MOF-Polymer Hybrid Materials: From Simple Composites to Tailored Architectures

Kalaj, Mark; Bentz, Kyle C.; Ayala, Jr., Sergio; Palomba, Joseph M.; Barcus, Kyle S.; Katayama, Yuji; Cohen, Seth M.

doi:10.1021/acs.chemrev.9b00575

MOF-Polymer Hybrid Materials: From Simple Composites to Tailored Architectures

Journal Article · Thu Jan 02 00:00:00 EST 2020 · Chemical Reviews

DOI:https://doi.org/10.1021/acs.chemrev.9b00575· OSTI ID:1779731

^[1]; Bentz, Kyle C. ^[2]; Ayala, Jr., Sergio ^[2]; Palomba, Joseph M. ^[2]; Barcus, Kyle S. ^[2]; Katayama, Yuji ^[3]; ^[2]

Univ. of California, San Diego, La Jolla, CA (United States); U.C. San Diego
Univ. of California, San Diego, La Jolla, CA (United States)
Univ. of California, San Diego, La Jolla, CA (United States); Asahi Kasei Corporation, Shizuoka (Japan)

Metal–organic frameworks (MOFs) are inherently crystalline, brittle porous solids. Conversely, polymers are flexible, malleable, and processable solids that are used for a broad range of commonly used technologies. The stark differences between the nature of MOFs and polymers has motivated efforts to hybridize crystalline MOFs and flexible polymers to produce composites that retain the desired properties of these disparate materials. Importantly, studies have shown that MOFs can be used to influence polymer structure, and polymers can be used to modulate MOF growth and characteristics. In this Review, we highlight the development and recent advances in the synthesis of MOF-polymer mixed-matrix membranes (MMMs) and applications of these MMMs in gas and liquid separations and purifications, including aqueous applications such as dye removal, toxic heavy metal sequestration, and desalination. Other elegant ways of synthesizing MOF-polymer hybrid materials, such as grafting polymers to and from MOFs, polymerization of polymers within MOFs, using polymers to template MOFs, and the bottom-up synthesis of polyMOFs and polyMOPs are also discussed. Furthermore, this review highlights recent papers in the advancement of MOF-polymer hybrid materials, as well as seminal reports that significantly advanced the field.

View Accepted Manuscript (DOE)

Research Organization:: Univ. of California, San Diego, La Jolla, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: FG02-08ER46519

OSTI ID:: 1779731

Journal Information:: Chemical Reviews, Journal Name: Chemical Reviews Journal Issue: 16 Vol. 120; ISSN 0009-2665

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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