Viscosity and liquid–liquid phase separation in healthy and stressed plant SOA

Smith, Natalie R.; Crescenzo, Giuseppe V.; Huang, Yuanzhou; Hettiyadura, Anusha P. S.; Siemens, Kyla; Li, Ying; Faiola, Celia L.; Laskin, Alexander; Shiraiwa, Manabu; Bertram, Allan K.; Nizkorodov, Sergey A.

doi:10.1039/D0EA00020E

Title: Viscosity and liquid–liquid phase separation in healthy and stressed plant SOA

Journal Article · Thu Mar 25 00:00:00 EDT 2021 · Environmental Science: Atmospheres

DOI:https://doi.org/10.1039/D0EA00020E· OSTI ID:1771245

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Department of Chemistry, University of California, Irvine, Irvine, CA 92697, USA
Department of Chemistry, University of British Columbia, Vancouver, BC, Canada
Department of Chemistry, Purdue University, West Lafayette, IN 47907, USA
Department of Chemistry, University of California, Irvine, Irvine, CA 92697, USA, Department of Ecology and Evolutionary Biology, University of California Irvine, Irvine, CA, 92697, USA

Molecular composition, viscosity, and phase state were investigated for secondary organic aerosol derived from synthetic mixtures of volatile organic compounds representing emissions from healthy and aphid-stressed Scots pine trees.

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Sponsoring Organization:: USDOE

Grant/Contract Number:: SC0018349

OSTI ID:: 1771245

Journal Information:: Environmental Science: Atmospheres, Journal Name: Environmental Science: Atmospheres Vol. 1 Journal Issue: 3; ISSN 2634-3606

