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Ozone transfer through the gas-solution interface during oxidative dissolution of plutonium dioxide

Journal Article · · Radiochemistry
OSTI ID:171781
;  [1]
  1. Khlopin Radium Inst., St. Petersburg (Russian Federation)
The rate of the ozone transfer through the gas-solution interface into 4 M HNO{sub 3} containing 1.5 x 10{sup {minus}2} M or no Ce has been evaluated. This rate is almost equal to the transfer rate in oxidative dissolution of PuO{sub 2} under the similar conditions and at (PuO{sub 2}){sub O} above 0.1 mol 1{sup {minus}1} solvent. The rate-determining stages of PuO{sub 2} dissolution under experimental conditions varying in a wide range have been elucidated.
OSTI ID:
171781
Journal Information:
Radiochemistry, Journal Name: Radiochemistry Journal Issue: 3 Vol. 37; ISSN RDIOEO; ISSN 1066-3622
Country of Publication:
United States
Language:
English