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Macroscopically aligned carbon nanotubes for flexible and high-temperature electronics, optoelectronics, and thermoelectrics

Journal Article · · Journal of Physics. D, Applied Physics

The remarkable flexibility, stable chemical structure, and extraordinary thermal, electrical, and optical properties of carbon nanotubes (CNTs) are promising for a variety of applications in flexible and/or high-temperature electronics, optoelectronics, and thermoelectrics, including wearables, refractory photonics, and waste heat harvesting. However, the long-standing problem in the preparation of CNT ensembles is to maintain the extraordinary properties of individual CNTs on a macroscopic scale; the polydispersity and randomness remain two main challenges. In this topical review, we will discuss three ways of creating wafer-scale aligned CNTs: direct growth of aligned CNTs by chemical vapor deposition, production of ultrahigh- conductivity CNT fibers through solution spinning and coating, and spontaneous formation of wafer-scale aligned CNT films via controlled vacuum filtration. Here, we will then describe flexible and high-temperature applications of these materials, such as flexible CNT broadband detectors, flexible strain sensors, spectrally selective thermal emitters, and thermoelectric devices.

Research Organization:
Rice Univ., Houston, TX (United States)
Sponsoring Organization:
USDOE Office of Energy Efficiency and Renewable Energy (EERE), Energy Efficiency Office. Advanced Manufacturing Office; USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation; Robert A. Welch Foundation
Grant/Contract Number:
EE0007865; FG02-06ER46308
OSTI ID:
1638468
Alternate ID(s):
OSTI ID: 23015342
Journal Information:
Journal of Physics. D, Applied Physics, Journal Name: Journal of Physics. D, Applied Physics Journal Issue: 6 Vol. 53; ISSN 0022-3727
Publisher:
IOP PublishingCopyright Statement
Country of Publication:
United States
Language:
English

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