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Performance Assessment of Portable Optical Particle Spectrometer (POPS)

Journal Article · · Sensors
DOI:https://doi.org/10.3390/s20216294· OSTI ID:1713325
Accurate representation of atmospheric aerosol properties is a long-standing problem in atmospheric research. Modern pilotless aerial systems provide a new platform for atmospheric in situ measurement. However, small airborne platforms require miniaturized instrumentation due to apparent size, power, and weight limitations. A Portable Optical Particle Spectrometer (POPS) is an emerged instrument to measure ambient aerosol size distribution with high time and size resolution, designed for deployment on a small unmanned aerial system (UAS) or tethered balloon system (TBS) platforms. This study evaluates the performance of a POPS with an upgraded laser heater and additional temperature sensors in the aerosol pathway. POPS maintains its performance under different environmental conditions as long as the laser temperature remains above 25 °C and the aerosol flow temperature inside the optical chamber is 15 °C higher than the ambient temperature. The comparison between POPS and an Ultra-High Sensitivity Aerosol Spectrometer (UHSAS) suggests that the coincidence error is less than 25% when the number concentration is less than 4000 cm–3. The size distributions measured by both of them remained unaffected up to 15,000 cm–3. While both instruments’ sizing accuracy is affected by the aerosol chemical composition and morphology, the influence is more profound on the POPS.
Research Organization:
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Atmospheric Radiation Measurement (ARM); Pacific Northwest National Laboratory (PNNL), Richland, WA (United States). Environmental Molecular Sciences Laboratory (EMSL)
Sponsoring Organization:
USDOE Office of Science (SC), Biological and Environmental Research (BER)
Contributing Organization:
PNNL, BNL, ANL, ORNL
Grant/Contract Number:
AC05-76RL01830; AC06-76RL01830
OSTI ID:
1713325
Alternate ID(s):
OSTI ID: 1721588
Report Number(s):
PNNL-SA--156649
Journal Information:
Sensors, Journal Name: Sensors Journal Issue: 21 Vol. 20; ISSN 1424-8220
Publisher:
MDPI AGCopyright Statement
Country of Publication:
United States
Language:
English

References (47)

Ueber die Berechnung der Expansivkraft des Wasserdunstes journal January 1828
Versuche über die Spannkräfte des Wasserdampfs journal January 1844
Beiträge zur Optik trüber Medien, speziell kolloidaler Metallösungen journal January 1908
Deployment of an unmanned aerial system to assist in mapping an intermittent stream: Scientific Briefing journal September 2015
Novel optical techniques for measurements of light extinction, scattering and absorption by single aerosol particles: Light extinction by single aerosols journal March 2011
Pollution and the planetary albedo journal December 1974
Effect of relative humidity on the size of atmospheric aerosol particles journal November 1974
Techniques for collection of representative aerosol samples journal August 1974
Application of the T-Matrix Method to the Measurement of Aspherical (Ellipsoidal) Particles with Forward Scattering Optical Particle Counters journal July 2000
Dispersion-equation coefficients for the refractive index and birefringence of calcite and quartz crystals journal May 1999
Aerosol light scattering measurements as a function of relative humidity: a comparison between measurements made at three different sites journal October 2001
A review of atmospheric aerosol measurements journal January 2000
Deliquescence and efflorescence behavior of individual NaCl and KCl mixture aerosol particles journal January 2014
Performance characteristics of the ultra high sensitivity aerosol spectrometer for particles between 55 and 800nm: Laboratory and field studies journal September 2008
Characterizing the performance of two optical particle counters (Grimm OPC1.108 and OPC1.109) under urban aerosol conditions journal October 2010
Field comparison of a personal cascade impactor sampler, an optical particle counter and CEN-EU standard methods for PM10, PM2.5 and PM1 measurement in urban environment journal November 2013
Optical particle spectrometry—Problems and prospects journal July 2009
Efflorescence Relative Humidity for Ammonium Sulfate Particles journal June 2006
A laboratory investigation of light scattering from representative components of mineral dust aerosol at a wavelength of 550 nm journal January 2008
From Agglomerates of Spheres to Irregularly Shaped Particles: Determination of Dynamic Shape Factors from Measurements of Mobility and Vacuum Aerodynamic Diameters journal March 2006
Sources of Error and Uncertainty in the Use of Cavity Ring Down Spectroscopy to Measure Aerosol Optical Properties journal November 2011
A Calibration Technique for Improving Refractive Index Retrieval from Aerosol Cavity Ring-Down Spectroscopy journal September 2013
Evaluation of DMA Size Selection of Dry Dispersed Mineral Dust Particles journal June 2015
A light-weight, high-sensitivity particle spectrometer for PM2.5 aerosol measurements journal December 2015
A practical set of miniaturized instruments for vertical profiling of aerosol physical properties journal March 2017
Refractive index retrievals for polystyrene latex spheres in the spectral range 220–420 nm journal June 2017
Mobility particle size spectrometers: Calibration procedures and measurement uncertainties journal October 2017
Scanning Electrical Mobility Spectrometer journal January 1990
Particle Morphology and Density Characterization by Combined Mobility and Aerodynamic Diameter Measurements. Part 1: Theory journal January 2004
Influence of Particle Refractive Index on the Lower Detection Limit of Light Scattering Aerosol Counters journal January 1996
On Differential Mobility Analyzer Resolution journal June 1999
Development of an autonomous unmanned aerial system for atmospheric data collection and research conference May 2016
Improved Magnus Form Approximation of Saturation Vapor Pressure journal April 1996
Development and Testing of Instrumentation for UAV-Based Flux Measurements within Terrestrial and Marine Atmospheric Boundary Layers journal July 2013
Airborne Aerosol in Situ Measurements during TCAP: A Closure Study of Total Scattering journal July 2015
An Overview of Particulate Matter Measurement Instruments journal September 2015
Unmanned Aerial Systems for Monitoring Trace Tropospheric Gases journal October 2017
Development and Validation of a UAV Based System for Air Pollution Measurements journal December 2016
Effects of relative humidity on aerosol light scattering in the Arctic journal January 2010
Effects of relative humidity on aerosol light scattering: results from different European sites journal January 2013
A new method for measuring optical scattering properties of atmospherically relevant dusts using the Cloud and Aerosol Spectrometer with Polarization (CASPOL) journal January 2013
Global indirect aerosol effects: a review journal January 2005
Prompt deliquescence and efflorescence of aerosol nanoparticles journal January 2006
Modification, calibration, and performance of the Ultra-High Sensitivity Aerosol Spectrometer for particle size distribution and volatility measurements during the Atmospheric Tomography Mission (ATom) airborne campaign journal January 2018
Aerosol size distributions during the Atmospheric Tomography Mission (ATom): methods, uncertainties, and data products journal January 2019
Humidity effects on the detection of soluble and insoluble nanoparticles in butanol operated condensation particle counters journal January 2019
Calibration of the passive cavity aerosol spectrometer probe for airborne determination of the size distribution journal January 2013

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