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Temporal Characterization of Tritium Smear Activities

Journal Article · · Health Physics
 [1];  [1]
  1. Thomas Jefferson National Accelerator Facility (TJNAF), Newport News, VA (United States)
Tritium collection efficiency varies as a function of smear media. The use of porous smear materials leads to an increase in the measured tritium activity as a function of time when the measurement is performed with liquid scintillation counters. Operational inclusion of the efficiency differences and the time dependence of the tritium smear activity is necessary to preclude inadvertently releasing materials or areas. Thomas Jefferson National Laboratory Radiological Control Department identified a contaminated stainless steel containment vessel that previously housed a target containing more than 37 TBq of tritium. The item was systematically sectioned and surveyed to compare three smear types: water-wetted cotton swabs, water-wetted paper smears, and ethanol-wetted Styrofoam wipes (NUC-Wipes™). The total activity of each section was determined using repeated decontamination. The time dependence of the measured activity was also studied. The measured activity of both paper smears and cotton swabs showed significant time dependence. The cotton swabs also showed significantly reduced collection efficiency. Given the widespread use of both of these media in routine contamination surveys, site operational limits were derived using fitted curves for time dependence and average efficiency results. In conclusion, the use of these more restrictive limits allows for rapid measurement of tritium smears while ensuring regulatory compliance.
Research Organization:
Thomas Jefferson National Accelerator Facility, Newport News, VA (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Nuclear Physics (NP)
Grant/Contract Number:
AC05-06OR23177
OSTI ID:
1785641
Report Number(s):
DOE/OR/23177--4994; JLAB-ESH--20-3217
Journal Information:
Health Physics, Journal Name: Health Physics Journal Issue: 5 Vol. 120; ISSN 0017-9078
Publisher:
Health Physics SocietyCopyright Statement
Country of Publication:
United States
Language:
English

References (5)

Assessing tritium contamination on three surfaces journal April 1995
Detecting Removable Surface Contamination journal January 1992
Wipe Testing for Surface Contamination by Tritiated Compounds journal January 1993
Adding Water to Liquid Scintillation Cocktail for Laboratory Wipe Tests journal January 1999
Use of Smears for Assessing Removable Contamination journal January 1999

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