Skip to main content
U.S. Department of Energy
Office of Scientific and Technical Information

Grain growth of nanocrystalline aluminum under tensile deformation: A combined in situ TEM and atomistic study

Journal Article · · Materialia
 [1];  [2];  [2];  [2];  [1];  [3];  [3];  [2];  [2];  [1]
  1. Georgia Institute of Technology, Atlanta, GA (United States). School of Materials Science and Engineering
  2. Georgia Institute of Technology, Atlanta, GA (United States). Woodruff School of Mechanical Engineering
  3. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)

Nanocrystalline Al thin films have been strained in situ in a transmission electron microscope using two separate nanomechanical techniques involving a push-to-pull device and a microelectromechanical system (MEMS) device. Deformation-induced grain growth was observed to occur via stress-assisted grain boundary migration with extensive grain growth occurring in the necked region, indicating that the increase in local stress drives the boundary migration. Under applied tensile stresses close to the ultimate tensile strength of 450 MPa for a nanocrystalline Al specimen, measured boundary migration speeds are 0.2 – 0.7 nm s-1 for grains outside necked region and increases to 2.5 nm s-1 for grains within the necked region where the local estimated tensile stresses are elevated to around 630 MPa. By tracking grain boundary motion over time, molecular dynamics simulations showed qualitative agreement in terms of pronounced grain boundary migration with the experimental observations. The combined in situ observation and molecular dynamics simulation results underscore the important role of stress-driven grain growth in plastically deforming nanocrystalline metals, leading to intergranular fracture through predominant grain boundary sliding in regions with large localized deformation.

Research Organization:
Sandia National Laboratories (SNL-NM), Albuquerque, NM (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
AC04-94AL85000
OSTI ID:
1781569
Alternate ID(s):
OSTI ID: 1784779
Report Number(s):
SAND--2021-4967J; 695720
Journal Information:
Materialia, Journal Name: Materialia Vol. 16; ISSN 2589-1529
Publisher:
ElsevierCopyright Statement
Country of Publication:
United States
Language:
English

References (56)

