Generation of bright phase-matched circularly-polarized extreme ultraviolet high harmonics

Kfir, Ofer; Grychtol, Patrik; Turgut, Emrah; Knut, Ronny; Zusin, Dmitriy; Popmintchev, Dimitar; Popmintchev, Tenio; Nembach, Hans; Shaw, Justin M.; Fleischer, Avner; Kapteyn, Henry; Murnane, Margaret; Cohen, Oren

doi:10.1038/nphoton.2014.293

Generation of bright phase-matched circularly-polarized extreme ultraviolet high harmonics

Journal Article · Mon Dec 08 00:00:00 EST 2014 · Nature Photonics

DOI:https://doi.org/10.1038/nphoton.2014.293· OSTI ID:1682255

^[1]; ^[2]; Turgut, Emrah ^[2]; Knut, Ronny ^[3]; Zusin, Dmitriy ^[2]; Popmintchev, Dimitar ^[2]; Popmintchev, Tenio ^[2]; Nembach, Hans ^[3]; Shaw, Justin M. ^[4]; Fleischer, Avner ^[5]; Kapteyn, Henry ^[2]; Murnane, Margaret ^[2]; Cohen, Oren ^[6]

Solid State Inst. and Physics Department, Haifa (Israel); JILA/University of Colorado Boulder
Univ. of Colorado, Boulder, CO (United States)
Univ. of Colorado, Boulder, CO (United States); National Inst. of Standards and Technology (NIST), Boulder, CO (United States)
National Inst. of Standards and Technology (NIST), Boulder, CO (United States)
Solid State Institute and Physics Department, Haifa (Israel); Ort Braude College, Karmiel (Israel)
Solid State Inst. and Physics Department, Haifa (Israel)

Circularly-polarized extreme ultraviolet and X-ray radiation is useful for analysing the structural, electronic and magnetic properties of materials. To date, such radiation has only been available at large-scale X-ray facilities such as synchrotrons. Here, we demonstrate the first bright, phase-matched, extreme ultraviolet circularly-polarized high harmonics source. The harmonics are emitted when bi-chromatic counter-rotating circularly-polarized laser pulses field-ionize a gas in a hollow-core waveguide. We use this new light source for magnetic circular dichroism measurements at the M-shell absorption edges of Co. We show that phase-matching of circularly-polarized harmonics is unique and robust, producing a photon flux comparable to linearly polarized high harmonic sources. Furthermore, this work represents a critical advance towards the development of table-top systems for element-specific imaging and spectroscopy of multiple elements simultaneously in magnetic and other chiral media with very high spatial and temporal resolution.

View Accepted Manuscript (DOE)

Research Organization:: Univ. of Colorado, Boulder, CO (United States)

Sponsoring Organization:: Israel Science Foundation; USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division

Grant/Contract Number:: SC0002002

OSTI ID:: 1682255

Journal Information:: Nature Photonics, Journal Name: Nature Photonics Journal Issue: 2 Vol. 9; ISSN 1749-4885

