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Tritium embrittlement of austenitic stainless-steel tubing at low helium contents

Journal Article · · Fusion Engineering and Design
Austenitic stainless steels are the standard materials for containment of hydrogen and tritium because of their resistance to mechanical property degradation in those environments. The mechanical performance of the primary containment material is critical for tritium handling, processing, and storage, thus comprehensive understanding of the processes of tritium embrittlement is an enabling capability for fusion energy. This work describes the investigation of the effects of low levels of tritium-decay-helium ingrowth on 304 L tubes. Long-term aging with tritium leads to high helium contents in austenitic stainless steels and can reduce fracture toughness by 95 %, but the details of behavior at low helium contents are not as well characterized. Here, we present results from tensile testing of tritium pre-charged 304 L tube specimens with a variety of starting microstructures that all contain a low level of helium. The results of the tritium exposed-and-aged materials are compared to previously reported results on similar specimens tested in an unexposed condition as well as the hydrogen precharged condition. Tritium precharging and aging for a short duration resulted in increased yield strengths, ultimate tensile strengths and slightly increased elongation to failure, comparable to higher concentrations of hydrogen precharging.
Research Organization:
Sandia National Laboratories (SNL-CA), Livermore, CA (United States); Savannah River Site (SRS), Aiken, SC (United States). Savannah River National Lab. (SRNL)
Sponsoring Organization:
USDOE National Nuclear Security Administration (NNSA)
Grant/Contract Number:
AC04-94AL85000; AC09-08SR22470; NA0003525
OSTI ID:
1772033
Alternate ID(s):
OSTI ID: 1833154
OSTI ID: 1776684
OSTI ID: 1782273
OSTI ID: 23194846
Report Number(s):
SAND--2021-2863J; SRNL-STI--2020-00545; 694691
Journal Information:
Fusion Engineering and Design, Journal Name: Fusion Engineering and Design Vol. 168; ISSN 0920-3796
Publisher:
ElsevierCopyright Statement
Country of Publication:
United States
Language:
English

References (10)

Hydrogen embrittlement of metals journal January 1972
Hydrogen-assisted crack propagation in 304L/308L and 21Cr–6Ni–9Mn/308L austenitic stainless steel fusion welds journal July 2012
Permeability, solubility and diffusivity of hydrogen isotopes in stainless steels at high gas pressures journal January 2007
Effects of alloy composition and strain hardening on tensile fracture of hydrogen-precharged type 316 stainless steels journal January 2008
Hydrogen compatibility of austenitic stainless steel tubing and orbital tube welds journal December 2014
Effect of microstructural and environmental variables on ductility of austenitic stainless steels journal March 2021
Tritium Aging Effects on Fracture Toughness of Stainless Steel Weldments journal April 2020
Effect of Hydrogen Isotopes on the Fracture Toughness Properties of Types 316L and 304L Stainless Steel Forgings conference November 2019
Tritium and Decay Helium Effects on Cracking Thresholds and Velocities in Stainless Steel journal March 2001
Tritium-Helium Effects in Metals journal September 1985

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