Formability of Ultrafine Grained Metals Produced by Severe Plastic Deformation-An Overview journal June 2018
Fast Parallel Algorithms for Short-Range Molecular Dynamics journal March 1995
MEMS-Based Nanomechanics: Influence of MEMS Design on Test Temperature journal July 2011
The role of glide and twinning in the final separation of ruptured gold crystals journal June 1982
The ductile fracture of metals: A microstructural viewpoint journal May 1983
Grain boundary sliding-migration of aluminum 〈110〉 Σ11 {113} symmetric tilt coincidence grain boundary and its interpretation based on the motion of perfect DSC dislocations journal February 1985
Hall-petch relation in nanocrystalline solids journal April 1991
Grain boundary migration: misorientation dependence journal January 2001
On the mechanisms of grain boundary migration journal January 2002
Elastic and tensile behavior of nanocrystalline copper and palladium journal October 1997
Size effects in materials due to microstructural and dimensional constraints: a comparative review journal October 1998
Strength and ductility of ultrafine grained aluminum and iron produced by ARB and annealing journal December 2002
Direct observation of deformation-induced grain growth during the nanoindentation of ultrafine-grained Al at room temperature journal October 2004
Stress-assisted discontinuous grain growth and its effect on the deformation behavior of nanocrystalline aluminum thin films journal May 2006
Coupling grain boundary motion to shear deformation journal November 2006
In situ TEM observations of fast grain-boundary motion in stressed nanocrystalline aluminum films journal August 2008
Dislocation starvation and exhaustion hardening in Mo alloy nanofibers journal March 2012
Inter- and intragranular plasticity mechanisms in ultrafine-grained Al thin films: An in situ TEM study journal January 2013
Size effects on intergranular crack growth mechanisms in ultrathin nanocrystalline gold free-standing films journal January 2018
MEMS based nanomechanical testing method with independent electronic sensing of stress and strain journal September 2016
Grain rotations in ultrafine-grained aluminum films studied using in situ TEM straining with automated crystal orientation mapping journal January 2017
Size effect on springback behavior due to plastic strain gradient hardening in microbending process of pure aluminum foils journal June 2010
Mechanical properties of nanocrystalline materials journal May 2006
Grain-boundary kinetics: A unified approach journal October 2018
Strain-induced coarsening in nano-grained films journal February 2007
Combination of in situ straining and ACOM TEM: A novel method for analysis of plastic deformation of nanocrystalline metals journal May 2013
In-Situ HREM Studies of Grain Boundary Migration journal April 2004
Linking stress-driven microstructural evolution in nanocrystalline aluminium with grain boundary doping of oxygen journal April 2016
In situ atomistic observation of disconnection-mediated grain boundary migration journal January 2019
Electron Beam Induced Artifacts During in situ TEM Deformation of Nanostructured Metals journal November 2015
Quantitative in situ TEM tensile fatigue testing on nanocrystalline metallic ultrathin films journal January 2013
Quantifying and observing viscoplasticity at the nanoscale: highly localized deformation mechanisms in ultrathin nanocrystalline gold films journal January 2016
In situ TEM measurement of activation volume in ultrafine grained gold journal January 2020
A Model for Boundary Diffusion Controlled Creep in Polycrystalline Materials journal June 1963
A versatile microelectromechanical system for nanomechanical testing journal January 2011
Plasticity mechanisms in ultrafine grained freestanding aluminum thin films revealed by in-situ transmission electron microscopy nanomechanical testing journal March 2014
On the mechanisms of grain boundary migration journal April 1980
Duality of dislocation content of grain boundaries journal September 2006
Evidence of grain boundary dislocation step motion associated to shear-coupled grain boundary migration journal April 2013
The Deformation and Ageing of Mild Steel: III Discussion of Results journal September 1951
Plastic deformation kinetics in nanocrystalline FCC metals based on the pile-up of dislocations journal July 2007
Visualization and analysis of atomistic simulation data with OVITO–the Open Visualization Tool journal December 2009
Dislocation Models of Crystal Grain Boundaries journal May 1950
Interatomic potentials for monoatomic metals from experimental data and ab initio calculations journal February 1999
Competing plastic deformation mechanisms in nanophase metals journal July 1999
Grain-boundary sliding in nanocrystalline fcc metals journal November 2001
Atomic mechanism for dislocation emission from nanosized grain boundaries journal June 2002
Temperature and Strain-Rate Dependence of Surface Dislocation Nucleation journal January 2008
The effects on grain-boundary processes of the steps in the boundary plane associated with the cores of grain-boundary dislocations journal May 1980
A MEMS Tensile Testing Technique for Measuring True Activation Volume and Effective Stress in Nanocrystalline Ultrathin Microbeams journal October 2017
A Maximum in the Strength of Nanocrystalline Copper journal September 2003
Experimental Observations of Stress-Driven Grain Boundary Migration journal December 2009
Mechanical behavior of nanocrystalline Cu and Pd journal May 1991
In situ Transmission Electron Microscopy Observations of Toughening Mechanisms in Ultra-fine Grained Columnar Aluminum Thin Films journal July 2005
Fatigue stress concentration and notch sensitivity in nanocrystalline metals journal March 2016
Atomic Mechanisms of Grain Boundary Motion journal December 2005

Similar Records

Deformation-Twin-Induced Grain Boundary Failure
Journal Article · Sat Dec 31 23:00:00 EST 2011 · Scripta Materialia · OSTI ID:1035211

Understanding and quantifying electron beam effects during in situ TEM nanomechanical tensile testing on metal thin films
Journal Article · Tue Oct 26 00:00:00 EDT 2021 · Acta Materialia · OSTI ID:1976777

Deformation behavior in bulk nanocrystalline-ultrafine aluminum :in situ evidence of plastic strain recovery.
Journal Article · Wed Apr 01 00:00:00 EDT 2009 · Scr. Materialia · OSTI ID:1001616