Critical review of FDM 3D printing of PLA biocomposites filled with biomass resources, characterization, biodegradability, upcycling and opportunities for biorefineries

Bhagia, Samarthya; Bornani, Kamlesh; Agrawal, Ruchi; Satlewal, Alok; Ďurkovič, Jaroslav; Lagaňa, Rastislav; Bhagia, Meher; Yoo, Chang Geun; Zhao, Xianhui; Kunc, Vlastimil; Pu, Yunqiao; Ozcan, Soydan; Ragauskas, Arthur J.

doi:10.1016/j.apmt.2021.101078

Title: Critical review of FDM 3D printing of PLA biocomposites filled with biomass resources, characterization, biodegradability, upcycling and opportunities for biorefineries

Journal Article · Wed Sep 01 00:00:00 EDT 2021 · Applied Materials Today

DOI:https://doi.org/10.1016/j.apmt.2021.101078· OSTI ID:1787429

Bhagia, Samarthya; Bornani, Kamlesh; Agrawal, Ruchi; Satlewal, Alok; Ďurkovič, Jaroslav; Lagaňa, Rastislav; Bhagia, Meher; Yoo, Chang Geun; Zhao, Xianhui; Kunc, Vlastimil; Pu, Yunqiao; Ozcan, Soydan; Ragauskas, Arthur J.

3D printing by fused deposition modeling (FDM) is an advanced additive manufacturing technology for making thermoplastic-based structures. Several studies have recently investigated 3D printing of polylactic acid (PLA) with biomass resources like cellulose, hemicellulose, lignin and whole biomass. Such biodegradable composites are better for the environment and can be used to replace non-biodegradable composites in a variety of applications. Therefore, a deep understanding of printing such biocomposites is needed for supporting such manufacturing. Recent developments focused on FDM printing of PLA filled with biomass resources have been critically reviewed to reveal the intricate aspects of manufacturing of such materials and characterization of the changes caused by biomass-based fillers. Properties of high molecular weight PLA, essentials of printing with PLA and conditions for filament extrusion and printing of biocomposites are discussed. Characterization results from mechanical testing, thermal analysis, viscoelastic properties, imaging and spectroscopy are reviewed for understanding the impact of filling biomass resources in PLA by printing. The latter sections discuss applications, upcycling & recycling and future opportunities for biorefineries.

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Research Organization:: Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1787429

Alternate ID(s):: OSTI ID: 1805017

Journal Information:: Applied Materials Today, Journal Name: Applied Materials Today Vol. 24 Journal Issue: C; ISSN 2352-9407

Publisher:: ElsevierCopyright Statement

Country of Publication:: Netherlands

Language:: English

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