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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High-order harmonic generation with twisted electrons Gemsheim, Sebastian; Rost, Jan-Michael Physical Review A, Vol. 100, Issue 4 https://doi.org/10.1103/physreva.100.043408	journal	October 2019
Pulse-length effects in strong-field ionization of atoms by co-rotating and counter-rotating bicircular laser pulses Abu-samha, Mahmoud; Madsen, Lars Bojer Physical Review A, Vol. 100, Issue 4 https://doi.org/10.1103/physreva.100.043415	journal	October 2019
Spectroscopy of atomic orbital sizes using bi-elliptical high-order harmonic generation Bordo, Eliyahu; Neufeld, Ofer; Kfir, Ofer Physical Review A, Vol. 100, Issue 4 https://doi.org/10.1103/physreva.100.043419	journal	October 2019
Modeling tomographic measurements of photoelectron vortices in counter-rotating circularly polarized laser pulses Armstrong, G. S. J.; Clarke, D. D. A.; Benda, J. Physical Review A, Vol. 100, Issue 6 https://doi.org/10.1103/physreva.100.063416	journal	December 2019
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Interference effect in high-order harmonic generation from degenerate current-carrying orbitals of polyatomic molecules Wang, Dian; Zhu, Xiaosong; Yuan, Hua Physical Review A, Vol. 101, Issue 2 https://doi.org/10.1103/physreva.101.023406	journal	February 2020
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Schemes for generation of isolated attosecond pulses of pure circular polarization Hernández-García, C.; Durfee, C. G.; Hickstein, D. D. Physical Review A, Vol. 93, Issue 4 https://doi.org/10.1103/physreva.93.043855	journal	April 2016
Possibility of introducing spin into attoscience with spin-polarized electrons produced by a bichromatic circularly polarized laser field Milošević, D. B. Physical Review A, Vol. 93, Issue 5 https://doi.org/10.1103/physreva.93.051402	journal	May 2016
Controlling electron-ion rescattering in two-color circularly polarized femtosecond laser fields Mancuso, Christopher A.; Hickstein, Daniel D.; Dorney, Kevin M. Physical Review A, Vol. 93, Issue 5 https://doi.org/10.1103/physreva.93.053406	journal	May 2016
Improved strong-field approximation and quantum-orbit theory: Application to ionization by a bicircular laser field Milošević, D. B.; Becker, W. Physical Review A, Vol. 93, Issue 6 https://doi.org/10.1103/physreva.93.063418	journal	June 2016
Multistart spiral electron vortices in ionization by circularly polarized UV pulses Ngoko Djiokap, J. M.; Meremianin, A. V.; Manakov, N. L. Physical Review A, Vol. 94, Issue 1 https://doi.org/10.1103/physreva.94.013408	journal	July 2016
Selection rules of high-order-harmonic generation: Symmetries of molecules and laser fields Liu, Xi; Zhu, Xiaosong; Li, Liang Physical Review A, Vol. 94, Issue 3 https://doi.org/10.1103/physreva.94.033410	journal	September 2016
Trajectory analysis of high-order-harmonic generation from periodic crystals Ikemachi, Takuya; Shinohara, Yasushi; Sato, Takeshi Physical Review A, Vol. 95, Issue 4 https://doi.org/10.1103/physreva.95.043416	journal	April 2017
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Electron rotational asymmetry in strong-field photodetachment from F − by circularly polarized laser pulses Armstrong, G. S. J.; Clarke, D. D. A.; Brown, A. C. Physical Review A, Vol. 99, Issue 2 https://doi.org/10.1103/physreva.99.023429	journal	February 2019
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Probing ultrafast spin dynamics with high-harmonic magnetic circular dichroism spectroscopy Willems, F.; Smeenk, C. T. L.; Zhavoronkov, N. Physical Review B, Vol. 92, Issue 22 https://doi.org/10.1103/physrevb.92.220405	journal	December 2015
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Controlling Nonsequential Double Ionization in Two-Color Circularly Polarized Femtosecond Laser Fields Mancuso, Christopher A.; Dorney, Kevin M.; Hickstein, Daniel D. Physical Review Letters, Vol. 117, Issue 13 https://doi.org/10.1103/physrevlett.117.133201	journal	September 2016
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Attoclock Photoelectron Interferometry with Two-Color Corotating Circular Fields to Probe the Phase and the Amplitude of Emitting Wave Packets Han, Meng; Ge, Peipei; Shao, Yun Physical Review Letters, Vol. 120, Issue 7 https://doi.org/10.1103/physrevlett.120.073202	journal	February 2018
