Synthesis, growth mechanisms, and applications of palladium-based nanowires and other one-dimensional nanostructures

Kumar, Abhishek; Mohammadi, Mohammad Moein; Swihart, Mark T.

doi:10.1039/c9nr05835d

Synthesis, growth mechanisms, and applications of palladium-based nanowires and other one-dimensional nanostructures

Journal Article · Thu Aug 15 00:00:00 EDT 2019 · Nanoscale

DOI:https://doi.org/10.1039/c9nr05835d· OSTI ID:1799847

^[1]; Mohammadi, Mohammad Moein ^[2]; ^[3]

Univ. at Buffalo, NY (United States); OSTI
Univ. at Buffalo, NY (United States)
Univ. at Buffalo, NY (United States); State Univ. of New York (SUNY), Buffalo, NY (United States)

Palladium-based nanostructures have attracted the attention of researchers due to their useful catalytic properties and unique ability to form hydrides, which finds application in hydrogen storage and hydrogen detection. Palladium-based nanowires have some inherent advantages over other Pd nanomaterials, combining high surface-to-volume ratio with good thermal and electron transport properties, and exposing high-index crystal facets that can have enhanced catalytic activity. Over the past two decades, both synthesis methods and applications of 1D palladium nanostructures have advanced greatly. In this review, we start by discussing different types of 1D palladium nanostructures before moving on to the different synthesis approaches that can produce them. Next, we discuss factors including kinetic vs. thermodynamic control of growth, oxidative etching, and surface passivation that affect palladium nanowire synthesis. We also review efforts to gain insight into growth mechanisms using different characterization tools. We discuss the effects of concentration of capping agents, reducing agents, metal halides, pH, and sacrificial oxidation on the growth of Pd-based nanowires in solution, from shape control, to yield, to aspect ratio. Various applications of palladium and palladium alloy nanowires are then discussed, including electrocatalysis, hydrogen storage, and sensing of hydrogen and other chemicals. We end with a summary and some perspectives on future research directions for this category of nanomaterials.

View Accepted Manuscript (DOE)

Research Organization:: State University of New York (SUNY), Albany, NY (United States)

Sponsoring Organization:: USDOE Office of Fossil Energy (FE); USDOE Office of Fossil Energy and Carbon Management (FECM)

Grant/Contract Number:: FE0026463

OSTI ID:: 1799847

Alternate ID(s):: OSTI ID: 1558128

Journal Information:: Nanoscale, Journal Name: Nanoscale Journal Issue: 41 Vol. 11; ISSN NANOHL; ISSN 2040-3364

Publisher:: Royal Society of ChemistryCopyright Statement

Country of Publication:: United States

Language:: English

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Ultralarge-area block copolymer lithography via soft graphoepitaxy Jeong, Seong-Jun; Kim, Sang Ouk Journal of Materials Chemistry, Vol. 21, Issue 16 https://doi.org/10.1039/c0jm04248j	journal	January 2011
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Highly efficient hydrogen storage with PdAg nanotubes Lu, Yizhong; Jin, Rutian; Chen, Wei Nanoscale, Vol. 3, Issue 6 https://doi.org/10.1039/c1nr10186b	journal	January 2011
Anisotropic growth of palladium twinned nanostructures controlled by kinetics and their unusual activities in galvanic replacement Wang, Chengming; Wang, Lili; Long, Ran Journal of Materials Chemistry, Vol. 22, Issue 17 https://doi.org/10.1039/c2jm30411b	journal	January 2012
Potential applications of two ultrathin Pd nanowires to the hydrogen economy Ju, Shin-Pon; Weng, Meng-Hsiung; Huang, Wen-Cheng Journal of Materials Chemistry, Vol. 22, Issue 38 https://doi.org/10.1039/c2jm33696k	journal	January 2012
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Networks of DNA-templated palladium nanowires: structural and electrical characterisation and their use as hydrogen gas sensors Al-Hinai, Mariam N.; Hassanien, Reda; Wright, Nicholas G. Faraday Discussions, Vol. 164 https://doi.org/10.1039/c3fd00017f	journal	January 2013
Facile synthesis of porous worm-like Pd nanotubes with high electrocatalytic activity and stability towards ethylene glycol oxidation Feng, Jiu-Ju; Zhou, Dan-Ling; Xi, Huan-Xiang Nanoscale, Vol. 5, Issue 15 https://doi.org/10.1039/c3nr01578e	journal	January 2013
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Palladium nanowires stabilized by thiol-functionalized ionic liquid: seed-mediated synthesis and heterogeneous catalyst for Sonogashira coupling reaction Gao, Shuyan; Zhang, Hongjie; Wang, Xiaomei Nanotechnology, Vol. 16, Issue 8 https://doi.org/10.1088/0957-4484/16/8/042	journal	May 2005
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