Pseudocapacitance: From Fundamental Understanding to High Power Energy Storage Materials

Fleischmann, Simon; Mitchell, James B.; Wang, Ruocun; Zhan, Cheng; Jiang, De-en; Presser, Volker; Augustyn, Veronica

doi:10.1021/acs.chemrev.0c00170

Pseudocapacitance: From Fundamental Understanding to High Power Energy Storage Materials

Journal Article · Sun Jun 28 00:00:00 EDT 2020 · Chemical Reviews

DOI:https://doi.org/10.1021/acs.chemrev.0c00170· OSTI ID:1650460

^[1]; Mitchell, James B. ^[1]; Wang, Ruocun ^[1]; Zhan, Cheng ^[2]; ^[3]; ^[4]; ^[1]

North Carolina State Univ., Raleigh, NC (United States)
Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Univ. of California, Riverside, CA (United States)
Leibniz Inst. for New Materials (INM), Saarbrucken (Germany); Saarland Univ., Saarbrucken (Germany)

There is an urgent global need for electrochemical energy storage that includes materials that can provide simultaneous high power and high energy density. One strategy to achieve this goal is with pseudocapacitive materials that take advantage of reversible surface or near-surface Faradaic reactions to store charge, surpassing the capacity limitations of electrical double-layer capacitors and mass transfer limitations of batteries. The past decade has seen tremendous growth in the understanding of pseudocapacitance as well as materials that exhibit this phenomenon. The purpose of this study is to examine the fundamental development of the concept of pseudocapacitance and how it came to prominence in electrochemical energy storage as well as to describe new classes of materials whose electrochemical energy storage behavior can be described as pseudocapacitive.

View Accepted Manuscript (DOE)

Research Organization:: Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)

Sponsoring Organization:: National Science Foundation (NSF); USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC52-07NA27344

OSTI ID:: 1650460

Report Number(s):: LLNL-JRNL--807161; 1010798

Journal Information:: Chemical Reviews, Journal Name: Chemical Reviews Journal Issue: 14 Vol. 120; ISSN 0009-2665

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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