Exfoliated MoS2 Sheets and Reduced Graphene Oxide-An Excellent and Fast Anode for Sodium-ion Battery

Sahu, Tuhin Subhra; Mitra, Sagar

doi:10.1038/srep12571

Exfoliated MoS₂ Sheets and Reduced Graphene Oxide-An Excellent and Fast Anode for Sodium-ion Battery

Journal Article · Tue Jul 28 00:00:00 EDT 2015 · Scientific Reports

DOI:https://doi.org/10.1038/srep12571· OSTI ID:1624786

Sahu, Tuhin Subhra ^[1]; Mitra, Sagar ^[2]

Indian Inst. of Technology Bombay (IITB), Mumbai (India); DOE/OSTI
Indian Inst. of Technology Bombay (IITB), Mumbai (India)

Three dimensional (3D) MoS₂ nanoflowers are successfully synthesized by hydrothermal method. Further, a composite of as prepared MoS₂ nanoflowers and rGO is constructed by simple ultrasonic exfoliation technique. The crystallography and morphological studies have been carried out by XRD, FE-SEM, TEM, HR-TEM and EDS etc. Here, XRD study revealed, a composite of exfoliated MoS₂ with expanded spacing of (002) crystal plane and rGO can be prepared by simple 40 minute of ultrasonic treatment. While, FE-SEM and TEM studies depict, individual MoS₂ nanoflowers with an average diameter of 200 nm are uniformly distributed throughout the rGO surface. When tested as sodium-ion batteries anode material by applying two different potential windows, the composite demonstrates a high reversible specific capacity of 575 mAhg^-1 at 100 mAg^-1 in between 0.01 V–2.6 V and 218 mAhg^-1 at 50 mAg^-1 when discharged in a potential range of 0.4 V–2.6 V. As per our concern, the results are one of the best obtained as compared to the earlier published one on MoS₂ based SIB anode material and more importantly this material shows such an excellent reversible Na-storage capacity and good cycling stability without addition of any expensive additive stabilizer, like fluoroethylene carbonate (FEC), in comparison to those in current literature.

View Accepted Manuscript (DOE)

Research Organization:: National Renewable Energy Laboratory (NREL), Golden, CO (United States)

Sponsoring Organization:: Ministry of New and Renewable Energy (MNRE); USDOE Office of Energy Efficiency and Renewable Energy (EERE); USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC36-08GO28308

OSTI ID:: 1624786

Journal Information:: Scientific Reports, Journal Name: Scientific Reports Journal Issue: 1 Vol. 5; ISSN 2045-2322

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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