skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Strong quantum effects in an almost classical antiferromagnet on a kagome lattice

Journal Article · · Physical Review. B, Condensed Matter and Materials Physics
 [1]
  1. Univ. of California, Irvine, CA (United States)

Two ubiquitous features of frustrated spin systems stand out: massive degeneracy of their ground states and flat, or dispersionless, excitation branches. In real materials, the former is frequently lifted by secondary interactions or quantum fluctuations, in favor of an ordered or spin-liquid state, but the latter often survive. In this paper, we demonstrate that flat modes may precipitate remarkably strong quantum effects even in the systems that are otherwise written off as almost entirely classical. The resultant spectral features should be reminiscent of the quasiparticle breakdown in quantum systems, only here the effect is strongly amplified by the flatness of spin-excitation branches, leading to the damping that is not vanishingly small even at S$$\gg$$1. We provide a theoretical analysis of excitation spectrum of the S=5/2 iron-jarosite to illustrate our findings and to suggest further studies of this and other frustrated spin systems.

Research Organization:
Univ. of California, Irvine, CA (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF)
Grant/Contract Number:
FG02-04ER46174; PHYS-1066293
OSTI ID:
1784345
Alternate ID(s):
OSTI ID: 1213962
Journal Information:
Physical Review. B, Condensed Matter and Materials Physics, Vol. 92, Issue 9; ISSN 1098-0121
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 15 works
Citation information provided by
Web of Science

References (51)

