Polymeric membranes for CO2 separation and capture

Han, Yang; Ho, W. S. Winston

doi:10.1016/j.memsci.2021.119244

Polymeric membranes for CO₂ separation and capture

Journal Article · Thu Mar 11 00:00:00 EST 2021 · Journal of Membrane Science

DOI:https://doi.org/10.1016/j.memsci.2021.119244· OSTI ID:1778643

Han, Yang ^[1]; ^[2]

The Ohio State Univ., Columbus, OH (United States); The Ohio State University
The Ohio State Univ., Columbus, OH (United States)

Over the past decade, CO₂ separation and capture have become the new bandwagon for polymer science and membrane research. This review presents the fundamentals of CO₂/gas separation in polymeric membranes and discusses how these principles underpin opportunities and challenges for post-combustion carbon capture (CO₂/N₂), hydrogen purification (CO₂/H₂), and natural gas and biogas sweetening (CO₂/CH₄). Emerging polymeric membrane materials are discussed, including a few polymers containing a high content of polar functional groups (i.e., ether oxygen-rich polymers and polymeric ionic liquids), shape-persisting glassy polymers (i.e., perfluoropolymers, thermally rearranged polymers, iptycene-containing polymers), and reactive polymers featuring facilitated transport. Moreover, the promising candidates for each CO₂ separation application are highlighted. Lastly, the permeability-selectivity data reviewed were plotted against their 2008 and 2019 upper bounds.

View Accepted Manuscript (DOE)

Research Organization:: The Ohio State Univ., Columbus, OH (United States)

Sponsoring Organization:: USDOE; USDOE Office of Fossil Energy (FE)

Grant/Contract Number:: FE0031635; FE0031731

OSTI ID:: 1778643

Alternate ID(s):: OSTI ID: 1778644
OSTI ID: 1782286

Journal Information:: Journal of Membrane Science, Journal Name: Journal of Membrane Science Vol. 628; ISSN 0376-7388

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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