Publisher:: Royal Society of Chemistry (RSC)Copyright Statement

Country of Publication:: United Kingdom

Language:: English

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Volatility and Viscosity Are Correlated in Terpene Secondary Organic Aerosol Formed in a Flow Reactor Champion, Wyatt M.; Rothfuss, Nicholas E.; Petters, Markus D. Environmental Science & Technology Letters, Vol. 6, Issue 9 https://doi.org/10.1021/acs.estlett.9b00412	journal	August 2019
Global distribution of particle phase state in atmospheric secondary organic aerosols Shiraiwa, Manabu; Li, Ying; Tsimpidi, Alexandra P. Nature Communications, Vol. 8, Issue 1 https://doi.org/10.1038/ncomms15002	journal	April 2017
Mixing times of organic molecules within secondary organic aerosol particles: a global planetary boundary layer perspective Maclean, Adrian M.; Butenhoff, Christopher L.; Grayson, James W. Atmospheric Chemistry and Physics, Vol. 17, Issue 21 https://doi.org/10.5194/acp-17-13037-2017	journal	January 2017
Hygroscopic Influence on the Semisolid-to-Liquid Transition of Secondary Organic Materials Bateman, Adam P.; Bertram, Allan K.; Martin, Scot T. The Journal of Physical Chemistry A, Vol. 119, Issue 19 https://doi.org/10.1021/jp508521c	journal	November 2014
Multiple functions of inducible plant volatiles Holopainen, J. Trends in Plant Science, Vol. 9, Issue 11 https://doi.org/10.1016/j.tplants.2004.09.006	journal	November 2004
α-Pinene-Derived organic coatings on acidic sulfate aerosol impacts secondary organic aerosol formation from isoprene in a box model Schmedding, Ryan; Ma, Mutian; Zhang, Yue Atmospheric Environment, Vol. 213 https://doi.org/10.1016/j.atmosenv.2019.06.005	journal	September 2019
A single parameter representation of hygroscopic growth and cloud condensation nucleus activity Petters, M. D.; Kreidenweis, S. M. Atmospheric Chemistry and Physics, Vol. 7, Issue 8 https://doi.org/10.5194/acp-7-1961-2007	journal	January 2007
Timescales of secondary organic aerosols to reach equilibrium at various temperatures and relative humidities Li, Ying; Shiraiwa, Manabu Atmospheric Chemistry and Physics, Vol. 19, Issue 9 https://doi.org/10.5194/acp-19-5959-2019	journal	January 2019
Plant volatiles and the environment: Plant volatiles and the environment Loreto, Francesco; Dicke, Marcel; Schnitzler, JÖRg-Peter Plant, Cell & Environment, Vol. 37, Issue 8 https://doi.org/10.1111/pce.12369	journal	June 2014
Hygroscopicity of secondary organic aerosols formed by oxidation of cycloalkenes, monoterpenes, sesquiterpenes, and related compounds Varutbangkul, V.; Brechtel, F. J.; Bahreini, R. Atmospheric Chemistry and Physics, Vol. 6, Issue 9 https://doi.org/10.5194/acp-6-2367-2006	journal	January 2006
Ozone uptake on glassy, semi-solid and liquid organic matter and the role of reactive oxygen intermediates in atmospheric aerosol chemistry Berkemeier, Thomas; Steimer, Sarah S.; Krieger, Ulrich K. Physical Chemistry Chemical Physics, Vol. 18, Issue 18 https://doi.org/10.1039/C6CP00634E	journal	January 2016
Gas-phase products and secondary aerosol yields from the photooxidation of 16 different terpenes Lee, Anita; Goldstein, Allen H.; Kroll, Jesse H. Journal of Geophysical Research, Vol. 111, Issue D17 https://doi.org/10.1029/2006JD007050	journal	January 2006
Particle-Phase Diffusion Modulates Partitioning of Semivolatile Organic Compounds to Aged Secondary Organic Aerosol Zaveri, Rahul A.; Shilling, John E.; Zelenyuk, Alla Environmental Science & Technology, Vol. 54, Issue 5 https://doi.org/10.1021/acs.est.9b05514	journal	January 2020
Adsorptive uptake of water by semisolid secondary organic aerosols: Water uptake of SOA Pajunoja, Aki; Lambe, Andrew T.; Hakala, Jani Geophysical Research Letters, Vol. 42, Issue 8 https://doi.org/10.1002/2015GL063142	journal	April 2015
Joint Impacts of Acidity and Viscosity on the Formation of Secondary Organic Aerosol from Isoprene Epoxydiols (IEPOX) in Phase Separated Particles Zhang, Yue; Chen, Yuzhi; Lei, Ziying ACS Earth and Space Chemistry, Vol. 3, Issue 12 https://doi.org/10.1021/acsearthspacechem.9b00209	journal	October 2019
An overview of the Amazonian Aerosol Characterization Experiment 2008 (AMAZE-08) Martin, S. T.; Andreae, M. O.; Althausen, D. Atmospheric Chemistry and Physics, Vol. 10, Issue 23 https://doi.org/10.5194/acp-10-11415-2010	journal	January 2010
Synergy between Secondary Organic Aerosols and Long-Range Transport of Polycyclic Aromatic Hydrocarbons Zelenyuk, Alla; Imre, Dan; Beránek, Josef Environmental Science & Technology, Vol. 46, Issue 22 https://doi.org/10.1021/es302743z	journal	November 2012
Molecular chemistry of organic aerosols through the application of high resolution mass spectrometry Nizkorodov, Sergey A.; Laskin, Julia; Laskin, Alexander Physical Chemistry Chemical Physics, Vol. 13, Issue 9 https://doi.org/10.1039/c0cp02032j	journal	January 2011
Amorphous and crystalline aerosol particles interacting with water vapor: conceptual framework and experimental evidence for restructuring, phase transitions and kinetic limitations Mikhailov, E.; Vlasenko, S.; Martin, S. T. Atmospheric Chemistry and Physics, Vol. 9, Issue 24 https://doi.org/10.5194/acp-9-9491-2009	journal	January 2009

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