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Title: Detailed measurements of transient two-stage ignition and combustion processes in high-pressure spray flames using simultaneous high-speed formaldehyde PLIF and schlieren imaging

Journal Article · · Proceedings of the Combustion Institute

This study investigates the low- and high-temperature ignition and combustion processes in a high-pressure spray flame of n-dodecane using simultaneous 50-kHz formaldehyde (HCHO) planar laser-induced fluorescence (PLIF) and 100-kHz schlieren imaging. The PLIF measurements were facilitated through the use of a pulse-burst-mode Nd:YAG laser, producing a 355-nm pulse-train with 300 pulses at 70 mJ/pulse, separated by 20-µs, in a 6-ms burst. The high-speed HCHO PLIF signal was imaged using a non-intensified CMOS camera with dynamic background emission correction. The acquisition rate of this HCHO PLIF diagnostic is unique to the research community, and when combined with high-speed schlieren imaging, provides unprecedented opportunity for analysis of the spatiotemporal evolution of fuel jet penetration and low- and high-temperature ignition processes relevant to internal combustion engine conditions. The present experiments are conducted in the Sandia constant-volume preburn vessel equipped with a new Spray A injector. The influences of ambient conditions are examined on the ignition delay times of the two-stage ignition events, HCHO structures, and lift-off length values. Consistent with past studies of traditional Spray A flames, the formation of HCHO is first observed in the jet peripheries where the equivalence ratio (Φ) is expected to be leaner and hotter and then grows in size and in intensity downstream into the jet core where Φ is expected to be richer and colder. The measurements demonstrate that the formation and propagation of HCHO from the leaner to richer region leads to high-temperature ignition events, supporting the identification of a phenomenon coined “cool-flame wave propagation” during the transient ignition process. Subsequent high-temperature ignition is found to consume the previously formed HCHO in the jet head, while the formation of HCHO persists in the fuel-rich zone near the flame base over the entire combustion period.

Research Organization:
Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
Sponsoring Organization:
USDOE National Nuclear Security Administration (NNSA)
Grant/Contract Number:
NA0003525
OSTI ID:
1720207
Alternate ID(s):
OSTI ID: 1870504
Report Number(s):
SAND2022-4993J; S1540748920306878; PII: S1540748920306878
Journal Information:
Proceedings of the Combustion Institute, Journal Name: Proceedings of the Combustion Institute Vol. 38 Journal Issue: 4; ISSN 1540-7489
Publisher:
ElsevierCopyright Statement
Country of Publication:
United States
Language:
English

References (25)

Combustion structure of free and wall-impinging diesel jets by simultaneous laser-induced fluorescence of formaldehyde, poly-aromatic hydrocarbons, and hydroxides journal June 2008
Visualization of Ignition Processes in High-Pressure Sprays with Multiple Injections of n-Dodecane journal January 2015
Transient Flame Development in a Constant-Volume Vessel Using a Split-Scheme Injection Strategy journal March 2017
Entrainment Waves in Diesel Jets journal April 2009
Importance of turbulence-chemistry interactions at low temperature engine conditions journal September 2017
Characterization of Spray A flame structure for parametric variations in ECN constant-volume vessels using chemiluminescence and laser-induced fluorescence journal December 2016
Diesel Spray Ignition Detection and Spatial/Temporal Correction journal January 2012
Schlieren Methodology for the Analysis of Transient Diesel Flame Evolution journal May 2013
Development and validation of an n-dodecane skeletal mechanism for spray combustion applications journal March 2014
Relationship Between Ignition Processes and the Lift-Off Length of Diesel Fuel Jets conference October 2005
Large eddy simulation of n-Dodecane spray combustion in a high pressure combustion vessel journal December 2014
Understanding the ignition mechanism of high-pressure spray flames journal January 2017
LES of a premixed jet flame DNS using a strained flamelet model journal December 2013
Formaldehyde laser-induced fluorescence imaging with a multi-band transmission filter journal January 2014
Experimental study of the stabilization mechanism of a lifted Diesel-type flame using combined optical diagnostics and laser-induced plasma ignition journal November 2018
Diesel fuel jet lift-off stabilization in the presence of laser-induced plasma ignition journal January 2009
The potential of on- and off-resonant formaldehyde imaging combined with bootstrapping in diesel sprays journal August 2017
Relationship Between Diesel Fuel Spray Vapor Penetration/Dispersion and Local Fuel Mixture Fraction journal April 2011
Experimental characterization of diesel ignition and lift-off length using a single-hole ECN injector journal September 2013
Large-eddy simulation on the influence of injection pressure in reacting Spray A journal May 2018
Comparison of Diesel Spray Combustion in Different High-Temperature, High-Pressure Facilities journal August 2010
Simultaneous formaldehyde PLIF and high-speed schlieren imaging for ignition visualization in high-pressure spray flames journal January 2015
Formaldehyde Visualization Near Lift-off Location in a Diesel Jet conference October 2006
Large eddy simulation of a reacting spray flame with multiple realizations under compression ignition engine conditions journal December 2015
Two-stage autoignition and edge flames in a high pressure turbulent jet journal July 2017