Dzyaloshinsky-Moriya Anisotropy in the Spin-1/2 Kagome Compound ZnCu 3 ( OH ) 6 Cl 2 journal July 2008
RVB description of the low-energy singlets of the spin 1/2 kagomé antiferromagnet journal October 2000
Possible Néel orderings of the Kagomé antiferromagnet journal February 1992
Antiferromagnetism. The Triangular Ising Net journal July 1950
Ghost modes and continuum scattering in the dimerized distorted kagome lattice antiferromagnet Rb$_2$Cu$_3$SnF$_{12}$ text January 2013
The ground-state phase diagram of the XXZ spin-s kagome antiferromagnet: A coupled-cluster study text January 2015
Magnon Decay in Noncollinear Quantum Antiferromagnets text January 2006
Spin Waves in the Frustrated Kagomé Lattice Antiferromagnet KFe 3 ( OH ) 6 ( SO 4 ) 2 journal June 2006
Spin-Liquid Ground State of the S = 1/2 Kagome Heisenberg Antiferromagnet journal April 2011
Order from disorder in a kagomé antiferromagnet journal August 1992
Spin tunneling in the kagomé antiferromagnet journal July 1993
Frustration and Dzyaloshinsky-Moriya anisotropy in the kagome francisites Cu 3 Bi ( SeO 3 ) 2 O 2 X   ( X   =   Br ,   Cl ) journal January 2015
Magnetic structure and spin waves in the Kagomé jarosite compound K Fe 3 ( S O 4 ) 2 ( O H ) 6 journal June 2006
Magnon Decay in Noncollinear Quantum Antiferromagnets journal November 2006
Spin waves in a triangular lattice antiferromagnet: Decays, spectrum renormalization, and singularities journal April 2009
β-Vesignieite BaCu3V2O8(OH)2: a structurally perfect S = 1/2 kagomé antiferromagnet journal January 2012
Dzyaloshinsky-Moriya interaction in vesignieite: A route to freezing in a quantum kagome antiferromagnet journal October 2013
Successive Phase Transitions and Extended Spin-Excitation Continuum in the S = 1 2 Triangular-Lattice Antiferromagnet Ba 3 CoSb 2 O 9 journal December 2012
Quasiparticle breakdown in a quantum spin liquid text January 2005
Quantum phase transition induced by Dzyaloshinskii-Moriya interactions in the kagome antiferromagnet journal October 2008
Antiferromagnetism. The Triangular Ising Net journal June 1973
Pinwheel valence-bond solid and triplet excitations in the two-dimensional deformed kagome lattice journal September 2010
The Resonating Valence Bond State in La2CuO4 and Superconductivity journal March 1987
Symmetry breaking due to Dzyaloshinsky-Moriya interactions in the kagomé lattice journal July 2002
Spin Dynamics of the Spin- 1 / 2 Kagome Lattice Antiferromagnet ZnCu 3 ( OH ) 6 Cl 2 journal March 2007
Quasiparticle breakdown in a quantum spin liquid journal March 2006
Symmetry breaking due to Dzyaloshinsky-Moriya interactions in the kagome lattice text January 2002
Quantum Selection of Order in an X X Z Antiferromagnet on a Kagome Lattice journal December 2014
Semiclassical spin dynamics of the antiferromagnetic Heisenberg model on the kagome lattice journal August 2014
Ground-state phase diagram of the XXZ spin- s kagome antiferromagnet: A coupled-cluster study journal March 2015
Spin liquids in frustrated magnets journal March 2010
Dynamics of Composite Haldane Spin Chains in IPA CuCl 3 journal February 2006
Hidden order in a frustrated system: Properties of the Heisenberg Kagomé antiferromagnet journal February 1992
Decay of quasiparticles in quantum spin liquids journal March 2006
RVB description of the low-energy singlets of the spin 1/2 kagome antiferromagnet text January 2000
Quantum dimer model for the spin- 1 2 kagome Z 2 spin liquid journal September 2014
Gapless spin-liquid phase in the kagome spin- 1 2 Heisenberg antiferromagnet journal February 2013
Cubic interactions and quantum criticality in dimerized antiferromagnets journal May 2011
Order by disorder in the classical Heisenberg kagomé antiferromagnet journal October 1993
Colloquium : Spontaneous magnon decays journal January 2013
Fractional excitations in the square-lattice quantum antiferromagnet journal December 2014
Spin Liquid State in the S = 1 / 2 Triangular Lattice Ba 3 CuSb 2 O 9 journal April 2011
Classical antiferromagnets on the Kagomé lattice journal April 1992
Fractionalized excitations in the spin-liquid state of a kagome-lattice antiferromagnet journal December 2012
Dispersionless Spin Waves and Underlying Field-Induced Magnetic Order in Gadolinium Gallium Garnet journal June 2015
Ghost modes and continuum scattering in the dimerized distorted kagome lattice antiferromagnet Rb 2 Cu 3 SnF 12 journal January 2014
Experimental Realization of a 2D Fractional Quantum Spin Liquid journal February 2001
A New Type of Antiferromagnetic Structure in the Rutile Type Crystal journal June 1959
Experimental Realization of a 2D Fractional Quantum Spin Liquid text January 2001
Order as an effect of disorder journal January 1980
Flat Bands and Wigner Crystallization in the Honeycomb Optical Lattice journal August 2007

Cited By (6)

Order and excitations in large S kagome-lattice antiferromagnets journal October 2015
Field-induced dynamical properties of the XXZ model on a honeycomb lattice journal January 2016
High-Field Expansion Approach to Kagome Antiferromagnets with Dzyaloshinskii-Moriya Interactions text January 2019
Spin clusters and low-energy excitations in rare earth kagome systems journal January 2017
High-field expansion approach to kagome antiferromagnets with Dzyaloshinskii-Moriya interactions journal September 2019
Theory of ground states for classical Heisenberg spin systems II preprint January 2017

Similar Records

Order and excitations in large-S kagomé-lattice antiferromagnets
Journal Article · Tue Oct 13 00:00:00 EDT 2015 · Physical Review. B, Condensed Matter and Materials Physics · OSTI ID:1784345

Manifolds of magnetic ordered states and excitations in the almost Heisenberg pyrochlore antiferromagnet MgCr2O4
Journal Article · Fri Apr 27 00:00:00 EDT 2018 · Physical Review B · OSTI ID:1784345

Quantum Versus Classical Spin Fragmentation in Dipolar Kagome Ice Ho 3 Mg 2 Sb 3 O 14
Journal Article · Tue Sep 29 00:00:00 EDT 2020 · Physical Review. X · OSTI ID:1784345