Long-life Li/polysulphide batteries with high sulphur loading enabled by lightweight three-dimensional nitrogen/sulphur-codoped graphene sponge

Zhou, Guangmin; Paek, Eunsu; Hwang, Gyeong S.; Manthiram, Arumugam

doi:10.1038/ncomms8760

Title: Long-life Li/polysulphide batteries with high sulphur loading enabled by lightweight three-dimensional nitrogen/sulphur-codoped graphene sponge

Journal Article · Fri Jul 17 00:00:00 EDT 2015 · Nature Communications

DOI:https://doi.org/10.1038/ncomms8760· OSTI ID:1623994

Zhou, Guangmin ^[1]; Paek, Eunsu ^[1]; Hwang, Gyeong S. ^[1]; Manthiram, Arumugam ^[1]

Univ. of Texas, Austin, TX (United States)

Lithium–sulphur batteries with a high theoretical energy density are regarded as promising energy storage devices for electric vehicles and large-scale electricity storage. However, the low active material utilization, low sulphur loading and poor cycling stability restrict their practical applications. Herein, we present an effective strategy to obtain Li/polysulphide batteries with high-energy density and long-cyclic life using three-dimensional nitrogen/sulphur codoped graphene sponge electrodes. The nitrogen/sulphur codoped graphene sponge electrode provides enough space for a high sulphur loading, facilitates fast charge transfer and better immobilization of polysulphide ions. The hetero-doped nitrogen/sulphur sites are demonstrated to show strong binding energy and be capable of anchoring polysulphides based on first-principles calculations. As a result, a high specific capacity of 1,200 mAh g^–1 at 0.2C rate, a high-rate capacity of 430 mAh g^–1 at 2C rate and excellent cycling stability for 500 cycles with ~0.078% capacity decay per cycle are achieved.

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Research Organization:: Ceramatec, Inc., West Valley City, UT (United States

Sponsoring Organization:: USDOE Advanced Research Projects Agency - Energy (ARPA-E); Robert A. Welch Foundation

Grant/Contract Number:: AR0000377; F-1535

OSTI ID:: 1623994

Journal Information:: Nature Communications, Vol. 6, Issue 1; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 868 works

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Sulfur–nitrogen co-doped porous carbon nanosheets to control lithium growth for a stable lithium metal anode Chen, Mei; Zheng, Jianhui; Sheng, Ouwei Journal of Materials Chemistry A, Vol. 7, Issue 31 https://doi.org/10.1039/c9ta05684j	journal	January 2019
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3D Ferroconcrete-Like Aminated Carbon Nanotubes Network Anchoring Sulfur for Advanced Lithium–Sulfur Battery Yan, M.; Chen, H.; Yu, Y. Apollo - University of Cambridge Repository https://doi.org/10.17863/cam.26943	text	January 2018
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Chem-Bonding and Phys-Trapping Se Electrode for Long-Life Rechargeable Batteries Wu, Tianjing; Ding, Zhiying; Jing, Mingjun Advanced Functional Materials, Vol. 29, Issue 9 https://doi.org/10.1002/adfm.201809014	journal	January 2019
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Rational Design of Binders for Stable Li‐S and Na‐S Batteries Guo, Qianyi; Zheng, Zijian Advanced Functional Materials, Vol. 30, Issue 6 https://doi.org/10.1002/adfm.201907931	journal	December 2019
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Recent Progress in the Design of Advanced Cathode Materials and Battery Models for High-Performance Lithium-X (X = O ₂ , S, Se, Te, I ₂ , Br ₂ ) Batteries Xu, Jiantie; Ma, Jianmin; Fan, Qinghua Advanced Materials, Vol. 29, Issue 28 https://doi.org/10.1002/adma.201606454	journal	May 2017
A Top-Down Strategy toward SnSb In-Plane Nanoconfined 3D N-Doped Porous Graphene Composite Microspheres for High Performance Na-Ion Battery Anode Qin, Jian; Wang, Tianshuai; Liu, Dongye Advanced Materials, Vol. 30, Issue 9 https://doi.org/10.1002/adma.201704670	journal	January 2018
Simultaneous Suppression of the Dendrite Formation and Shuttle Effect in a Lithium-Sulfur Battery by Bilateral Solid Electrolyte Interface Fan, Ling; Chen, Suhua; Zhu, Jingyi Advanced Science, Vol. 5, Issue 9 https://doi.org/10.1002/advs.201700934	journal	July 2018
Polysulfide-Shuttle Control in Lithium-Sulfur Batteries with a Chemically/Electrochemically Compatible NaSICON-Type Solid Electrolyte Yu, Xingwen; Bi, Zhonghe; Zhao, Feng Advanced Energy Materials, Vol. 6, Issue 24 https://doi.org/10.1002/aenm.201601392	journal	August 2016
Hierarchical Structures Based on Two-Dimensional Nanomaterials for Rechargeable Lithium Batteries Cong, Lina; Xie, Haiming; Li, Jinghong Advanced Energy Materials, Vol. 7, Issue 12 https://doi.org/10.1002/aenm.201601906	journal	January 2017
Bi ₂ S ₃ /Ketjen Black as a Highly Efficient Bifunctional Catalyst for Long‐Cycle Lithium‐Oxygen Batteries Xu, Peng; Zhu, Jiajia; Chen, Congdi ChemElectroChem, Vol. 6, Issue 15 https://doi.org/10.1002/celc.201900191	journal	May 2019
Few‐Layer Boron Nitride with Engineered Nitrogen Vacancies for Promoting Conversion of Polysulfide as a Cathode Matrix for Lithium–Sulfur Batteries Yi, Yikun; Li, Hongping; Chang, Honghong Chemistry – A European Journal, Vol. 25, Issue 34 https://doi.org/10.1002/chem.201900884	journal	May 2019
Electrospun zeolitic imidazolate framework-derived nitrogen-doped carbon nanofibers with high performance for lithium-sulfur batteries Yao, Shanshan; Xue, Sikang; Peng, Sihuang International Journal of Energy Research, Vol. 43, Issue 5 https://doi.org/10.1002/er.4389	journal	February 2019
N-doped Mesoporous Carbon/Graphene Aerogels as Sulfur Hosts for High-Performance Lithium-Sulfur Batteries Li, Zhengzheng; Tan, Yingbin ChemistrySelect, Vol. 3, Issue 16 https://doi.org/10.1002/slct.201800704	journal	April 2018
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