Split-pulse X-ray photon correlation spectroscopy with seeded X-rays from X-ray laser to study atomic-level dynamics

Shinohara, Yuya; Osaka, Taito; Inoue, Ichiro; Iwashita, Takuya; Dmowski, Wojciech; Ryu, Chae Woo; Sarathchandran, Yadu; Egami, Takeshi

doi:10.1038/s41467-020-20036-z

Title: Split-pulse X-ray photon correlation spectroscopy with seeded X-rays from X-ray laser to study atomic-level dynamics

Journal Article · Fri Dec 04 00:00:00 EST 2020 · Nature Communications

DOI:https://doi.org/10.1038/s41467-020-20036-z· OSTI ID:1731015

; Osaka, Taito; Inoue, Ichiro;

; Dmowski, Wojciech;

; Sarathchandran, Yadu;

Abstract With their brilliance and temporal structure, X-ray free-electron laser can unveil atomic-scale details of ultrafast phenomena. Recent progress in split-and-delay optics (SDO), which produces two X-ray pulses with time-delays, offers bright prospects for observing dynamics at the atomic-scale. However, their insufficient pulse energy has limited its application either to phenomena with longer correlation length or to measurement with a fixed delay-time. Here we show that the combination of the SDO and self-seeding of X-rays increases the pulse energy and makes it possible to observe the atomic-scale dynamics in a timescale of picoseconds. We show that the speckle contrast in scattering from water depends on the delay-time as expected. Our results demonstrate the capability of measurement using the SDO with seeded X-rays for resolving the dynamics in temporal and spatial scales that are not accessible by other techniques, opening opportunities for studying the atomic-level dynamics.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division; Japan Society for the Promotion of Science (JSPS)

Grant/Contract Number:: AC05-00OR22725; 18K18307; 19K20604; 2018B8041; 2019A8043; 2019B8011

OSTI ID:: 1731015

Alternate ID(s):: OSTI ID: 1735454

Journal Information:: Nature Communications, Journal Name: Nature Communications Vol. 11 Journal Issue: 1; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United Kingdom

Language:: English

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