The Effects of Temperature on the Assembly of Gold Nanoparticle by Interpolymer Complexation

Kim, Hyeong Jin; Wang, Wenjie; Mallapragada, Surya K.; Vaknin, David

doi:10.1021/acs.jpclett.0c03749

The Effects of Temperature on the Assembly of Gold Nanoparticle by Interpolymer Complexation

Journal Article · Tue Feb 02 00:00:00 EST 2021 · Journal of Physical Chemistry Letters

DOI:https://doi.org/10.1021/acs.jpclett.0c03749· OSTI ID:1771105

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Ames Lab., and Iowa State Univ., Ames, IA (United States)
Ames Lab., Ames, IA (United States)

Using synchrotron-based small-angle X-ray scattering techniques, we demonstrate that poly(ethylene glycol)-functionalized gold nanoparticles (PEG-AuNPs) are assembled into close-packed structures that include short-range order with face-centered cubic structure, where crystalline qualities are varied by controlling the electrolyte concentration, pH, and temperature of the suspensions. Here, we show that interpolymer complexation with poly(acrylic acid) (PAA) is induced by lowering the pH level of the PEG-AuNPs suspensions, and furthermore, increasing the temperature of the suspension strengthens interparticle attraction, leading to improved supercrystal structures. Our results indicate that this strategy creates robust nanoparticle superlattices with high thermal stability. The effects of PAA and PEG chain lengths on the assemblies are also investigated, and their optimal conditions for creating improved superlattices are discussed.

View Accepted Manuscript (DOE)

Research Organization:: Ames Laboratory (AMES), Ames, IA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC02-06CH11357; AC02-07CH11358

OSTI ID:: 1771105

Alternate ID(s):: OSTI ID: 1766135
OSTI ID: 1767237

Report Number(s):: IS-J--10,438

Journal Information:: Journal of Physical Chemistry Letters, Journal Name: Journal of Physical Chemistry Letters Journal Issue: 5 Vol. 12; ISSN 1948-7185

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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