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Use of Mo/ller-Plesset Perturbation Theory in Molecular Calculations: Spectroscopic Constants of First Row Diatomic Molecules.

Journal Article · · Journal of Chemical Physics
DOI:https://doi.org/10.1063/1.476308· OSTI ID:1770379
The convergence of Mo/ller–Plesset perturbation expansions (MP2–MP4/MP5) for the spectroscopic constants of a selected set of diatomic molecules (BH, CH, HF, N2, CO, and F2) has been investigated. It was found that the second-order perturbation contributions to the spectroscopic constants are strongly dependent on basis set, more so for HF and CO than for BH.
Research Organization:
Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)
Sponsoring Organization:
USDOE
DOE Contract Number:
AC05-76RL01830
OSTI ID:
1770379
Report Number(s):
PNNL-SA-29506
Journal Information:
Journal of Chemical Physics, Journal Name: Journal of Chemical Physics Journal Issue: 12 Vol. 108; ISSN 0021-9606
Country of Publication:
United States
Language:
English

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