Optical Chirality in Nonlinear Optics: Application to High Harmonic Generation Neufeld, Ofer; Cohen, Oren Physical Review Letters, Vol. 120, Issue 13 https://doi.org/10.1103/physrevlett.120.133206	journal	March 2018
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Conservation of Torus-knot Angular Momentum in High-order Harmonic Generation Pisanty, Emilio; Rego, Laura; San Román, Julio Physical Review Letters, Vol. 122, Issue 20 https://doi.org/10.1103/physrevlett.122.203201	journal	May 2019
Magneto-Optical Functions at the 3 p Resonances of Fe, Co, and Ni: Ab initio Description and Experiment Willems, F.; Sharma, S.; v. Korff Schmising, C. Physical Review Letters, Vol. 122, Issue 21 https://doi.org/10.1103/physrevlett.122.217202	journal	May 2019
Background-Free Measurement of Ring Currents by Symmetry-Breaking High-Harmonic Spectroscopy Neufeld, Ofer; Cohen, Oren Physical Review Letters, Vol. 123, Issue 10 https://doi.org/10.1103/physrevlett.123.103202	journal	September 2019
Attosecond-Scale Streaking Methods for Strong-Field Ionization by Tailored Fields Eicke, Nicolas; Brennecke, Simon; Lein, Manfred Physical Review Letters, Vol. 124, Issue 4 https://doi.org/10.1103/physrevlett.124.043202	journal	January 2020
Spin-constrained orbital-angular-momentum control in high-harmonic generation Kong, F.; Zhang, C.; Larocque, H. Physical Review Research, Vol. 1, Issue 3 https://doi.org/10.1103/physrevresearch.1.032008	journal	October 2019
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Controlling Subcycle Optical Chirality in the Photoionization of Chiral Molecules Rozen, S.; Comby, A.; Bloch, E. Physical Review X, Vol. 9, Issue 3 https://doi.org/10.1103/physrevx.9.031004	journal	July 2019
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Interferometric control of the ellipticity of a femtosecond extreme ultraviolet source Gruson, V.; Weber, S. J.; Barreau, L. Journal of the Optical Society of America B, Vol. 35, Issue 4 https://doi.org/10.1364/josab.35.000a15	journal	January 2018
Spectral shifts and asymmetries in mid-infrared assisted high-order harmonic generation Major, Balázs; Balogh, Emeric; Kovács, Katalin Journal of the Optical Society of America B, Vol. 35, Issue 4 https://doi.org/10.1364/josab.35.000a32	journal	January 2018
Study of the circular dichroism of He ⁺ ion Chen, Jen-Hao; Liu, Jinn-Liang; Jheng, Shih-Da Journal of the Optical Society of America B, Vol. 36, Issue 12 https://doi.org/10.1364/josab.36.003597	journal	January 2019
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Isolated elliptically polarized attosecond soft X-ray with high-brilliance using polarization gating of harmonics from relativistic plasmas at oblique incidence Chen, Zi-Yu; Li, Xiao-Ya; Li, Bo-Yuan Optics Express, Vol. 26, Issue 4 https://doi.org/10.1364/oe.26.004572	journal	January 2018
Helicity asymmetry in strong-field ionization of atoms by a bicircular laser field Gazibegović-Busuladžić, A.; Becker, W.; Milošević, D. B. Optics Express, Vol. 26, Issue 10 https://doi.org/10.1364/oe.26.012684	journal	January 2018
All-optical characterization of the two-dimensional waveform and the Gouy phase of an infrared pulse based on plasma fluorescence of gas Saito, Nariyuki; Ishii, Nobuhisa; Kanai, Teruto Optics Express, Vol. 26, Issue 19 https://doi.org/10.1364/oe.26.024591	journal	January 2018
Polarization-based tachometer for measuring spinning rotors Prost, Emilien; Hertz, Edouard; Billard, Franck Optics Express, Vol. 26, Issue 24 https://doi.org/10.1364/oe.26.031839	journal	January 2018
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Circularly polarized extreme ultraviolet high harmonic generation in graphene Chen, Zi-Yu; Qin, Rui Optics Express, Vol. 27, Issue 3 https://doi.org/10.1364/oe.27.003761	journal	January 2019
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Observation of selection rules for circularly polarized fields in high-harmonic generation from a crystalline solid Saito, Nariyuki; Xia, Peiyu; Lu, Faming Optica, Vol. 4, Issue 11 https://doi.org/10.1364/optica.4.001333	journal	January 2017
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Generating circularly polarized radiation in the extreme ultraviolet spectral range at the free-electron laser FLASH Korff Schmising, Clemens Von; Weder, David; Noll, Tino Technische Universität Berlin https://doi.org/10.14279/depositonce-10039	text	January 2017
