Dynamics of correlation-frozen antinodal quasiparticles in superconducting cuprates

Cilento, Federico; Manzoni, Giulia; Sterzi, Andrea; Peli, Simone; Ronchi, Andrea; Crepaldi, Alberto; Boschini, Fabio; Cacho, Cephise; Chapman, Richard; Springate, Emma; Eisaki, Hiroshi; Greven, Martin; Berciu, Mona; Kemper, Alexander F.; Damascelli, Andrea; Capone, Massimo; Giannetti, Claudio; Parmigiani, Fulvio

doi:10.1126/sciadv.aar1998

Dynamics of correlation-frozen antinodal quasiparticles in superconducting cuprates

Journal Article · Fri Feb 23 00:00:00 EST 2018 · Science Advances

DOI:https://doi.org/10.1126/sciadv.aar1998· OSTI ID:1625984

^[1]; Manzoni, Giulia ^[2]; ^[2]; ^[3]; Ronchi, Andrea ^[4]; Crepaldi, Alberto ^[5]; Boschini, Fabio ^[6]; ^[7]; Chapman, Richard ^[7]; ^[7]; Eisaki, Hiroshi ^[8]; Greven, Martin ^[9]; Berciu, Mona ^[6]; ^[10]; Damascelli, Andrea ^[6]; ^[11]; ^[3]; Parmigiani, Fulvio ^[12]

Elettra-Sincrotrone Trieste, Basovizza (Italy); DOE/OSTI
Elettra-Sincrotrone Trieste, Basovizza (Italy); Univ. degli Studi di Trieste (Italy). Dipartimento di Fisica
Univ. Cattolica del Sacro Cuore, Brescia (Italy). Interdisciplinary Labs. for Advanced Materials Physics
Univ. Cattolica del Sacro Cuore, Brescia (Italy). Interdisciplinary Labs. for Advanced Materials Physics; Katholieke Univ. Leuven, Heverlee (Belgium). Dept. of Physics and Astronomy
Ecole Polytechnique Federale Lausanne (Switzlerland). Inst. of Physics
Univ. of British Columbia, Vancouver, BC (Canada). Dept. of Physics and Astronomy; Univ. of British Columbia, Vancouver, BC (Canada). Quantum Matter Inst.
Harwell Science and Innovation Campus, Didcot (United Kingdom). CLF-Artemis@Rutherford Appleton Lab.
National Inst. of Advanced Industrial Science and Technology (AIST), Tsukuba (Japan). Nanoelectronics Research Inst.
Univ. of Minnesota, Minneapolis, MN (United States). School of Physics and Astronomy
North Carolina State Univ., Raleigh, NC (United States). Dept. of Physics
National Simulation Center, Trieste (Italy). Scuola Internazionale Superiore di Studi Avanzati (SISSA) and Consiglio Nazionale delle Ricerche–Istituto Officina dei Materiali (CNR-IOM) Democritos
Elettra-Sincrotrone Trieste, Basovizza (Italy); Univ. degli Studi di Trieste (Italy). Dipartimento di Fisica; Univ. of Cologne (Germany). International Faculty

Many puzzling properties of high–critical temperature (T_c) superconducting (HTSC) copper oxides have deep roots in the nature of the antinodal quasiparticles, the elementary excitations with wave vector parallel to the Cu–O bonds. These electronic states are most affected by the onset of antiferromagnetic correlations and charge instabilities, and they host the maximum of the anisotropic superconducting gap and pseudogap. We use time-resolved extremeultraviolet photoemission with proper photon energy (18 eV) and time resolution (50 fs) to disclose the ultrafast dynamics of the antinodal states in a prototypical HTSC cuprate. After photoinducing a nonthermal charge redistribution within the Cu and O orbitals, we reveal a dramatic momentum-space differentiation of the transient electron dynamics. Whereas the nodal quasiparticle distribution is heated up as in a conventional metal, new quasiparticle states transiently emerge at the antinodes, similarly to what is expected for a photoexcited Mott insulator, where the frozen charges can be released by an impulsive excitation. This transient antinodal metallicity is mapped into the dynamics of the O-2p bands, thus directly demonstrating the intertwining between the lowand high-energy scales that is typical of correlated materials. Our results suggest that the correlation-driven freezing of the electrons moving along the Cu–O bonds, analogous to the Mott localization mechanism, constitutes the starting point for any model of high-T_c superconductivity and other exotic phases of HTSC cuprates.

View Accepted Manuscript (DOE)

Research Organization:: SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)

Sponsoring Organization:: Alfred P. Sloan; Canada First Research Excellence Fund (CFREF); Canada Foundation for Innovation (CFI); Canada Research Chairs Program; European Union’s Horizon 2020; Killam; LASERLAB-EUROPE; Natural Sciences and Engineering Research Council of Canada (NSERC); Swiss National Science Foundation (SNF); USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC02-76SF00515

OSTI ID:: 1625984

Journal Information:: Science Advances, Journal Name: Science Advances Journal Issue: 2 Vol. 4; ISSN 2375-2548

Publisher:: AAASCopyright Statement

Country of Publication:: United States

Language:: English

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