Minimizing Current and Voltage Losses to Reach 25% Efficient Monolithic Two-Terminal Perovskite–Silicon Tandem Solar Cells

Bush, Kevin A.; Manzoor, Salman; Frohna, Kyle; Yu, Zhengshan J.; Raiford, James A.; Palmstrom, Axel F.; Wang, Hsin-Ping; Prasanna, Rohit; Bent, Stacey F.; Holman, Zachary C.; McGehee, Michael D.

doi:10.1021/acsenergylett.8b01201

Minimizing Current and Voltage Losses to Reach 25% Efficient Monolithic Two-Terminal Perovskite–Silicon Tandem Solar Cells

Journal Article · Mon Aug 20 00:00:00 EDT 2018 · ACS Energy Letters

DOI:https://doi.org/10.1021/acsenergylett.8b01201· OSTI ID:1693709

^[1]; Manzoor, Salman ^[2]; Frohna, Kyle ^[3]; Yu, Zhengshan J. ^[2]; Raiford, James A. ^[4]; Palmstrom, Axel F. ^[4]; Wang, Hsin-Ping ^[4]; ^[4]; ^[4]; Holman, Zachary C. ^[2]; ^[5]

Stanford Univ., CA (United States); University of Colorado Boulder
Arizona State Univ., Tempe, AZ (United States)
Stanford Univ., CA (United States); Trinity College, Dublin (Ireland)
Stanford Univ., CA (United States)
Stanford Univ., CA (United States); Univ. of Colorado, Boulder, CO (United States)

The rapid rise in efficiency and tunable bandgap of metal-halide perovskites makes them highly attractive for use in tandems on silicon. Recently we demonstrated a perovskite–silicon monolithic two-terminal tandem with 23.6% power conversion efficiency. Here, we present work on optical optimization to improve light harvesting that includes thinning out the top transparent electrode to reduce front-surface reflection and parasitic absorption; introducing metal fingers to minimize series resistance losses; and further minimizing reflection loss with a polydimethylsiloxane (PDMS) stamp with random, pyramidal texture. Additionally, to reduce voltage loss while achieving current matching, we employ poly[bis(4-phenyl)(2,4,6-trimethylphenyl)amine] (PTAA) as a hole transport material instead of NiO_x and a wider 1.68 eV bandgap perovskite composition. Furthermore, these optimizations boost the open-circuit voltage to 1.77 V and the short-circuit current density to 18.4 mA/cm², culminating in a 25% efficient perovskite–silicon tandem with a 1 cm² active area.

View Accepted Manuscript (DOE)

Research Organization:: Stanford Univ., CA (United States)

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE), Renewable Power Office. Solar Energy Technologies Office

Grant/Contract Number:: EE0008167

OSTI ID:: 1693709

Alternate ID(s):: OSTI ID: 1539559

Journal Information:: ACS Energy Letters, Journal Name: ACS Energy Letters Journal Issue: 9 Vol. 3; ISSN 2380-8195

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

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