Attosecond control of spin polarization in electron–ion recollision driven by intense tailored fields Ayuso, David; Jimenez Galan, Alvaro; Morales, Felipe Humboldt-Universität zu Berlin https://doi.org/10.18452/24375	text	January 2017
High harmonic interferometry of the Lorentz force in strong mid-infrared laser fields Pisanty, Emilio; Hickstein, Daniel; Galloway, Benjamin R. Humboldt-Universität zu Berlin https://doi.org/10.18452/24377	text	January 2018
Roadmap of ultrafast x-ray atomic and molecular physics Young, Linda; Ueda, Kiyoshi; Gühr, Markus Universität Potsdam https://doi.org/10.25932/publishup-42423	text	January 2019
Ellipticity dependence of high-harmonic generation in solids originating from coupled intraband and interband dynamics Tancogne-Dejean, Nicolas; Muecke, Oliver; Kärtner, Franz X. Deutsches Elektronen-Synchrotron, DESY, Hamburg https://doi.org/10.3204/pubdb-2017-11098	text	January 2017
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Roadmap of ultrafast x-ray atomic and molecular physics Young, Linda; Ueda, Kiyoshi; Gühr, Markus Deutsches Elektronen-Synchrotron, DESY, Hamburg https://doi.org/10.3204/pubdb-2019-00875	text	January 2018
Polarization-state-resolved high-harmonic spectroscopy of solids Rossi, Giulio Maria; Yang, Y.; Scheiba, F. Deutsches Elektronen-Synchrotron, DESY, Hamburg https://doi.org/10.3204/pubdb-2019-01359	text	January 2019
Symphony on strong field approximation Amini, Kasra; Biegert, Jens; Calegari, Francesca Deutsches Elektronen-Synchrotron, DESY, Hamburg https://doi.org/10.3204/pubdb-2020-00145	text	January 2019
Bicircular High-Harmonic Spectroscopy Reveals Dynamical Symmetries of Atoms and Molecules Baykusheva, Denitsa; Sabbir, Ahsan, Md; Lin, Nan ETH Zurich https://doi.org/10.3929/ethz-a-010625328	text	January 2016
Perspectives of Attosecond Spectroscopy for the Understanding of Fundamental Electron Correlations Kraus, Peter M.; Wörner, Hans Jakob ETH Zurich https://doi.org/10.3929/ethz-b-000263942	text	January 2018
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A Rotating-Frame Perspective on High-Harmonic Generation of Circularly Polarized Light Reich, Daniel M.; Madsen, Lars Bojer arXiv https://doi.org/10.48550/arxiv.1602.07166	text	January 2016
Trajectory analysis of high-harmonic generation from periodic crystals Ikemachi, Takuya; Shinohara, Yasushi; Sato, Takeshi arXiv https://doi.org/10.48550/arxiv.1611.08033	text	January 2016
Nanoscale Magnetic Imaging using Circularly Polarized High-Harmonic Radiation Kfir, Ofer; Zayko, Sergey; Nolte, Christina arXiv https://doi.org/10.48550/arxiv.1706.07695	preprint	January 2017
Signatures of electronic structure in bi-circular high-harmonic spectroscopy Baykusheva, Denitsa; Brennecke, Simon; Lein, Manfred arXiv https://doi.org/10.48550/arxiv.1710.04474	text	January 2017
Dynamical synchronization transition in interacting electron systems Nag, Tanay; Slager, Robert-Jan; Higuchi, Takuya arXiv https://doi.org/10.48550/arxiv.1802.02161	text	January 2018
Control of attosecond light polarization in two-color bi-circular fields Jiménez-Galán, Álvaro; Zhavoronkov, Nick; Ayuso, David arXiv https://doi.org/10.48550/arxiv.1805.02250	text	January 2018
Spin constrained orbital angular momentum control in high-harmonic generation Kong, F.; Zhang, C.; Larocque, H. arXiv https://doi.org/10.48550/arxiv.1810.05894	text	January 2018
$R$-matrix with Time-dependence Theory for Ultrafast Atomic Processes in Arbitrary Light Fields Clarke, D. D. A.; Armstrong, G. S. J.; Brown, A. C. arXiv https://doi.org/10.48550/arxiv.1812.00234	text	January 2018
Controlling Sub-Cycle Optical Chirality in the Photoionization of Chiral Molecules Rozen, Shaked; Comby, Antoine; Bloch, Etienne arXiv https://doi.org/10.48550/arxiv.1906.11325	preprint	January 2019
Electron rotational asymmetry in strong-field photodetachment from F$^-$ by circularly polarized laser pulses Armstrong, G. S. J.; Clarke, D. D. A.; Brown, A. C. arXiv https://doi.org/10.48550/arxiv.1911.00290	text	January 2019
Modeling tomographic measurements of photoelectron vortices in counter-rotating circularly polarized laser pulses Armstrong, G. S. J.; Clarke, D. D. A.; Benda, J. arXiv https://doi.org/10.48550/arxiv.1912.08133	text	January 2019