Dilution impacts on smoke aging: evidence in Biomass Burning Observation Project (BBOP) data

Hodshire, Anna L.; Ramnarine, Emily; Akherati, Ali; Alvarado, Matthew L.; Farmer, Delphine K.; Jathar, Shantanu H.; Kreidenweis, Sonia M.; Lonsdale, Chantelle R.; Onasch, Timothy B.; Springston, Stephen R.; Wang, Jian; Wang, Yang; Kleinman, Lawrence I.; Sedlacek III, Arthur J.; Pierce, Jeffrey R.

doi:10.5194/acp-21-6839-2021

Dilution impacts on smoke aging: evidence in Biomass Burning Observation Project (BBOP) data

Journal Article · Wed May 05 00:00:00 EDT 2021 · Atmospheric Chemistry and Physics (Online)

DOI:https://doi.org/10.5194/acp-21-6839-2021· OSTI ID:1781880

; Ramnarine, Emily; ; Alvarado, Matthew L.; ; ; ; Lonsdale, Chantelle R.; ; ; ; ; ; ;

Abstract. Biomass burning emits vapors and aerosols into the atmosphere that can rapidly evolve as smoke plumes travel downwind and dilute, affecting climate- and health-relevant properties of the smoke. To date, theory has been unable to explain observed variability in smoke evolution. Here, we use observational data from the Biomass Burning Observation Project (BBOP) field campaign and show that initial smoke organic aerosol mass concentrations can help predict changes in smoke aerosol aging markers, number concentration, and number mean diameter between 40–262 nm. Because initial field measurements of plumes are generally >10 min downwind, smaller plumes will have already undergone substantial dilution relative to larger plumes and have lower concentrations of smoke species at these observations closest to the fire. The extent to which dilution has occurred prior to the first observation is not a directly measurable quantity. We show that initial observed plume concentrations can serve as a rough indicator of the extent of dilution prior to the first measurement, which impacts photochemistry, aerosol evaporation, and coagulation. Cores of plumes have higher concentrations than edges. By segregating the observed plumes into cores and edges, we find evidence that particle aging, evaporation, and coagulation occurred before the first measurement. We further find that on the plume edges, the organic aerosol is more oxygenated, while a marker for primary biomass burning aerosol emissions has decreased in relative abundance compared to the plume cores. Finally, we attempt to decouple the roles of the initial concentrations and physical age since emission by performing multivariate linear regression of various aerosol properties (composition, size) on these two factors.

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Research Organization:: Brookhaven National Laboratory (BNL), Upton, NY (United States); Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). ARM Data Center; Washington Univ., St. Louis, MO (United States)

Sponsoring Organization:: NOAA; USDOE; USDOE Office of Science (SC), Biological and Environmental Research (BER); USDOE Office of Science (SC), Biological and Environmental Research (BER). Earth and Environmental Systems Science Division

Contributing Organization:: Argonne National Lab. (ANL), Argonne, IL (United States); Pacific Northwest National Lab. (PNNL), Richland, WA (United States)

Grant/Contract Number:: SC0012704; SC0014287; SC0019000; SC0020259

OSTI ID:: 1781880

Alternate ID(s):: OSTI ID: 1837837
OSTI ID: 1784265
OSTI ID: 1785936

Report Number(s):: BNL--221553-2021-JAAM

Journal Information:: Atmospheric Chemistry and Physics (Online), Journal Name: Atmospheric Chemistry and Physics (Online) Journal Issue: 9 Vol. 21; ISSN 1680-7324

Publisher:: Copernicus GmbHCopyright Statement

Country of Publication:: Germany

Language:: English

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