Functional metal–organic frameworks as effective sensors of gases and volatile compounds

Li, Hai-Yang; Zhao, Shu-Na; Zang, Shuang-Quan; Li, Jing

doi:10.1039/c9cs00778d

Title: Functional metal–organic frameworks as effective sensors of gases and volatile compounds

Journal Article · Tue Aug 04 00:00:00 EDT 2020 · Chemical Society Reviews

DOI:https://doi.org/10.1039/c9cs00778d· OSTI ID:1646891

Li, Hai-Yang ^[1]; Zhao, Shu-Na ^[1];

^[1];

^[2]

Zhengzhou University (China)
Rutgers Univ., Piscataway, NJ (United States)

Developing efficient sensor materials with superior performance for selective, fast and sensitive detection of gases and volatile organic compounds (VOCs) is essential for human health and environmental protection, through monitoring indoor and outdoor air pollutions, managing industrial processes, controlling food quality and assisting early diagnosis of diseases. Metal–organic frameworks (MOFs) are a unique type of crystalline and porous solid material constructed from metal nodes (metal ions or clusters) and functional organic ligands. They have been investigated extensively for possible use as high performance sensors for the detection of many different gases and VOCs in recent years, due to their large surface area, tunable pore size, functionalizable sites and intriguing properties, such as electrical conductivity, magnetism, ferroelectricity, luminescence and chromism. The high porosity of MOFs allows them to interact strongly with various analytes, including gases and VOCs, thus resulting in easily measurable responses to different physicochemical parameters. Although much of the recent work on MOF-based luminescent sensors have been summarized in several excellent reviews (up to 2018), a comprehensive overview of these materials for sensing gases and VOCs based on chemiresistive, magnetic, ferroelectric, and colorimertic mechanisms is missing. In this review, we highlight the most recent progress in developing MOF sensing and switching materials with an emphasis on sensing mechanisms based on electricity, magnetism, ferroelectricity and chromism. We provide a comprehensive analysis on the MOF–analyte interactions in these processes, which play a key role in the sensing performance of the MOF-based sensors and switches. We discuss in detail possible applications of MOF-based sensing and switching materials in detecting oxygen, water vapor, toxic industrial gases (such as hydrogen sulfide, ammonia, sulfur dioxide, nitrous oxide, carbon oxides and carbon disulfide) and VOCs (such as aromatic and aliphatic hydrocarbons, ketones, alcohols, aldehydes, chlorinated hydrocarbons and N,N'-dimethylformamide). Altogether, this review serves as a timely source of information and provides insight for the future development of advanced MOF materials as next-generation gas and VOC sensors.

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Research Organization:: Rutgers Univ., Piscataway, NJ (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0019902

OSTI ID:: 1646891

Alternate ID(s):: OSTI ID: 1644724

Journal Information:: Chemical Society Reviews, Vol. 49, Issue 17; ISSN 0306-0012

Publisher:: Royal Society of ChemistryCopyright Statement

Country of Publication:: United States

Language:: English

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A dual-emission probe to detect moisture and water in organic solvents based on green-Tb ³⁺ post-coordinated metal–organic frameworks with red carbon dots Wu, Jing-Xing; Yan, Bing Dalton Transactions, Vol. 46, Issue 21 https://doi.org/10.1039/C7DT01352C	journal	January 2017
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Copper(I) Metal–Organic Framework: Visual Sensor for Detecting Small Polar Aliphatic Volatile Organic Compounds Yu, Yang; Ma, Jian-Ping; Zhao, Chao-Wei Inorganic Chemistry, Vol. 54, Issue 24 https://doi.org/10.1021/acs.inorgchem.5b02150	journal	December 2015
Layer-structured lanthanide coordination polymers constructed from 3,5-bis(3,5-dicarboxylphenyl)-pyridine ligand as fluorescent probe for nitroaromatics and metal ions Shi, Xiangxiang; Fan, Yong; Xu, Jianing Inorganica Chimica Acta, Vol. 483 https://doi.org/10.1016/j.ica.2018.08.050	journal	November 2018
Single-Phase White-Light-Emitting and Photoluminescent Color-Tuning Coordination Assemblies Pan, Mei; Liao, Wei-Ming; Yin, Shao-Yun Chemical Reviews, Vol. 118, Issue 18 https://doi.org/10.1021/acs.chemrev.8b00222	journal	August 2018
Ratiometric Fluorescence Sensing and Real-Time Detection of Water in Organic Solvents with One-Pot Synthesis of Ru@MIL-101(Al)–NH ₂ Yin, Hua-Qing; Yang, Ji-Chun; Yin, Xue-Bo Analytical Chemistry, Vol. 89, Issue 24 https://doi.org/10.1021/acs.analchem.7b03723	journal	November 2017
Composite materials combining multiple luminescent MOFs and superparamagnetic microparticles for ratiometric water detection Wehner, T.; Seuffert, M. T.; Sorg, J. R. Journal of Materials Chemistry C, Vol. 5, Issue 39 https://doi.org/10.1039/C7TC03312E	journal	January 2017
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A portable self-calibrating logic detector for gradient detection of formaldehyde based on luminescent metal organic frameworks Zhang, Yu; Yan, Bing Journal of Materials Chemistry C, Vol. 7, Issue 19 https://doi.org/10.1039/C9TC01288E	journal	January 2019
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Aqueous phase nitric oxide detection by an amine-decorated metal–organic framework Desai, Aamod V.; Samanta, Partha; Manna, Biplab Chemical Communications, Vol. 51, Issue 28 https://doi.org/10.1039/C5CC00773A	journal	January 2015
High-mobility band-like charge transport in a semiconducting two-dimensional metal–organic framework Dong, Renhao; Han, Peng; Arora, Himani Nature Materials, Vol. 17, Issue 11 https://doi.org/10.1038/s41563-018-0189-z	journal	October 2018
Gas sensing using porous materials for automotive applications Wales, Dominic J.; Grand, Julien; Ting, Valeska P. Chemical Society Reviews, Vol. 44, Issue 13 https://doi.org/10.1039/C5CS00040H	journal	January 2015
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State of the Art and Prospects in Metal–Organic Framework (MOF)-Based and MOF-Derived Nanocatalysis Wang, Qi; Astruc, Didier Chemical Reviews, Vol. 120, Issue 2 https://doi.org/10.1021/acs.chemrev.9b00223	journal	June 2019
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Transition-metal-based (Zn2+ and Cd2+) metal-organic frameworks as fluorescence “turn-off” sensors for highly sensitive and selective detection of hydrogen sulfide Yang, Xu-Feng; Zhu, Hai-Bin; Liu, Min Inorganica Chimica Acta, Vol. 466 https://doi.org/10.1016/j.ica.2017.06.067	journal	September 2017
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New Porous Crystals of Extended Metal-Catecholates Hmadeh, Mohamad; Lu, Zheng; Liu, Zheng Chemistry of Materials, Vol. 24, Issue 18, p. 3511-3513 https://doi.org/10.1021/cm301194a	journal	August 2012
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Turn-On Luminescence Sensing and Real-Time Detection of Traces of Water in Organic Solvents by a Flexible Metal-Organic Framework Douvali, Antigoni; Tsipis, Athanassios C.; Eliseeva, Svetlana V. Angewandte Chemie International Edition, Vol. 54, Issue 5 https://doi.org/10.1002/anie.201410612	journal	December 2014

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