Unusual Dynamic Charge Correlations in Simple-Tetragonal HgBa 2 CuO 4 + δ

Yu, B.; Tabis, W.; Bialo, I.; Yakhou, F.; Brookes, N. B.; Anderson, Z.; Tang, Y.; Yu, G.; Greven, M.

doi:10.1103/PhysRevX.10.021059

Title: Unusual Dynamic Charge Correlations in Simple-Tetragonal ${HgBa}_{2} {CuO}_{4 + δ}$

Journal Article · Tue Jun 16 00:00:00 EDT 2020 · Physical Review. X

DOI:https://doi.org/10.1103/PhysRevX.10.021059· OSTI ID:1633499

Yu, B.;

;

; Yakhou, F.; Brookes, N. B.;

; Tang, Y.; Yu, G.; Greven, M.

The charge-density-wave (CDW) instability in the underdoped, pseudogap part of the cuprate phase diagram has been a major recent research focus, yet measurements of dynamic, energy-resolved charge correlations are still in their infancy. Such information is crucial in order to help discern the connection between CDW and pseudogap phenomena, and to understand the extent to which charge correlations in general shape the phase diagram. We report a resonant inelastic x-ray scattering study of the underdoped cuprate superconductor HgBa₂CuO_4+δ (T_c = 70 K). At 250 K, above the previously established temperature T_CDW ≈ 200 K that signifies the onset of quasistatic short-range CDW order, we observe significant dynamic correlations that are broadly peaked at about 40 meV and centered at the two- dimensional wave vector q_CDW. This energy scale is comparable to both the superconducting gap and the low-energy pseudogap. At 70 K, we observe a quasistatic CDW peak at q_CDW, but the dynamic correlations around 40 meV remain virtually unchanged, and we identify a new feature: dynamic correlations well above the optic phonon range that are broadly peaked in the 150–200 meV range. A similar energy scale was previously identified in other experiments as a high-energy pseudogap. The observation of three distinct features in the charge response is highly unusual for a CDW system and suggests that charge order in the cuprates is complex. We demonstrate that other single-layer cuprates exhibit approximately the same relative strength of high- to low-temperature energy-integrated charge signal, which points to the universal existence of significant dynamic correlations. Intriguingly, the two energy scales identified here are also comparable to those of the superconducting glue function extracted from other spectroscopic techniques, consistent with a dual charge and magnetic nature of the pairing glue. We further determine the paramagnon dispersion along [1, 0], across q_CDW, and find it to be consistent with magnetic excitations measured by inelastic neutron scattering. Unlike for some other cuprates, our result points to the absence of a discernible coupling between charge and magnetic excitations.

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Research Organization:: Univ. of Minnesota, Minneapolis, MN (United States)

Sponsoring Organization:: USDOE; USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division; National Science Centre

Grant/Contract Number:: SC0016371; UMO-2019/32/T/ST3/0019

OSTI ID:: 1633499

Alternate ID(s):: OSTI ID: 1656783

Journal Information:: Physical Review. X, Journal Name: Physical Review. X Vol. 10 Journal Issue: 2; ISSN 2160-3308

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 22 works

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Universal superconducting precursor in three classes of unconventional superconductors Pelc, D.; Anderson, Z.; Yu, B. Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-10635-w	journal	June 2019
Universal quantum oscillations in the underdoped cuprate superconductors Barišić, Neven; Badoux, Sven; Chan, Mun K. Nature Physics, Vol. 9, Issue 12 https://doi.org/10.1038/nphys2792	journal	November 2013

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Title: Unusual Dynamic Charge Correlations in Simple-Tetragonal ${HgBa}_{2} {CuO}_{4 + δ}$