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Cooperative carbon capture and steam regeneration with tetraamine-appended metal–organic frameworks

Journal Article · · Science
 [1];  [2];  [1];  [3];  [4];  [1];  [1];  [5];  [6];  [7];  [5];  [8]
  1. Department of Chemistry, University of California, Berkeley, CA 94720, USA.
  2. Department of Chemistry, University of California, Berkeley, CA 94720, USA., Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA.
  3. Department of Chemistry; University of California; Berkeley; CA 94720; USA.; Department of Chemical and Biomolecular Engineering; University of California; Berkeley; CA 94720; USA.; Berkeley Energy and Climate Institute; University of California; Berkeley; CA 94720; USA.
  4. Department of Physics; University of California; Berkeley; CA 94720; USA.; Molecular Foundry; Lawrence Berkeley National Laboratory; Berkeley; CA 94720; USA.; Computational Science Research Center; Korea Institute of Science and Technology; Seoul 02792; Republic of Korea.
  5. Corporate Strategic Research, ExxonMobil Research and Engineering Company, Annandale, NJ 08801, USA.
  6. Department of Physics, University of California, Berkeley, CA 94720, USA., Molecular Foundry, Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA., Kavli Energy Nanosciences Institute, University of California, Berkeley, CA 94720, USA.
  7. Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA., Department of Chemical and Biomolecular Engineering, University of California, Berkeley, CA 94720, USA.
  8. Department of Chemistry; University of California; Berkeley; CA 94720; USA.; Materials Sciences Division; Lawrence Berkeley National Laboratory; Berkeley; CA 94720; USA.; Department of Chemical and Biomolecular Engineering; University of California; Berkeley; CA 94720; USA.

Natural gas has become the dominant source of electricity in the United States, and technologies capable of efficiently removing carbon dioxide (CO 2 ) from the flue emissions of natural gas–fired power plants could reduce their carbon intensity. However, given the low partial pressure of CO 2 in the flue stream, separation of CO 2 is particularly challenging. Taking inspiration from the crystal structures of diamine-appended metal–organic frameworks exhibiting two-step cooperative CO 2 adsorption, we report a family of robust tetraamine-functionalized frameworks that retain cooperativity, leading to the potential for exceptional efficiency in capturing CO 2 under the extreme conditions relevant to natural gas flue emissions. The ordered, multimetal coordination of the tetraamines imparts the materials with extraordinary stability to adsorption-desorption cycling with simulated humid flue gas and enables regeneration using low-temperature steam in lieu of costly pressure or temperature swings.

Research Organization:
Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
Sponsoring Organization:
National Institutes of Health (NIH); USDOE; USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
AC02-05CH11231; AC02-06CH11357
OSTI ID:
1772272
Alternate ID(s):
OSTI ID: 1783103
Journal Information:
Science, Journal Name: Science Journal Issue: 6502 Vol. 369; ISSN 0036-8075
Publisher:
American Association for the Advancement of Science (AAAS)Copyright Statement
Country of Publication:
United States
Language:
English

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