Factors controlling the oxygen isotopic composition of lacustrine authigenic carbonates in Western China: implications for paleoclimate reconstructions

Li, Huashu; Liu, Xingqi; Tripati, Aradhna; Feng, Shengnan; Elliott, Ben; Whicker, Chloe; Arnold, Alexandrea; Kelley, Anne Marie

doi:10.1038/s41598-020-73422-4

Title: Factors controlling the oxygen isotopic composition of lacustrine authigenic carbonates in Western China: implications for paleoclimate reconstructions

Journal Article · Thu Oct 01 00:00:00 EDT 2020 · Scientific Reports

DOI:https://doi.org/10.1038/s41598-020-73422-4· OSTI ID:1669166

Li, Huashu; Liu, Xingqi; Tripati, Aradhna; Feng, Shengnan; Elliott, Ben; Whicker, Chloe; Arnold, Alexandrea; Kelley, Anne Marie

Abstract In the carbonate-water system, at equilibrium, the oxygen isotopic composition of carbonate is dependent not only on the temperature but also on the isotopic composition of host water in which the carbonate is formed. In this study, lake surface sediment and water samples were collected from 33 terminal lakes in Western China to evaluate controls on the oxygen isotopic composition of lacustrine authigenic carbonates (δ ¹⁸ O _carb ) and its spatial distribution. Our results show that water oxygen isotopic composition (δ ¹⁸ O _water ) rather than lake summer water temperature (T _water ), is the main determinant of δ ¹⁸ O _carb , irrespective of whether oxygen isotope equilibrium is achieved. There are significant linear correlations between δ ¹⁸ O _carb and elevation, as well as that between δ ¹⁸ O _carb and latitude for lakes located on the Tibetan Plateau. In Western China, the spatial distribution of δ ¹⁸ O _carb is consistent with that of δ ¹⁸ O _water , and is ultimately controlled by the isotopic composition of local precipitation (δ ¹⁸ O _{precipitation} ) that depends on the source of water vapor. Therefore, changes in δ ¹⁸ O _carb can be predominantly interpreted as variations of δ ¹⁸ O _water , which in turn represent changes in δ ¹⁸ O _{precipitation} for paleoclimate reconstructions in this region, and may be relevant to studies of other areas.

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Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); National Natural Science Foundation of China (NSFC); National Science Foundation (NSF)

Grant/Contract Number:: FG02-13ER16402; SC0010288; 41572338; EAR-1352212

OSTI ID:: 1669166

Alternate ID(s):: OSTI ID: 1816830

Journal Information:: Scientific Reports, Journal Name: Scientific Reports Vol. 10 Journal Issue: 1; ISSN 2045-2322

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United Kingdom

Language:: English

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Title: Factors controlling the oxygen isotopic composition of lacustrine authigenic carbonates in Western China: implications for paleoclimate reconstructions

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