Measurement of distribution coefficients on TODGA resin and development of a group separation for mixed activation and fission product samples

Louie, Christina A.; Morrison, Erin C.; Thomas, May-Lin; Arrigo, Leah M.; Seiner, Brienne N.

doi:10.1007/s10967-020-07460-7

Measurement of distribution coefficients on TODGA resin and development of a group separation for mixed activation and fission product samples

Journal Article · Mon Nov 30 23:00:00 EST 2020 · Journal of Radioanalytical & Nuclear Chemistry

DOI:https://doi.org/10.1007/s10967-020-07460-7· OSTI ID:1764026

Louie, Christina A. ^[1]; Morrison, Erin C. ^[2]; Thomas, May-Lin ^[3]; Arrigo, Leah M. ^[2]; Seiner, Brienne N. ^[2]

WASHINGTON STATE UNIV
BATTELLE (PACIFIC NW LAB)
PNNL

Batch equilibrium experiments were performed to determine the distribution coefficients for Sc, Ir, and Ta on N,N,N’,N’tetraoctyl-1,5-diglycolamide (TODGA) resin in various acid matrices. Distribution coefficients were determined in hydrochloric acid (Sc, Ir), nitric acid (Sc, Ta), and a mixture of nitric acid and 0.2M hydrofluoric acid (Sc, Ir, Ta). The distribution coefficients determined through these experiments were then utilized to create a group separation method for activation products, fission products, and environmental constituents.

Research Organization:: Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)

Sponsoring Organization:: USDOE

DOE Contract Number:: AC05-76RL01830

OSTI ID:: 1764026

Report Number(s):: PNNL-SA-156231

Journal Information:: Journal of Radioanalytical & Nuclear Chemistry, Journal Name: Journal of Radioanalytical & Nuclear Chemistry Journal Issue: 3 Vol. 326

Country of Publication:: United States

Language:: English

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