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Title: Large eddy simulation of hydrogen piloted CH4/air premixed combustion with CO2 dilution

Journal Article · · Journal of the Energy Institute

Large eddy simulation (LES) of constant adiabatic temperature, hydrogen-piloted, turbulent lean premixed methane/air jet flames with varying amounts of CO2 addition are reported. Constant adiabatic temperature is achieved by increasing the fuel flow rate slightly to account for the higher specific heat of CO2 compared to N2. Such flames are relevant to low NOx gas turbines with high hydrogen content fuels and Exhaust Gas Recirculation (EGR). A newly designed burner called Piloted Axisymmetric Reactor Assisted Turbulent (PARAT) flame burner was utilized. The operating conditions in the experiment were selected to highlight the kinetic effects of CO2 addition by matching the Reynolds numbers, Lewis numbers and adiabatic flame temperatures. The LES simulations utilize a finite rate chemistry solver with DRM19 combustion mechanism with adaptive zoning and a dynamic structure turbulence model. A five-level adaptive mesh refinement (AMR) improves the velocity and temperature gradient resolution. The LES predicts the experimentally observed increase in flame length with CO2 levels caused by a decrease in the turbulent flame speed. The computational results also capture the experimentally observed departure from the thin flame limit and a collapse of the root mean square (RMS) versus mean temperature profiles for the three levels of CO2. The flame structure analysis illustrated super-equilibrium CO concentrations because of non-equilibrium chemistry effects caused by the external addition of CO2.

Research Organization:
Purdue Univ., West Lafayette, IN (United States)
Sponsoring Organization:
USDOE Office of Fossil Energy (FE)
Grant/Contract Number:
FE0011822; FG02-03ER15391
OSTI ID:
1799757
Alternate ID(s):
OSTI ID: 1615051
Journal Information:
Journal of the Energy Institute, Vol. 93, Issue 3; ISSN 1743-9671
Publisher:
ElsevierCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 5 works
Citation information provided by
Web of Science

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