL)
  5. Science and Technology Facilities Council (STFC), Oxford (United Kingdom). Rutherford Appleton Lab. (RAL); Univ. College London (United Kingdom)

In this work, we analyze the low-energy dynamics of quasi-one-dimensional, large-$$\textit{S}$$ quantum antiferromagnets with easy-axis anisotropy, using a semiclassical nonlinear sigma model. The saddle point approximation leads to a sine-Gordon equation which supports soliton solutions. These correspond to the movement of spatially extended domain walls. Long-range magnetic order is a consequence of a weak interchain coupling. Below the ordering temperature, the coupling to nearby chains leads to an energy cost associated with the separation of two domain walls. From the kink-antikink two-soliton solution, we compute the effective confinement potential. At distances large compared to the size of the solitons the potential is linear, as expected for pointlike domain walls. At small distances the gradual annihilation of the solitons weakens the effective attraction and renders the potential quadratic. From numerically solving the effective one-dimensional Schrödinger equation with this nonlinear confinement potential we compute the soliton bound state spectrum. We apply the theory to CaFe2O4, an anisotropic $$\textit{S}$$ = 5/2 magnet based upon antiferromagnetic zigzag chains. Using inelastic neutron scattering, we are able to resolve seven discrete energy levels for spectra recorded slightly below the Néel temperature $$T_N$$ ≈ 200 K. These modes are well described by our nonlinear confinement model in the regime of large spatially extended solitons.

Research Organization:
Rutgers Univ., Piscataway, NJ (United States)
Sponsoring Organization:
USDOE Office of Science (SC); Engineering and Physical Sciences Research Council (EPSRC); Science and Technology Facilities Council (STFC)
Grant/Contract Number:
FG02-07ER46382; EP/P013449/1
OSTI ID:
1800461
Journal Information:
Physical Review. B, Vol. 102, Issue 2; ISSN 2469-9950
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English

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