Transition metal-based bimetallic MOFs and MOF-derived catalysts for electrochemical oxygen evolution reaction

Li, Songsong; Gao, Yangqin; Li, Ning; Ge, Lei; Bu, Xianhui; Feng, Pingyun

doi:10.1039/d0ee03697h

Transition metal-based bimetallic MOFs and MOF-derived catalysts for electrochemical oxygen evolution reaction

Journal Article · Fri Mar 05 00:00:00 EST 2021 · Energy & Environmental Science

DOI:https://doi.org/10.1039/d0ee03697h· OSTI ID:1843741

Li, Songsong ^[1]; Gao, Yangqin ^[2]; ^[2]; Ge, Lei ^[2]; ^[3]; ^[4]

China Univ. of Petroleum Beijing (China); Univ. of California, Riverside, CA (United States); UC Riverside
China Univ. of Petroleum Beijing (China)
California State Univ. (CalState), Long Beach, CA (United States)
Univ. of California, Riverside, CA (United States)

The oxygen evolution reaction (OER) is a critical electrochemical reaction in water splitting and rechargeable metal–air batteries. It plays a pivotal role in achieving high-efficiency clean-energy production and energy storage in these devices. Transition metal-based bimetallic MOFs (TMB MOFs) with two different metal ions possess specific synergistic effects, which could exhibit OER performance and stability superior to those of the corresponding monometallic MOFs for water oxidation. Benefiting from the diversity of chemical composition and structural type, TMB MOFs can also serve as precursors and templates to obtain alloy-particle-decorated carbon materials with high surface area, or metal compounds such as bimetallic sulfides, phosphides, and hydroxides with atomic-level mixing of heterometallic elements. These materials with high-density active sites exhibit much improved catalytic activity in the water oxidation reaction. Furthermore, this article aims to review the recent progress with TMB MOFs and their derivatives in relation to applications as electrocatalysts in OER, including analysis of the mechanism of the OER process with the assistance of DFT calculations and in situ or operando techniques.

View Accepted Manuscript (DOE)

Research Organization:: Univ. of California, Riverside, CA (United States)

Sponsoring Organization:: USDOE; USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0010596

OSTI ID:: 1843741

Alternate ID(s):: OSTI ID: 1769452

Journal Information:: Energy & Environmental Science, Journal Name: Energy & Environmental Science Journal Issue: 4 Vol. 14; ISSN 1754-5692

Publisher:: Royal Society of ChemistryCopyright Statement

Country of Publication:: United States

Language:: English

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